Ultrafast Self-Induced X-Ray Transparency and Loss of Magnetic Diffraction

• Published in: Physical review letters Vol. 121; no. 13
• Main Authors: Chen, Z., Higley, D. J., Beye, M., Hantschmann, M., Mehta, V., Hellwig, O., Mitra, A., Bonetti, S., Bucher, M., Carron, S., Chase, T., Jal, E., Kukreja, R., Liu, T., Reid, A. H., Dakovski, G. L., Föhlisch, A., Schlotter, W. F., Dürr, H. A., Stöhr, J.
• Format: Journal Article
• Language: English
• Published: United States American Physical Society (APS) 28-09-2018
• Subjects: ATOMIC AND MOLECULAR PHYSICS
• ISSN: 0031-9007; 1079-7114

Using ultrafast ≃2.5 fs and ≃25 fs self-amplified spontaneous emission pulses of increasing intensity and a novel experimental scheme, we report the concurrent increase of stimulated emission in the forward direction and loss of out-of-beam diffraction contrast for a Co/Pd multilayer sample. The experimental results are quantitatively accounted for by a statistical description of the pulses in conjunction with the optical Bloch equations. Here, the dependence of the stimulated sample response on the incident intensity, coherence time, and energy jitter of the employed pulses reveals the importance of increased control of x-ray free electron laser radiation.