Nonmagnetic Sn doping effect on the electronic and magnetic properties of antiferromagnetic topological insulator MnBi2Te4

• Published in: Physica. B, Condensed matter Vol. 657
• Main Authors: Changdar, Susmita, Ghosh, Susanta, Vijay, Kritika, Kar, Indrani, Routh, Sayan, Maheshwari, P.K., Ghorai, Soumya, Banik, Soma, Thirupathaiah, S.
• Format: Journal Article
• Language: English
• Published: Elsevier B.V 15-05-2023
• Subjects: Anomalous Hall effect; Antiferromagnetic ordering; Magnetic topological insulator; Mn1-xSnxBi2Te4; Single crystals; Transport properties; Anomalous Hall effect; Single crystals; Antiferromagnetic ordering; Mn1-xSnxBi2Te4; Transport properties; Magnetic topological insulator
• ISSN: 0921-4526; 1873-2135
• DOI: 10.1016/j.physb.2023.414799

We investigated the effect of nonmagnetic Sn doping on the electronic and magnetic properties of antiferromagnetic topological insulator MnBi2Te4. We observe that the Sn doping reduces out-of-plane antiferromagnetic (AFM) interactions in Mn1−xSnxBi2Te4 for up to 68% of Sn concentration and above, the system is found to be a paramagnetic. In this way, the anomalous Hall effect observed at a very high critical field of 7.8 T in MnBi2Te4 is reduced to 2 T at 68% of Sn doping. Electrical transport measurements suggest that all compositions are metallic in nature, while the low temperature resistivity is sensitive to the AFM ordering and to the doping-induced disorder. Hall effect study demonstrates that Sn actually dopes electrons into the system, thus, enhancing the electron carrier density almost by two orders at 68% of Sn. In contrast, SnBi2Te4 is found to be a p-type metal. Angle-resolved photoemission spectroscopy (ARPES) studies show that the topological properties are intact at least up to 55% of Sn doping as the Dirac surface states are present near the Fermi level. But in SnBi2Te4 we are unable to detect the surface states due to heavy hole doping. Thus, the Sn doping significantly affects the electronic and magnetic properties of MnBi2Te4.
•AHE observed at 7.8 T in MnBi2Te4 is reduced to 2.2 T by 68% of Sn doping.•By 68% Sn doping, the electron density enhances almost by two orders.•Further Sn doping decreases electron density, making SnBi2Te4 a p-type system.•The ARPES data confirm Dirac surface states are intact at least up to 55% Sn doping.•Topological states in SnBi2Te4 could not be detected due to heavy hole doping.•AFM ordering is highly sensitive to the Sn concentration.