Stress enhancement in the delayed yielding of colloidal gels
Networks of aggregated colloidal particles are solidlike and can sustain an applied shear stress while exhibiting little or no creep; however, ultimately they will catastrophically fail. We show that the time delay for this yielding decreases in two distinct exponential regimes with applied stress....
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Published in: | Physical review letters Vol. 106; no. 24; p. 248303 |
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Main Authors: | , , , |
Format: | Journal Article |
Language: | English |
Published: |
United States
17-06-2011
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Subjects: | |
Online Access: | Get full text |
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Summary: | Networks of aggregated colloidal particles are solidlike and can sustain an applied shear stress while exhibiting little or no creep; however, ultimately they will catastrophically fail. We show that the time delay for this yielding decreases in two distinct exponential regimes with applied stress. This behavior is universal and found for a variety of colloidal gel systems. We present a bond-rupture model that quantitatively describes this behavior and highlights the role of mesoscopic structures. Our result gives new insight into the nature of yielding in these soft solid materials. |
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Bibliography: | ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 |
ISSN: | 0031-9007 1079-7114 1079-7114 |
DOI: | 10.1103/physrevlett.106.248303 |