Greatly amplified spontaneous emission of colloidal quantum dots mediated by a dielectric-plasmonic hybrid nanoantenna

• Published in: Nanophotonics (Berlin, Germany) Vol. 8; no. 12; pp. 2313 - 2319
• Main Authors: Yang, Guoce, Niu, Yijie, Wei, Hong, Bai, Benfeng, Sun, Hong-Bo
• Format: Journal Article
• Language: English
• Published: Berlin De Gruyter 13-11-2019; Walter de Gruyter GmbH
• Subjects: Core loss; Decay rate; Dielectric strength; Emissions control; Emitters; Energy harvesting; Far fields; Field emission; Light emission; nanoantenna; Nanoantennas; Nanoparticles; Optical communication; Photon density; plasmonics; Polaritons; Purcell effect; Quantum dots; Quantum efficiency; silicon nanoparticle; Spontaneous emission; Wireless communications
• ISSN: 2192-8606; 2192-8614
• DOI: 10.1515/nanoph-2019-0332

Optical nanoantennas can efficiently harvest electromagnetic energy from nanoscale space and boost the local radiation to the far field. The dielectric-metal nanogap is a novel design that can help to overcome the core issue of optical loss in all-metal nanostructures while enabling photon density of states larger than that in all-dielectric counterparts. This article reports that a crystalline spherical silicon nanoparticle on metal film (SiNPoM) nanoantenna can largely enhance the spontaneous emission intensity of quantum dots by an area-normalized factor of 69 and the decay rate by 42-fold compared with quantum dots on glass. A high total quantum efficiency of over 80%, including ~20% for far-field radiation and ~60% for surface plasmon polaritons, is obtained in simulation. Thanks to not only the low optical loss in dielectric nanoparticles but also the appropriate gap thickness which weakens the non-radiative decay due to the quenching from metal. Mie resonant modes additionally provide the flexible control of far-field emission patterns. Such a simple optical nanoantenna can be combined with various nanoscale optical emitters and easily extended to form large area metasurfaces functioning as active regions in light-emitting devices in applications such as advanced display, wireless optical communication, and quantum technology.