Self-Hybridized Vibrational-Mie Polaritons in Water Droplets

We study the self-hybridization between Mie modes supported by water droplets with stretching and bending vibrations in water molecules. Droplets with radii >2.7  μm are found to be polaritonic on the onset of the ultrastrong light-matter coupling regime. Similarly, the effect is observed in larg...

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Bibliographic Details
Published in:Physical review letters Vol. 132; no. 19; p. 193804
Main Authors: Canales, Adriana, Kotov, Oleg V, Küçüköz, Betül, Shegai, Timur O
Format: Journal Article
Language:English
Published: United States 10-05-2024
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Summary:We study the self-hybridization between Mie modes supported by water droplets with stretching and bending vibrations in water molecules. Droplets with radii >2.7  μm are found to be polaritonic on the onset of the ultrastrong light-matter coupling regime. Similarly, the effect is observed in larger deuterated water droplets at lower frequencies. Our results indicate that polaritonic states are ubiquitous and occur in water droplets in mists, fogs, and clouds. This finding may have implications not only for polaritonic physics but also for aerosol and atmospheric sciences.
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ISSN:0031-9007
1079-7114
1079-7114
DOI:10.1103/PhysRevLett.132.193804