Critical trajectories for aerosol particles: Their determination for impaction in fibrous filters and in oscillating bubbles

• Published in: Journal of aerosol science Vol. 69; pp. 98 - 112
• Main Authors: Clement, C.F., Dunnett, S.J.
• Format: Journal Article
• Language: English
• Published: Oxford Elsevier Ltd 01-03-2014; Elsevier
• Subjects: Aerosols; Chemistry; Colloidal state and disperse state; Exact sciences and technology; Fibrous filter; Filtration; General and physical chemistry; Numerical simulation; Particle deposition; Particle deposition; Numerical simulation; Filtration; Fibrous filter; Particle; Bubble; Filter; Aerosols; Trajectory; Deposition
• ISSN: 0021-8502; 1879-1964
• DOI: 10.1016/j.jaerosci.2013.12.004

Critical trajectories for aerosol particles in a gas flow are the ones which divide an aerosol flux into different parts, for example aerosol which is, and is not deposited. They can exist in all gas flows in which aerosol motion is governed by gas velocity rather than by diffusion and we describe two mathematical methods for their calculation. For deposition by impaction on a filter fibre it is necessary to solve the differential equations for particle motion and an efficient iterative procedure is used to obtain the critical trajectories.
Jonas and Schütz (1988) have shown that aerosol impaction is an important mechanism for the removal of aerosol from an oscillating sodium vapour bubble formed during a hypothetical core disruptive accident in a fast reactor. For these one-dimensional oscillations, when the gas velocity within a bubble is a linear function of position, we extend their work by calculating critical trajectories directly from the integral equation describing a depositing particle for two models with different initial conditions. With initially entrained uniform aerosol, the percentage impacted is independent of the inclusion of gravity in the calculations as long as regions empty of aerosol do not appear in the bubbles. Numerical results are obtained for a wide range of amplitudes of bubble oscillations and aerosol in the size range 1-30μm. In agreement with Jonas and Schütz, we find that a considerable fraction of the aerosol at larger sizes is removed by impaction. The theory is also shown to apply to other types of bubble oscillation including those of a spherical bubble.
•Critical trajectories divide trajectories in a given gas flow into different streams, e.g. for impaction or no impaction.•An efficient iterative procedure is given for finding the limiting trajectory for deposition on a fibre in a fibrous filter.•The procedure would be applicable for determining aerosol passage into the lungs.•The integral equation for the critical trajectory is solved directly for deposition in the time-dependent flow field within an oscillating bubble.•Calculations are performed for aerosol deposition in an oscillating bubble in the liquid sodium in a fast reactor.