Additive-manufactured anisotropic magnets for harsh environments

• Published in: Journal of magnetism and magnetic materials Vol. 586; p. 171165
• Main Authors: Podmiljšak, Benjamin, Kobe, Spomenka, Tomše, Tomaž, Bek, Marko, Kotnik, Tomaž, Slemenik Perše, Lidija, Žagar, Ema, Saje, Boris, Žužek, Kristina, Šturm, Sašo
• Format: Journal Article
• Language: English
• Published: Elsevier B.V 15-11-2023
• ISSN: 0304-8853
• DOI: 10.1016/j.jmmm.2023.171165

•Successful print of PPS filament mixed with Sr-ferrite in a commercially available material extrusion 3D printer.•Achieved full anisotropy printed magnetic material, just by using a permanent magnet for particle orientation.•3D printed magnetic materials using material extrusion can be used in harsh environments.
We describe the fabrication of SrFe12O19-based filaments, using polyphenylene sulphide (PPS) as the binder for the magnetic particles, and the subsequent printing of this filament with a 3D printer. PPS is an ideal polymer for applications in harsh environments, making it applicable for the automotive industry, where it is widely used with injection moulding. However, 3D printing this polymer introduces a major challenge. Because PPS is more difficult to extrude than polyamide, the filling factor in this study was set to 70 wt. %, which is lower than when used in injection moulding (close to 90 wt. %). The filament with a diameter of 2.75 mm was printed into a disk-shaped magnet with a diameter of 10 mm and a height of 4 mm using a HAGE 3D printer that uses a belt system for the filament extrusion. The magnets were printed onto a glass surface and onto a bulk Nd-Fe-B permanent magnet with an external magnetic field, parallel to the printer’s z-axis. Printing in the presence of a magnetic field was found to increase the magnet’s remanent magnetization by 61%, compared to an isotropic print. Without an external magnetic field we achieved a remanence of 23.9 emu/g for the 70 wt.% filling fraction, while when printing in a magnetic field, the value of the remanence improved to 39.7 emu/g because of the improved magnetic texture.