Time-resolved double ionization with few cycle laser pulses

Ionization of D2 launches a vibrational wave packet on the ground state of D+2. Removal of the second electron places a pair of D+ ions onto a Coulombic potential. Measuring the D+ kinetic energy determines the time delay between the first and the second ionization. Caught between a falling ionizati...

Full description

Saved in:
Bibliographic Details
Published in:Physical review letters Vol. 91; no. 9; p. 093002
Main Authors: Légaré, F, Litvinyuk, I V, Dooley, P W, Quéré, F, Bandrauk, A D, Villeneuve, D M, Corkum, P B
Format: Journal Article
Language:English
Published: United States 29-08-2003
Online Access:Get full text
Tags: Add Tag
No Tags, Be the first to tag this record!
Description
Summary:Ionization of D2 launches a vibrational wave packet on the ground state of D+2. Removal of the second electron places a pair of D+ ions onto a Coulombic potential. Measuring the D+ kinetic energy determines the time delay between the first and the second ionization. Caught between a falling ionization and a rapidly rising intensity, the typical lifetime of the D+2 intermediate is less than 5 fs when an intense 8.6 fs laser pulse is used. We simulate Coulomb explosion imaging of the ground state wave function of D2 by a 4 fs optical pulse and compare with our experimental observations.
Bibliography:ObjectType-Article-1
SourceType-Scholarly Journals-1
ObjectType-Feature-2
content type line 23
ISSN:0031-9007
1079-7114
DOI:10.1103/PhysRevLett.91.093002