Magic numbers in the magnetic properties of gadolinium clusters

Gadolinium clusters (N = 11-92) in a molecular beam exhibit dramatic size dependences in their magnetic properties. Two principal behaviors are observed: rigid rotor precession and nutation when the magnetic moment is tightly locked to the lattice by crystal anisotropy, and superparamagnetism when t...

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Bibliographic Details
Published in:Physical review letters Vol. 68; no. 11; pp. 1774 - 1777
Main Authors: Douglass, DC, Bucher, JP, Bloomfield, LA
Format: Journal Article
Language:English
Published: United States 16-03-1992
Online Access:Get full text
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Summary:Gadolinium clusters (N = 11-92) in a molecular beam exhibit dramatic size dependences in their magnetic properties. Two principal behaviors are observed: rigid rotor precession and nutation when the magnetic moment is tightly locked to the lattice by crystal anisotropy, and superparamagnetism when the moment is approximately free. Partially locked behavior is also seen. Magnetic moments of approx 3 mu sub B /atom are observed, with Curie temperatures substantially above the bulk value. Moments that remain locked > 300K may permit ultrahigh density magnetic memory.
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ISSN:0031-9007
1079-7114
DOI:10.1103/physrevlett.68.1774