Pollution of hazardous substances in industrial construction and demolition wastes and their multi-path risk within an abandoned pesticide manufacturing plant
Exploration of heavy metals and organic pollutants, their leaching capacity along with health and environmental risks in contaminated industrial construction and demolition waste (ICDW) within a pesticide manufacturing plant were investigated. A maximum content of 90.8 mg·kg-1 Cd was found present i...
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Published in: | Frontiers of environmental science & engineering Vol. 11; no. 1; pp. 123 - 135 |
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01-02-2017
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Abstract | Exploration of heavy metals and organic pollutants, their leaching capacity along with health and environmental risks in contaminated industrial construction and demolition waste (ICDW) within a pesticide manufacturing plant were investigated. A maximum content of 90.8 mg·kg-1 Cd was found present in the wastes, which might originate from phosphorus rocks and industrial sulfuric acid used in pesticide production processes. An average concentration of 979.8 mg·kg-1 dichlorovos and other 11 organophosphorus pesticide were also detected. Relatively high leaching rates of around 4.14‰ were obtained from laboratory simulated ICDW using both glacial acetic acidsodium hydroxide and deionized water. Pesticide pollutants had the strongest tendency to retaining on dry bricks (leaching rate 1.68 9‰) compared to mortar-coatings, etc. due to their different physical characteristics and octanol-water partioning coefficient. Mobility of pesticide from on-site ICDW by water was spatially correlated to waste types, process sections and human activities, with a flux of leaching rate between 5.9‰ to 27.4%. Risk-based corrective action (RBCA) model was used to simulate the risk of contaminated ICDW debris randomly scattered. Oral and demlal ingestion amount by local workers was 9.8 × 10-3 and 1.9 × 10-2 mg.(kg-d)-1, respectively. Potential leaching risk to aquatic systems exceeded the limit for nearly 75% waste. Environmental and health risk exceedance was found in most ICDW, while the risk value of the most severely contaminated brick waste was 660 times beyond critical level. Implications for waste management involving construction and deconstruction work, waste transferring and regulation supplying were also provided. |
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AbstractList | Exploration of heavy metals and organic pollutants, their leaching capacity along with health and environmental risks in contaminated industrial construction and demolition waste (ICDW) within a pesticide manufacturing plant were investigated. A maximum content of 90.8 mg·kg-1 Cd was found present in the wastes, which might originate from phosphorus rocks and industrial sulfuric acid used in pesticide production processes. An average concentration of 979.8 mg·kg-1 dichlorovos and other 11 organophosphorus pesticide were also detected. Relatively high leaching rates of around 4.14‰ were obtained from laboratory simulated ICDW using both glacial acetic acidsodium hydroxide and deionized water. Pesticide pollutants had the strongest tendency to retaining on dry bricks (leaching rate 1.68 9‰) compared to mortar-coatings, etc. due to their different physical characteristics and octanol-water partioning coefficient. Mobility of pesticide from on-site ICDW by water was spatially correlated to waste types, process sections and human activities, with a flux of leaching rate between 5.9‰ to 27.4%. Risk-based corrective action (RBCA) model was used to simulate the risk of contaminated ICDW debris randomly scattered. Oral and demlal ingestion amount by local workers was 9.8 × 10-3 and 1.9 × 10-2 mg.(kg-d)-1, respectively. Potential leaching risk to aquatic systems exceeded the limit for nearly 75% waste. Environmental and health risk exceedance was found in most ICDW, while the risk value of the most severely contaminated brick waste was 660 times beyond critical level. Implications for waste management involving construction and deconstruction work, waste transferring and regulation supplying were also provided. Exploration of heavy metals and organic pollutants, their leaching capacity along with health and environmental risks in contaminated industrial construction and demolition waste (ICDW) within a pesticide manufacturing plant were investigated. A maximum content of 90.8 mg•kg–1 Cd was found present in the wastes, which might originate from phosphorus rocks and industrial sulfuric acid used in pesticide production processes. An average concentration of 979.8 mg•kg–1 dichlorovos and other 11 organophosphorus pesticide were also detected. Relatively high leaching rates of around 4.14‰were obtained from laboratory simulated ICDW using both glacial acetic acid-sodium hydroxide and deionized water. Pesticide pollutants had the strongest tendency to retaining on dry bricks (leaching rate 1.68‰) compared to mortar-coatings, etc. due to their different physical characteristics and octanol-water partioning coefficient. Mobility of pesticide from on-site ICDW by water was spatially correlated to waste types, process sections and human activities, with a flux of leaching rate between 5.9‰ to 27.4%. Risk-based corrective action (RBCA) model was used to simulate the risk of contaminated ICDW debris randomly scattered. Oral and dermal ingestion amount by local workers was 9.8 × 10–3 and 1.9 × 10–2 mg•(kg•d)–1, respectively. Potential leaching risk to aquatic systems exceeded the limit for nearly 75% waste. Environmental and health risk exceedance was found in most ICDW, while the risk value of the most severely contaminated brick waste was 660 times beyond critical level. Implications for waste management involving construction and deconstruction work, waste transferring and regulation supplying were also provided. Exploration of heavy metals and organic pollutants, their leaching capacity along with health and environmental risks in contaminated industrial construction and demolition waste (ICDW) within a pesticide manufacturing plant were investigated. A maximum content of 90.8 mg•kg –1 Cd was found present in the wastes, which might originate from phosphorus rocks and industrial sulfuric acid used in pesticide production processes. An average concentration of 979.8 mg•kg –1 dichlorovos and other 11 organophosphorus pesticide were also detected. Relatively high leaching rates of around 4.14‰were obtained from laboratory simulated ICDW using both glacial acetic acid-sodium hydroxide and deionized water. Pesticide pollutants had the strongest tendency to retaining on dry bricks (leaching rate 1.68‰) compared to mortar-coatings, etc. due to their different physical characteristics and octanol-water partioning coefficient. Mobility of pesticide from on-site ICDW by water was spatially correlated to waste types, process sections and human activities, with a flux of leaching rate between 5.9‰ to 27.4%. Risk-based corrective action (RBCA) model was used to simulate the risk of contaminated ICDW debris randomly scattered. Oral and dermal ingestion amount by local workers was 9.8 × 10 –3 and 1.9 × 10 –2 mg•(kg•d) –1 , respectively. Potential leaching risk to aquatic systems exceeded the limit for nearly 75% waste. Environmental and health risk exceedance was found in most ICDW, while the risk value of the most severely contaminated brick waste was 660 times beyond critical level. Implications for waste management involving construction and deconstruction work, waste transferring and regulation supplying were also provided. Pollution pattern of metals and organic pesticide in demolition waste is studied. Organophosphorus pesticide can be everlasting on surface of demolition waste. Leaching potential of pollutants from simulated and onsite waste varies spatially. Direct oral and dermal ingestion, leaching potential into water exceed the limit. Implications for demolition waste management in industrial plants are proposed. Exploration of heavy metals and organic pollutants, their leaching capacity along with health and environmental risks in contaminated industrial construction and demolition waste (ICDW) within a pesticide manufacturing plant were investigated. A maximum content of 90.8 mg·kg −1 Cd was found present in the wastes, which might originate from phosphorus rocks and industrial sulfuric acid used in pesticide production processes. An average concentration of 979.8 mg·kg −1 dichlorovos and other 11 organophosphorus pesticide were also detected. Relatively high leaching rates of around 4.14‰ were obtained from laboratory simulated ICDW using both glacial acetic acid- sodium hydroxide and deionized water. Pesticide pollutants had the strongest tendency to retaining on dry bricks (leaching rate 1.68‰) compared to mortar-coatings, etc. due to their different physical characteristics and octanol-water partioning coefficient. Mobility of pesticide from on-site ICDW by water was spatially correlated to waste types, process sections and human activities, with a flux of leaching rate between 5.9‰ to 27.4%. Risk-based corrective action (RBCA) model was used to simulate the risk of contaminated ICDW debris randomly scattered. Oral and dermal ingestion amount by local workers was 9.8 × 10 −3 and 1.9 × 10 −2 mg·(kg·d) −1, respectively. Potential leaching risk to aquatic systems exceeded the limit for nearly 75% waste. Environmental and health risk exceedance was found in most ICDW, while the risk value of the most severely contaminated brick waste was 660 times beyond critical level. Implications for waste management involving construction and deconstruction work, waste transferring and regulation supplying were also provided. |
ArticleNumber | 12 |
Author | Sun, Yanqiu Yu, Yi Gao, Xiaofeng Zhao, Xin Zhao, Youcai Huang, Sheng Xu, Dongsheng Xie, Tian Ma, Jianli |
AuthorAffiliation | The State Key Laboratory of Pollution Control and Resource Reuse, Tongji University, Shanghai 200092, China Shanghai Chengpei Enterprise Management Consulting Co., Ltd., Shanghai 200232, China Tianjin Academy of Environmental Sciences, Tianjin 300191, China Debin Environmental Protection and Technology Holding Co., Ltd., Shanghai 200092, China Shanghai Design Institute in Environmental Sanitary Engineering, Shanghai 200092, China |
Author_xml | – sequence: 1 givenname: Sheng surname: Huang fullname: Huang, Sheng organization: The State Key Laboratory of Pollution Control and Resource Reuse, Tongji University, Shanghai 200092, China – sequence: 2 givenname: Xin surname: Zhao fullname: Zhao, Xin organization: Shanghai Chengpei Enterprise Management Consulting Co., Ltd., Shanghai 200232, China – sequence: 3 givenname: Yanqiu surname: Sun fullname: Sun, Yanqiu organization: The State Key Laboratory of Pollution Control and Resource Reuse, Tongji University, Shanghai 200092, China – sequence: 4 givenname: Jianli surname: Ma fullname: Ma, Jianli organization: Tianjin Academy of Environmental Sciences, Tianjin 300191, China – sequence: 5 givenname: Xiaofeng surname: Gao fullname: Gao, Xiaofeng organization: The State Key Laboratory of Pollution Control and Resource Reuse, Tongji University, Shanghai 200092, China – sequence: 6 givenname: Tian surname: Xie fullname: Xie, Tian organization: The State Key Laboratory of Pollution Control and Resource Reuse, Tongji University, Shanghai 200092, China – sequence: 7 givenname: Dongsheng surname: Xu fullname: Xu, Dongsheng organization: Debin Environmental Protection and Technology Holding Co., Ltd., Shanghai 200092, China – sequence: 8 givenname: Yi surname: Yu fullname: Yu, Yi organization: Shanghai Design Institute in Environmental Sanitary Engineering, Shanghai 200092, China – sequence: 9 givenname: Youcai surname: Zhao fullname: Zhao, Youcai email: zhaoyoucai@tongji.edu.cn organization: The State Key Laboratory of Pollution Control and Resource Reuse, Tongji University, Shanghai 200092, China |
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CitedBy_id | crossref_primary_10_1016_j_jclepro_2017_06_232 crossref_primary_10_1080_00038628_2018_1564646 crossref_primary_10_1007_s10668_019_00393_6 crossref_primary_10_1080_10643389_2019_1571354 crossref_primary_10_1108_JEDT_08_2019_0203 crossref_primary_10_1007_s11783_017_0931_9 crossref_primary_10_1016_j_jhydrol_2017_07_016 crossref_primary_10_1016_j_jclepro_2019_118163 crossref_primary_10_1016_j_jclepro_2020_125071 crossref_primary_10_1016_j_scitotenv_2023_163340 crossref_primary_10_1016_j_chemosphere_2021_130760 |
Cites_doi | 10.1016/j.chemgeo.2010.11.028 10.1177/0734242X15602963 10.1016/j.microc.2012.03.020 10.2136/sssaj2010.0019 10.1016/j.chemosphere.2003.08.026 10.1007/s10098-006-0078-z 10.1002/ps.1101 10.1016/S0956-053X(01)00007-1 10.1016/S0045-6535(97)00317-2 10.1016/0045-6535(91)90048-I 10.1016/S0950-4230(98)00062-X 10.1089/ees.2006.23.239 10.1039/C6EM00019C 10.1007/s11356-014-4058-2 10.1080/00103629409369207 10.1007/s11783-011-0370-y 10.1016/j.jhazmat.2010.04.116 10.1016/S0166-1116(97)80204-X 10.2166/9781780401072 |
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Notes | Exploration of heavy metals and organic pollutants, their leaching capacity along with health and environmental risks in contaminated industrial construction and demolition waste (ICDW) within a pesticide manufacturing plant were investigated. A maximum content of 90.8 mg·kg-1 Cd was found present in the wastes, which might originate from phosphorus rocks and industrial sulfuric acid used in pesticide production processes. An average concentration of 979.8 mg·kg-1 dichlorovos and other 11 organophosphorus pesticide were also detected. Relatively high leaching rates of around 4.14‰ were obtained from laboratory simulated ICDW using both glacial acetic acidsodium hydroxide and deionized water. Pesticide pollutants had the strongest tendency to retaining on dry bricks (leaching rate 1.68 9‰) compared to mortar-coatings, etc. due to their different physical characteristics and octanol-water partioning coefficient. Mobility of pesticide from on-site ICDW by water was spatially correlated to waste types, process sections and human activities, with a flux of leaching rate between 5.9‰ to 27.4%. Risk-based corrective action (RBCA) model was used to simulate the risk of contaminated ICDW debris randomly scattered. Oral and demlal ingestion amount by local workers was 9.8 × 10-3 and 1.9 × 10-2 mg.(kg-d)-1, respectively. Potential leaching risk to aquatic systems exceeded the limit for nearly 75% waste. Environmental and health risk exceedance was found in most ICDW, while the risk value of the most severely contaminated brick waste was 660 times beyond critical level. Implications for waste management involving construction and deconstruction work, waste transferring and regulation supplying were also provided. Industrial demolition wastes; Heavy metals; Pesticides; Leaching characteristics; Risk assessment ;Waste management 10-1013/X Document received on :2016-09-12 Waste management Leaching characteristics Document accepted on :2016-12-14 Risk assessment Pesticides Industrial demolition wastes Heavy metals |
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PublicationTitle | Frontiers of environmental science & engineering |
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Snippet | Exploration of heavy metals and organic pollutants, their leaching capacity along with health and environmental risks in contaminated industrial construction... Pollution pattern of metals and organic pesticide in demolition waste is studied. Organophosphorus pesticide can be everlasting on surface of demolition waste.... |
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SubjectTerms | Acetic acid Aquatic environment Bricks Cadmium Construction industry wastes Contamination Deionization Demolition Earth and Environmental Science Environment Environmental risk Hazardous materials Health risks Heavy metals Industrial demolition wastes Industrial pollution Ingestion Leaching Leaching characteristics Manufacturing Manufacturing industry Octanol Organophosphorus pesticides Pesticides Physical characteristics Physical properties Pollutants Research Article Risk assessment Sodium hydroxide Sulfuric acid Waste disposal Waste management Wastes Water pollution 多路径 工业硫酸 建筑废弃物 有害物质 有机污染物 有机磷农药 正辛醇-水分配系数 环境风险 |
Title | Pollution of hazardous substances in industrial construction and demolition wastes and their multi-path risk within an abandoned pesticide manufacturing plant |
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