Active interrogation of Special Nuclear Material containers using AmBe quasi-forward biased directional source and PGNAA

• Published in: Applied radiation and isotopes Vol. 156; no. C; p. 108974
• Main Authors: Paaren, Kyle M., Kilby, Seth, Lee, Hyoung K.
• Format: Journal Article
• Language: English
• Published: England Elsevier Ltd 01-02-2020; Elsevier
• Subjects: AmBe; Angular distribution; MCNP; NJOY; Simulation; TENDL; AmBe; Angular distribution; NJOY; Simulation; MCNP; TENDL
• ISSN: 0969-8043; 1872-9800
• DOI: 10.1016/j.apradiso.2019.108974

Special Nuclear Material (SNM) including 95% 235U and 239Pu is capable of being identified by utilizing a quasi-forward directional AmBe source from Patent No: US20190013109A1 using Prompt Gamma Neutron Activation Analysis (PGNAA) simulated with Monte-Carlo N-Particle transport 6.2 (MCNP). HPGe and LaBr3 detector arrays were used to identify and quantify the peak-to-background and peak-to-total ratios of the associated photon spectra from the SNM encased in a polyethylene shield. The conducted simulations varied the volume of the SNM and neutron source strength in the MCNP data card to conduct an uncertainty analysis. Photopeaks identified include K-shell X-rays from 235U and 239Pu, 61 keV from fission, 2.223 MeV prompt gamma from hydrogen, 511 keV annihilation, and a single and double escape peak from the prompt gamma interaction from hydrogen. Relationships between peak-to-total and peak-to-background as a function of SNM and particle history were investigated to aid in the analysis. The capabilities of both detector systems to acquire well resolved photopeak with a 5% relative error or less, with a 1 Ci source activity, and a peak-to-background ratio of 1.15. This was determined to take 326 s for LaBr3 and 163 s for HPGe which is comparable to current methods for material detection which take between 100 and 900 s to acquire.
•Peak-to-total and peak-to-background ratios for photopeaks were quantified.•LaBr3 and HPGe detector arrays acquired well resolved photopeaks.•Acquisition time for a well resolved photopeak was between 100 and 900 s.•Acquisition time comparable to current active interrogation technology.•Photopeaks identified include K-shell X-rays, fission, and 1H prompt gamma.