Fabrication of nanocrystalline diamond capsules by hot-filament chemical vapor deposition for direct-drive inertial confinement fusion experiments

• Published in: Diamond and related materials Vol. 135; p. 109896
• Main Authors: Kawasaki, K., Yamada, H., Nagatomo, H., Hironaka, Y., Yamanoi, K., Tanaka, D., Idesaka, T., Mokuno, Y., Chayahara, A., Shimaoka, T., Mima, K., Somekawa, T., Tsukamoto, M., Sato, Y., Iwamoto, A., Shigemori, K.
• Format: Journal Article
• Language: English
• Published: Elsevier B.V 01-05-2023
• Subjects: Diamond capsule; Direct-drive inertial confinement fusion; Hot-filament chemical vapor deposition; Nanocrystalline diamond; Diamond capsule; Direct-drive inertial confinement fusion; Nanocrystalline diamond; Hot-filament chemical vapor deposition
• ISSN: 0925-9635; 1879-0062
• DOI: 10.1016/j.diamond.2023.109896

Direct-drive inertial confinement fusion (ICF), where a fuel capsule is imploded by high-power laser beams to cause ignition, is a promising energy production method that does not emit any greenhouse gases. Diamond is an ideal capsule material for direct-drive ICF. Its low compressibility and high density, which exceed those of conventional capsule materials (e.g., plastic), are advantageous for the robust implosion of fuel capsules. We are developing polycrystalline diamond capsules using the hot-filament chemical vapor deposition (HF-CVD) technique. HF-CVD is ideal for capsule fabrication for power plants of the future because it is inexpensive and amenable to mass production, as its deposition area can be extended by only increasing the number of filaments. In this study, we improved upon our previous fabrication process and obtained nanocrystalline diamond capsules of better quality. The capsules were comprehensively characterized, employing both the typical parameters (i.e., surface morphology and sp2 content) as well as parameters important for direct-drive ICF application (i.e., tungsten and hydrogen contents, capsule thickness, density, and mode amplitudes of surface roughness). The characterized hollow nanocrystalline diamond capsules were introduced into the laser experiment at the GEKKO laser facility at Osaka University, where a capsule can be spherically irradiated by 12 high-power laser beams. The experimental results showed successful implosion, and the implosion dynamics were well reproduced by radiation hydrodynamic simulation code calculations. These results verify the accurate characterization and quality of the nanocrystalline diamond capsules as being applicable to laser irradiation experiments.
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•Diamond capsule was fabricated by hot filament chemical vapor deposition.•Fabricated capsules were comprehensively characterized.•Laser experiment demonstrated successful implosion of the fabricated capsules.