Photoelectrochemical properties of poly(terthiophene) films modified with a fullerene derivative
This work reports on the photoelectrochemical properties of an interface comprised by poly(terthiophene) films electrochemically synthesized onto indium–tin oxide substrates and modified with 1-(3-methoxycarbonyl)-propyl-1-phenyl-(6,6)C61. Important photoelectrical parameters, such as flat band pote...
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| Published in: | Thin solid films Vol. 515; no. 4; pp. 2644 - 2649 |
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| Format: | Journal Article |
| Language: | English |
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Elsevier B.V
05-12-2006
Elsevier Science |
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| Abstract | This work reports on the photoelectrochemical properties of an interface comprised by poly(terthiophene) films electrochemically synthesized onto indium–tin oxide substrates and modified with 1-(3-methoxycarbonyl)-propyl-1-phenyl-(6,6)C61. Important photoelectrical parameters, such as flat band potential, density of charge carriers and depletion layer width were determined for the pristine and hybrid films. The cathodic photocurrent reflected the p-type semiconducting behavior of the electrosynthesized poly(terthiophene)s. Addition of the acceptor molecule improves the photocurrent at zero bias (∼6 μA cm−2 at 100 mW cm−2) indicating the fullerene derivative acts as an exciton dissociation center, improving the number of charge carriers transported through the polymer to reach the solid–liquid electrolyte interface. |
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| AbstractList | This work reports on the photoelectrochemical properties of an interface comprised by poly(terthiophene) films electrochemically synthesized onto indium-tin oxide substrates and modified with 1-(3-methoxycarbonyl)-propyl-1-phenyl-(6,6)C61. Important photoelectrical parameters, such as flat band potential, density of charge carriers and depletion layer width were determined for the pristine and hybrid films. The cathodic photocurrent reflected the p-type semiconducting behavior of the electrosynthesized poly(terthiophene)s. Addition of the acceptor molecule improves the photocurrent at zero bias (~6 muA cm(-2)at 100 mW cm(-2)) indicating the fullerene derivative acts as an exciton dissociation center, improving the number of charge carriers transported through the polymer to reach the solid-liquid electrolyte interface. This work reports on the photoelectrochemical properties of an interface comprised by poly(terthiophene) films electrochemically synthesized onto indium–tin oxide substrates and modified with 1-(3-methoxycarbonyl)-propyl-1-phenyl-(6,6)C61. Important photoelectrical parameters, such as flat band potential, density of charge carriers and depletion layer width were determined for the pristine and hybrid films. The cathodic photocurrent reflected the p-type semiconducting behavior of the electrosynthesized poly(terthiophene)s. Addition of the acceptor molecule improves the photocurrent at zero bias (∼6 μA cm−2 at 100 mW cm−2) indicating the fullerene derivative acts as an exciton dissociation center, improving the number of charge carriers transported through the polymer to reach the solid–liquid electrolyte interface. |
| Author | Girotto, Emerson M. Nogueira, Ana Flávia Santos, Marcos J.L. |
| Author_xml | – sequence: 1 givenname: Marcos J.L. surname: Santos fullname: Santos, Marcos J.L. organization: Departamento de Química, Universidade Estadual de Maringá, UEM, 87020-900, Maringá-PR, Brazil – sequence: 2 givenname: Emerson M. surname: Girotto fullname: Girotto, Emerson M. organization: Departamento de Química, Universidade Estadual de Maringá, UEM, 87020-900, Maringá-PR, Brazil – sequence: 3 givenname: Ana Flávia surname: Nogueira fullname: Nogueira, Ana Flávia email: anaflavia@iqm.unicamp.br organization: Instituto de Química, Universidade Estadual de Campinas, UNICAMP, CP 6154, 13084-971, Campinas-SP, Brazil |
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| CitedBy_id | crossref_primary_10_1039_c1pp05221g crossref_primary_10_1002_solr_201900395 crossref_primary_10_1016_j_tsf_2017_02_051 crossref_primary_10_1016_j_jnoncrysol_2008_06_077 crossref_primary_10_1016_j_polymdegradstab_2015_11_006 crossref_primary_10_3390_polym13121977 crossref_primary_10_1039_c3py00143a crossref_primary_10_3390_nano12091408 |
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| Issue | 4 |
| Keywords | Fullerene Poly(terthiophene) Electrochemistry Conducting polymer Interface Liquid solid interface Charge carriers Semiconductor materials Hybrid material Photocurrents Charge transport Thin films Tin oxides Conducting polymers Fullerenes Indium oxides Photoconductivity Carrier density |
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| Snippet | This work reports on the photoelectrochemical properties of an interface comprised by poly(terthiophene) films electrochemically synthesized onto indium–tin... This work reports on the photoelectrochemical properties of an interface comprised by poly(terthiophene) films electrochemically synthesized onto indium-tin... |
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| SubjectTerms | Chemistry Condensed matter: electronic structure, electrical, magnetic, and optical properties Conducting polymer Cross-disciplinary physics: materials science; rheology Electrochemistry Electronic structure and electrical properties of surfaces, interfaces, thin films and low-dimensional structures Electronic transport phenomena in thin films and low-dimensional structures Exact sciences and technology Fullerene Fullerenes and related materials; diamonds, graphite General and physical chemistry Interface Kinetics and mechanism of reactions Materials science Photoconduction and photovoltaic effects; photodielectric effects Physics Poly(terthiophene) Specific materials Surface conductivity and carrier phenomena |
| Title | Photoelectrochemical properties of poly(terthiophene) films modified with a fullerene derivative |
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