Oil drop stretch and rupture behavior at throat and pore junction during imbibition with active nanofluid: A microfluidic approach

• Published in: Colloids and surfaces. A, Physicochemical and engineering aspects Vol. 653; p. 130012
• Main Authors: Sun, Yongpeng, Xin, Yan, Wei, Li’nan, Ding, Fei, Gao, Zhanwu, Liu, Hanbin, Tang, Meirong, Du, Xianfei, Dai, Caili
• Format: Journal Article
• Language: English
• Published: Elsevier B.V 20-11-2022
• Subjects: Active nanofluid; Enhanced oil recovery; Imbibition; Interfacial tension; Microfluidic; Oil drop stretch process; Active nanofluid; Imbibition; Oil drop stretch process; Enhanced oil recovery; Interfacial tension; Microfluidic
• ISSN: 0927-7757; 1873-4359
• DOI: 10.1016/j.colsurfa.2022.130012

Imbibition is an effective method to recover oil from small pore and throat. Here we report the formation of oil drop at pore and throat junction during spontaneous imbibition with active nanofluid. A T-channel microfluidic model combined with high-speed camera was used to observe the stretch and rupture process of oil discharged from throat to pore. When oil drop was discharged from throat gradually, its width/length was kept deceasing before rupturing. With more active content in the aqueous phase, the interfacial tension decreased from 33.8 to 8.7 mN/m, and the oil recovery increased by 12.4% by spontaneous imbibition. The oil drop rupture frequency increased by 3.0 times, but the length and width of the oil drop decreased by 32.2% and 28.0%, respectively. The reduced size of the oil drop would benefit the oil transportation in porous media. Higher flow rate in pores and throat would all intensify rupturing of the oil drop. Moreover, small throat could further reinforce the rupturing process. From combination of fluid flow rate, interfacial tension, and viscosity, higher capillary number reduced the maximum dimensionless width and length of the oil drop by 44.3% and 42.7%, respectively. The reduced size of oil drops ruptured at pore and throat junction contributes to the transportation of oil in porous media. Overall, this study provides a basic theory for active nanofluid to enhance imbibition oil recovery in tight reservoirs.
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•A T-shaped microfluidic model was used to observe the stretch and rupture process of oil drop.•Oil drop rupture morphology and frequency were affected by various parameters.•Higher capillary number reduced the maximum dimensionless width and height of the oil drop.•The reduced size of ruptured oil drops contributes to their transportation in porous media.