Discrepancy in response functions obtained from Stokes and anti-Stokes low-frequency light scattering in liquid

Discrepancy in response functions obtained from Stokes and anti-Stokes low-frequency light scattering in liquid

The relation between intensities of Stokes and anti-Stokes light scattering in low-frequency region has been investigated for liquid carbon disulfide at room temperature. The commonly used relation between these scattering intensities breaks down in the energy region of the relaxational mode. This l...

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Published in:Journal of luminescence Vol. 87; pp. 779 - 781
Main Authors: Watanabe, J, Watanabe, Y, Tango, M, Kinoshita, S
Format: Journal Article
Language:English
Published: Elsevier B.V 01-05-2000
Subjects:
Anti-Stokes scattering
Relaxational mode
Response function
Stokes scattering
Response function
Relaxational mode
Stokes scattering
Anti-Stokes scattering
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Abstract The relation between intensities of Stokes and anti-Stokes light scattering in low-frequency region has been investigated for liquid carbon disulfide at room temperature. The commonly used relation between these scattering intensities breaks down in the energy region of the relaxational mode. This leads to a discrepancy in linear response functions obtained from the Stokes and anti-Stokes scattering separately. The behavior may be related to the fact that the mode interacts with other bath modes and is strongly dissipative.
AbstractList The relation between intensities of Stokes and anti-Stokes light scattering in low-frequency region has been investigated for liquid carbon disulfide at room temperature. The commonly used relation between these scattering intensities breaks down in the energy region of the relaxational mode. This leads to a discrepancy in linear response functions obtained from the Stokes and anti-Stokes scattering separately. The behavior may be related to the fact that the mode interacts with other bath modes and is strongly dissipative.
Author Watanabe, Y
Watanabe, J
Tango, M
Kinoshita, S
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Keywords Response function
Relaxational mode
Stokes scattering
Anti-Stokes scattering
Language English
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Loudon (BIB2) 1978; 7
L.D. Landau, E.M. Lifshits, Electrodynamics of Continuous Media, Pergamon, Oxford, 1960.
W. Hayes, R. Loudon, Scattering of Light by Crystals, Wiley, New York, 1978.
10.1016/S0022-2313(99)00402-0_BIB3
Kinoshita (10.1016/S0022-2313(99)00402-0_BIB4) 1999; 301
10.1016/S0022-2313(99)00402-0_BIB1
Loudon (10.1016/S0022-2313(99)00402-0_BIB2) 1978; 7
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  publication-title: Chem. Phys. Lett.
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  contributor:
    fullname: Kinoshita
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Snippet The relation between intensities of Stokes and anti-Stokes light scattering in low-frequency region has been investigated for liquid carbon disulfide at room...
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StartPage 779
SubjectTerms Anti-Stokes scattering
Relaxational mode
Response function
Stokes scattering
Title Discrepancy in response functions obtained from Stokes and anti-Stokes low-frequency light scattering in liquid
URI https://dx.doi.org/10.1016/S0022-2313(99)00402-0
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