Optical structure modification induced by lattice strain in Mn-doped CdSe QDs
Narrow size distribution manganese-doped cadmium selenide quantum dots (Mn-doped CdSe QDs) successfully synthesized using inverse Micelle technique with organic solvent and surfactant possesses zinc blende structure with physical size ranging from 3 to 14 nm and crystallite size 2.46–5.46 nm. Mn-dop...
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| Published in: | Optical materials Vol. 86; pp. 441 - 448 |
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| Main Authors: | , , , , , , |
| Format: | Journal Article |
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Elsevier B.V
01-12-2018
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| Abstract | Narrow size distribution manganese-doped cadmium selenide quantum dots (Mn-doped CdSe QDs) successfully synthesized using inverse Micelle technique with organic solvent and surfactant possesses zinc blende structure with physical size ranging from 3 to 14 nm and crystallite size 2.46–5.46 nm. Mn-doped CdSe QDs observed to growth larger QDs compared to pure CdSe QDs at significantly same reaction times. The lattice parameter compressed with QDs sizes growth due to the introduction of lattice strain provoked by the incorporation of Mn atoms into CdSe QDs lattice. The Mn-doped CdSe QDs shows a slight blue-shift on absorption and emission spectra's compared to pure CdSe even though is possessed larger QDs. The band gap structure modification prominently affected by the lattice strain were transition of Stoke's, Rayleigh to anti-Stoke`s shifts observed as the Mn-doped CdSe QDs size growth. The typical red-shift of absorption and emission wavelength observed with growth of QDs sizes. The role of oleic acid as a surfactant and capping agent shows in FTIR spectra. The lattice strain tailored the binding energy between the ion prominently on the surface of the QDs with growth of QDs sizes.
•Synthesis and characterizations of Mn-doped CdSe QDs at different sizes.•Unique pattern of HOMO/LUMO electron transition with temporal evolution of QDs size.•Modification of optical structure of QDs expected to be induced by manganese doping mechanism. |
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| AbstractList | Narrow size distribution manganese-doped cadmium selenide quantum dots (Mn-doped CdSe QDs) successfully synthesized using inverse Micelle technique with organic solvent and surfactant possesses zinc blende structure with physical size ranging from 3 to 14 nm and crystallite size 2.46–5.46 nm. Mn-doped CdSe QDs observed to growth larger QDs compared to pure CdSe QDs at significantly same reaction times. The lattice parameter compressed with QDs sizes growth due to the introduction of lattice strain provoked by the incorporation of Mn atoms into CdSe QDs lattice. The Mn-doped CdSe QDs shows a slight blue-shift on absorption and emission spectra's compared to pure CdSe even though is possessed larger QDs. The band gap structure modification prominently affected by the lattice strain were transition of Stoke's, Rayleigh to anti-Stoke`s shifts observed as the Mn-doped CdSe QDs size growth. The typical red-shift of absorption and emission wavelength observed with growth of QDs sizes. The role of oleic acid as a surfactant and capping agent shows in FTIR spectra. The lattice strain tailored the binding energy between the ion prominently on the surface of the QDs with growth of QDs sizes.
•Synthesis and characterizations of Mn-doped CdSe QDs at different sizes.•Unique pattern of HOMO/LUMO electron transition with temporal evolution of QDs size.•Modification of optical structure of QDs expected to be induced by manganese doping mechanism. |
| Author | Wahab, Yasmin Abdul Hamizi, Nor Aliya Pivehzhani, Omid Akbarzadeh Saat, Asmalina Mohamed Al-Douri, Yarub Chowdhury, Zaira Zaman Johan, Mohd Rafie |
| Author_xml | – sequence: 1 givenname: Nor Aliya surname: Hamizi fullname: Hamizi, Nor Aliya email: aliyahamizi@um.edu.my organization: Nanotechnology & Catalysis Research Centre, Deputy Vice Chancellor (Research & Innovation) Office, University of Malaya, 50603, Kuala Lumpur, Malaysia – sequence: 2 givenname: Mohd Rafie surname: Johan fullname: Johan, Mohd Rafie organization: Nanotechnology & Catalysis Research Centre, Deputy Vice Chancellor (Research & Innovation) Office, University of Malaya, 50603, Kuala Lumpur, Malaysia – sequence: 3 givenname: Zaira Zaman surname: Chowdhury fullname: Chowdhury, Zaira Zaman organization: Nanotechnology & Catalysis Research Centre, Deputy Vice Chancellor (Research & Innovation) Office, University of Malaya, 50603, Kuala Lumpur, Malaysia – sequence: 4 givenname: Yasmin Abdul surname: Wahab fullname: Wahab, Yasmin Abdul organization: Nanotechnology & Catalysis Research Centre, Deputy Vice Chancellor (Research & Innovation) Office, University of Malaya, 50603, Kuala Lumpur, Malaysia – sequence: 5 givenname: Yarub surname: Al-Douri fullname: Al-Douri, Yarub organization: Nanotechnology & Catalysis Research Centre, Deputy Vice Chancellor (Research & Innovation) Office, University of Malaya, 50603, Kuala Lumpur, Malaysia – sequence: 6 givenname: Asmalina Mohamed surname: Saat fullname: Saat, Asmalina Mohamed organization: Universiti Kuala Lumpur Malaysian Institute of Marine Engineering Technology (UniKL MIMET) Department, Dataran Industri Teknologi Kejuruteraan Marin, Bandar Teknologi Maritim, Jalan Pantai Remis, 32200, Lumut Perak, Malaysia – sequence: 7 givenname: Omid Akbarzadeh surname: Pivehzhani fullname: Pivehzhani, Omid Akbarzadeh organization: Nanotechnology & Catalysis Research Centre, Deputy Vice Chancellor (Research & Innovation) Office, University of Malaya, 50603, Kuala Lumpur, Malaysia |
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| CitedBy_id | crossref_primary_10_3390_pr7100639 crossref_primary_10_1016_j_matlet_2020_128847 crossref_primary_10_1016_j_physb_2023_415623 crossref_primary_10_1016_j_jallcom_2019_152711 crossref_primary_10_1021_acsanm_0c02166 crossref_primary_10_1016_j_intermet_2021_107272 |
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