Disorder promotes ferromagnetism: Rounding of the quantum phase transition in Sr_{1-x}Ca_xRuO_3

Physical Review Letters 108, 185701 (2012) The subtle interplay of randomness and quantum fluctuations at low temperatures gives rise to a plethora of unconventional phenomena in systems ranging from quantum magnets and correlated electron materials to ultracold atomic gases. Particularly strong dis...

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Main Authors: Demko, L, Bordacs, S, Vojta, T, Nozadze, D, Hrahsheh, F, Svoboda, C, Dora, B, Yamada, H, Kawasaki, M, Tokura, Y, Kezsmarki, I
Format: Journal Article
Language:English
Published: 16-02-2012
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Summary:Physical Review Letters 108, 185701 (2012) The subtle interplay of randomness and quantum fluctuations at low temperatures gives rise to a plethora of unconventional phenomena in systems ranging from quantum magnets and correlated electron materials to ultracold atomic gases. Particularly strong disorder effects have been predicted to occur at zero-temperature quantum phase transitions. Here, we demonstrate that the composition-driven ferromagnetic-to-paramagnetic quantum phase transition in Sr1-xCaxRuO3 is completely destroyed by the disorder introduced via the different ionic radii of the randomly distributed Sr and Ca ions. Using a magneto-optical technique, we map the magnetic phase diagram in the composition-temperature space. We find that the ferromagnetic phase is significantly extended by the disorder and develops a pronounced tail over a broad range of the composition x. These findings are explained by a microscopic model of smeared quantum phase transitions in itinerant magnets. Moreover, our theoretical study implies that correlated disorder is even more powerful in promoting ferromagnetism than random disorder.
DOI:10.48550/arxiv.1202.3810