Glycosaminoglycan-Mimetic Biomaterials. 1. Nonsulfated and Sulfated Glycopolymers by Cyanoxyl-Mediated Free-Radical Polymerization
A series of N-acetyl-D-glucosamine-containing glycomonomers was synthesized as an initial step in the synthesis of glycosaminoglycanmimetic glycopolymers. It was shown that cyanoxyl-mediated free-radical polymerization is an original and straightforward approach for obtaining water-soluble glycopoly...
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| Published in: | Macromolecules Vol. 33; no. 4; pp. 1123 - 1125 |
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| Main Authors: | , , , , |
| Format: | Journal Article |
| Language: | English |
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American Chemical Society
22-02-2000
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| Abstract | A series of N-acetyl-D-glucosamine-containing glycomonomers was synthesized as an initial step in the synthesis of glycosaminoglycanmimetic glycopolymers. It was shown that cyanoxyl-mediated free-radical polymerization is an original and straightforward approach for obtaining water-soluble glycopolymers with high monosaccharide contents and low polydispersity indexes. |
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| AbstractList | A series of N-acetyl-D-glucosamine-containing glycomonomers was synthesized as an initial step in the synthesis of glycosaminoglycanmimetic glycopolymers. It was shown that cyanoxyl-mediated free-radical polymerization is an original and straightforward approach for obtaining water-soluble glycopolymers with high monosaccharide contents and low polydispersity indexes. |
| Author | Chaikof, E. L Gnanou, Y Grande, D Baskaran, S Baskaran, C |
| Author_xml | – sequence: 1 givenname: D surname: Grande fullname: Grande, D – sequence: 2 givenname: S surname: Baskaran fullname: Baskaran, S – sequence: 3 givenname: C surname: Baskaran fullname: Baskaran, C – sequence: 4 givenname: Y surname: Gnanou fullname: Gnanou, Y – sequence: 5 givenname: E. L surname: Chaikof fullname: Chaikof, E. L |
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| Cites_doi | 10.1021/ma00112a049 10.1007/978-1-4615-1885-3_11 10.1021/ma9816315 10.1002/anie.199316713 10.1016/S0959-440X(96)80037-6 10.1021/ma00015a002 10.1126/science.7536345 10.1021/ma00220a024 10.1021/ma00023a005 10.1021/ma9512519 10.1021/ma971329g 10.1021/cr00020a006 10.1021/ma00125a030 |
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| Keywords | Monodispersed polymer Side chain Aminoglycoside Preparation Acrylamide copolymer Organic sulfate Glycosaminoglycan Olefin derivative copolymer Radical copolymerization Experimental study |
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| References | Gallagher J. (ma991579sb00006/ma991579sb00006_1) 1995 Roy R. (ma991579sb00004/ma991579sb00004_1) 1996; 6 Fraser C. (ma991579sb00011/ma991579sb00011_1) 1995; 28 Toshima K. (ma991579sb00003/ma991579sb00003_1) 1993; 93 Nishimura S.-I. (ma991579sb00015/ma991579sb00015_1) 1991; 24 Nishimura S.-I. (ma991579sb00014/ma991579sb00014_1) 1990; 23 Ohno K. (ma991579sb00013/ma991579sb00013_1) 1998; 31 Druliner J. D. (ma991579sb00016/ma991579sb00016_1) 1991; 24 Nomura K. (ma991579sb00012/ma991579sb00012_1) 1996; 29 Yamada K. (ma991579sb00009/ma991579sb00009_1) 1997 ma991579sb00017/ma991579sb00017_1 Linhardt R. J. (ma991579sb00001/ma991579sb00001_1) 1996 Miyata T. (ma991579sb00007/ma991579sb00007_1) 1997; 5 Matsuoka K. (ma991579sb00008/ma991579sb00008_1) 1995; 28 Van Boeckel C. A. A. (ma991579sb00002/ma991579sb00002_1) 1993; 32 Yamada K. (ma991579sb00010/ma991579sb00010_1) 1999; 32 Gnanou Y. (ma991579sb00018/ma991579sb00018_1) 1999; 40 Ornitz D. M. (ma991579sb00005/ma991579sb00005_1) 1995; 268 |
| References_xml | – volume: 28 start-page: 2961 year: 1995 ident: ma991579sb00008/ma991579sb00008_1 publication-title: Macromolecules doi: 10.1021/ma00112a049 contributor: fullname: Matsuoka K. – start-page: 125 volume-title: Glycoimmunology year: 1995 ident: ma991579sb00006/ma991579sb00006_1 doi: 10.1007/978-1-4615-1885-3_11 contributor: fullname: Gallagher J. – volume: 40 start-page: 99 issue: 2 year: 1999 ident: ma991579sb00018/ma991579sb00018_1 publication-title: Polym. Prepr. (Am. Chem. Soc., Div. Polym. Chem.) contributor: fullname: Gnanou Y. – volume: 32 start-page: 3553 year: 1999 ident: ma991579sb00010/ma991579sb00010_1 publication-title: Macromolecules doi: 10.1021/ma9816315 contributor: fullname: Yamada K. – volume-title: Biomedical Functions and Biotechnology of Natural and Artificial Polymers year: 1996 ident: ma991579sb00001/ma991579sb00001_1 contributor: fullname: Linhardt R. J. – volume: 32 start-page: 1671 year: 1993 ident: ma991579sb00002/ma991579sb00002_1 publication-title: Angew. Chem., Int. Ed. Engl. doi: 10.1002/anie.199316713 contributor: fullname: Van Boeckel C. A. A. – volume: 6 start-page: 692 year: 1996 ident: ma991579sb00004/ma991579sb00004_1 publication-title: Curr. Opin. Struct. Biol. doi: 10.1016/S0959-440X(96)80037-6 contributor: fullname: Roy R. – volume: 24 start-page: 4236 year: 1991 ident: ma991579sb00015/ma991579sb00015_1 publication-title: Macromolecules doi: 10.1021/ma00015a002 contributor: fullname: Nishimura S.-I. – volume: 5 start-page: 198 year: 1997 ident: ma991579sb00007/ma991579sb00007_1 publication-title: Trends Polym. Sci. contributor: fullname: Miyata T. – volume: 268 start-page: 432 year: 1995 ident: ma991579sb00005/ma991579sb00005_1 publication-title: Science doi: 10.1126/science.7536345 contributor: fullname: Ornitz D. M. – volume: 23 start-page: 4182 year: 1990 ident: ma991579sb00014/ma991579sb00014_1 publication-title: Macromolecules doi: 10.1021/ma00220a024 contributor: fullname: Nishimura S.-I. – volume: 24 start-page: 6079 year: 1991 ident: ma991579sb00016/ma991579sb00016_1 publication-title: Macromolecules doi: 10.1021/ma00023a005 contributor: fullname: Druliner J. D. – volume-title: Part A: Polym. Chem year: 1997 ident: ma991579sb00009/ma991579sb00009_1 contributor: fullname: Yamada K. – ident: ma991579sb00017/ma991579sb00017_1 – volume: 29 start-page: 540 year: 1996 ident: ma991579sb00012/ma991579sb00012_1 publication-title: Macromolecules doi: 10.1021/ma9512519 contributor: fullname: Nomura K. – volume: 31 start-page: 1064 year: 1998 ident: ma991579sb00013/ma991579sb00013_1 publication-title: Macromolecules doi: 10.1021/ma971329g contributor: fullname: Ohno K. – volume: 93 start-page: 1503 year: 1993 ident: ma991579sb00003/ma991579sb00003_1 publication-title: Chem. Rev. doi: 10.1021/cr00020a006 contributor: fullname: Toshima K. – volume: 28 start-page: 7248 year: 1995 ident: ma991579sb00011/ma991579sb00011_1 publication-title: Macromolecules doi: 10.1021/ma00125a030 contributor: fullname: Fraser C. |
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| SubjectTerms | Amines Applied sciences Biomaterials Catalysts Copolymerization Exact sciences and technology Free radical polymerization Free radicals Glucose Nuclear magnetic resonance spectroscopy Organic polymers Physicochemistry of polymers Preparation, kinetics, thermodynamics, mechanism and catalysts Size exclusion chromatography |
| Title | Glycosaminoglycan-Mimetic Biomaterials. 1. Nonsulfated and Sulfated Glycopolymers by Cyanoxyl-Mediated Free-Radical Polymerization |
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