Ultrafast Optical Generation of Coherent Bright and Dark Surface Phonon Polaritons in Nanowires

• Published in: ACS photonics Vol. 7; no. 8; pp. 1923 - 1931
• Main Authors: Mante, Pierre-Adrien, Lehmann, Sebastian, Shapiro, Daniel Finkelstein, Lee, Kayin, Wallentin, Jesper, Borgström, Magnus T, Yartsev, Arkady
• Format: Journal Article
• Language: English
• Published: American Chemical Society 19-08-2020
• Subjects: Atom and Molecular Physics and Optics; Atom- och molekylfysik och optik; Condensed Matter Physics; Den kondenserade materiens fysik; Doping; Fysik; Nanowires; Natural Sciences; Naturvetenskap; Optical properties; Phonons; Physical Sciences; Polarization; coherence; surface phonon polaritons; subwavelength confinement; ultrafast
• ISSN: 2330-4022; 2330-4022
• DOI: 10.1021/acsphotonics.0c00537

The subwavelength confinement and enhanced electric field created by plasmons allow precise sensing and enhanced light–matter interaction. However, the high frequency and short lifetime of plasmons limit the full potential of this technology. It is crucial to find substitutes and to study their dynamics. Here, we propose an experimental approach allowing the time-domain study of surface phonon polaritons. We first build a theoretical framework for the interaction of ultrashort pulses of light with polar materials. We then perform femtosecond pump–probe experiments and demonstrate the generation and time-resolved detection of surface phonon polaritons. By comparing experiments and simulations, we show the presence of both bright and dark modes with quality factors up to 115. We then investigate mode-dependent decay and energy transfer to the environment. Our results offer a platform for the experimental exploration of the dynamics of surface phonon polaritons and of the role of coherence in energy transfer.