Competing short-range magnetic correlations, metamagnetic behavior and spin-phonon coupling in Nd^sub 2^CoMnO^sub 6^ double perovskite

We report the presence of ferromagnetic short-range interactions, metamagnetic transitions an spin-phonon coupling on monoclinic polycrystalline Nd2CoMnO6 double perovskite. DC thermomagnetic characterization shows a paramagnetic to ferromagnetic transition at TC1∼168 K and further to a cluster glas...

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Published in:Journal of alloys and compounds Vol. 773; p. 770
Main Authors: Das, Ranjana R, Lekshmi, P Neenu, Das, SC, Santhosh, PN
Format: Journal Article
Language:English
Published: Lausanne Elsevier BV 30-01-2019
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Abstract We report the presence of ferromagnetic short-range interactions, metamagnetic transitions an spin-phonon coupling on monoclinic polycrystalline Nd2CoMnO6 double perovskite. DC thermomagnetic characterization shows a paramagnetic to ferromagnetic transition at TC1∼168 K and further to a cluster glass like magnetic transition at TC2∼135 K. Griffiths phase like features are also observed, attributed to the presence of competing magnetic interactions. Step like nature observed in the virgin curves of magnetic isotherms implies the presence of metamagnetic features. Additionally, temperature evolution of Raman spectra signatures spin-phonon coupling extending up to Griffiths like phase region indicating the possibility of magnetoelectric coupling in Nd2CoMnO6.
AbstractList We report the presence of ferromagnetic short-range interactions, metamagnetic transitions an spin-phonon coupling on monoclinic polycrystalline Nd2CoMnO6 double perovskite. DC thermomagnetic characterization shows a paramagnetic to ferromagnetic transition at TC1∼168 K and further to a cluster glass like magnetic transition at TC2∼135 K. Griffiths phase like features are also observed, attributed to the presence of competing magnetic interactions. Step like nature observed in the virgin curves of magnetic isotherms implies the presence of metamagnetic features. Additionally, temperature evolution of Raman spectra signatures spin-phonon coupling extending up to Griffiths like phase region indicating the possibility of magnetoelectric coupling in Nd2CoMnO6.
Author Das, Ranjana R
Lekshmi, P Neenu
Santhosh, PN
Das, SC
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Snippet We report the presence of ferromagnetic short-range interactions, metamagnetic transitions an spin-phonon coupling on monoclinic polycrystalline Nd2CoMnO6...
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StartPage 770
SubjectTerms Correlation analysis
Coupling
Ferromagnetism
Magnetic fields
Magnetic transitions
Magnetism
Perovskite
Perovskites
Phase transitions
Raman spectra
Title Competing short-range magnetic correlations, metamagnetic behavior and spin-phonon coupling in Nd^sub 2^CoMnO^sub 6^ double perovskite
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