Sensing Spin Wave Excitations by Spin Defects in Few-Layer Thick Hexagonal Boron Nitride

Optically active spin defects in wide band-gap semiconductors serve as a local sensor of multiple degrees of freedom in a variety of "hard" and "soft" condensed matter systems. Taking advantage of the recent progress on quantum sensing using van der Waals (vdW) quantum materials,...

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Main Authors: Zhou, Jingcheng, Lu, Hanyi, Chen, Di, Huang, Mengqi, Yan, Gerald Q, Al-matouq, Faris, Chang, Jiu, Djugba, Dziga, Jiang, Zhigang, Wang, Hailong, Du, Chunhui Rita
Format: Journal Article
Language:English
Published: 01-05-2024
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Abstract Optically active spin defects in wide band-gap semiconductors serve as a local sensor of multiple degrees of freedom in a variety of "hard" and "soft" condensed matter systems. Taking advantage of the recent progress on quantum sensing using van der Waals (vdW) quantum materials, here we report direct measurements of spin waves excited in magnetic insulator Y3Fe5O12 (YIG) by boron vacancy $V_B^-$ spin defects contained in few-layer thick hexagonal boron nitride nanoflakes. We show that the ferromagnetic resonance and parametric spin excitations can be effectively detected by $V_B^-$ spin defects under various experimental conditions through optically detected magnetic resonance measurements. The off-resonant dipole interaction between YIG magnons and $V_B^-$ spin defects is mediated by multi-magnon scattering processes, which may find relevant applications in a range of emerging quantum sensing, computing, and metrology technologies. Our results also highlight the opportunities offered by quantum spin defects in layered two-dimensional vdW materials for investigating local spin dynamic behaviors in magnetic solid-state matters.
AbstractList Optically active spin defects in wide band-gap semiconductors serve as a local sensor of multiple degrees of freedom in a variety of "hard" and "soft" condensed matter systems. Taking advantage of the recent progress on quantum sensing using van der Waals (vdW) quantum materials, here we report direct measurements of spin waves excited in magnetic insulator Y3Fe5O12 (YIG) by boron vacancy $V_B^-$ spin defects contained in few-layer thick hexagonal boron nitride nanoflakes. We show that the ferromagnetic resonance and parametric spin excitations can be effectively detected by $V_B^-$ spin defects under various experimental conditions through optically detected magnetic resonance measurements. The off-resonant dipole interaction between YIG magnons and $V_B^-$ spin defects is mediated by multi-magnon scattering processes, which may find relevant applications in a range of emerging quantum sensing, computing, and metrology technologies. Our results also highlight the opportunities offered by quantum spin defects in layered two-dimensional vdW materials for investigating local spin dynamic behaviors in magnetic solid-state matters.
Author Lu, Hanyi
Du, Chunhui Rita
Chen, Di
Djugba, Dziga
Huang, Mengqi
Wang, Hailong
Yan, Gerald Q
Chang, Jiu
Al-matouq, Faris
Zhou, Jingcheng
Jiang, Zhigang
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  fullname: Du, Chunhui Rita
BackLink https://doi.org/10.48550/arXiv.2405.00802$$DView paper in arXiv
https://doi.org/10.1126/sciadv.adk8495$$DView published paper (Access to full text may be restricted)
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Snippet Optically active spin defects in wide band-gap semiconductors serve as a local sensor of multiple degrees of freedom in a variety of "hard" and "soft"...
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Title Sensing Spin Wave Excitations by Spin Defects in Few-Layer Thick Hexagonal Boron Nitride
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