Evidence of magnetodielectric coupling in multiferroic Pb ( Fe 0.5 Nb 0.5 ) O 3 ceramics from ferroelectric measurements and electron paramagnetic resonance
Magnetodielectric coupling effects of single phase multiferroic Pb ( Fe 0.5 Nb 0.5 ) O 3 ceramics have been studied using standard ferroelectric measurements and electron paramagnetic resonance (EPR). Changes in the electrical polarization behavior were observed in the paramagnetic to weakly magneti...
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| Published in: | Applied physics letters Vol. 93; no. 17; pp. 172902 - 172902-3 |
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| Main Authors: | , , , , |
| Format: | Journal Article |
| Language: | English |
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American Institute of Physics
28-10-2008
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| Abstract | Magnetodielectric coupling effects of single phase multiferroic
Pb
(
Fe
0.5
Nb
0.5
)
O
3
ceramics have been studied using standard ferroelectric measurements and electron paramagnetic resonance (EPR). Changes in the electrical polarization behavior were observed in the paramagnetic to weakly magnetized antiferromagnetic transition near 103 K associated with a rhombohedral to monoclinic symmetry reduction. The analysis of changes in the EPR spectral parameters confirms the transition from paramagnetic to weakly magnetized antiferromagnetic and reveals noticeable anomalies in the high temperature region near the ferroelectric-paraelectric transition (383 K), which are correlated with the tetragonal-to-cubic symmetry change and the characteristic diffuse phase transition of this material. |
|---|---|
| AbstractList | Magnetodielectric coupling effects of single phase multiferroic
Pb
(
Fe
0.5
Nb
0.5
)
O
3
ceramics have been studied using standard ferroelectric measurements and electron paramagnetic resonance (EPR). Changes in the electrical polarization behavior were observed in the paramagnetic to weakly magnetized antiferromagnetic transition near 103 K associated with a rhombohedral to monoclinic symmetry reduction. The analysis of changes in the EPR spectral parameters confirms the transition from paramagnetic to weakly magnetized antiferromagnetic and reveals noticeable anomalies in the high temperature region near the ferroelectric-paraelectric transition (383 K), which are correlated with the tetragonal-to-cubic symmetry change and the characteristic diffuse phase transition of this material. |
| Author | Siqueiros, Jesús M. Raymond, Oscar Alvarez, Guillermo Font, Reynaldo Portelles, Jorge |
| Author_xml | – sequence: 1 givenname: Reynaldo surname: Font fullname: Font, Reynaldo organization: Facultad de Física, Universidad de la Habana, San Lázaro y L, Vedado, La Habana 10400, Cuba – sequence: 2 givenname: Guillermo surname: Alvarez fullname: Alvarez, Guillermo organization: Facultad de Física, Universidad de la Habana, San Lázaro y L, Vedado, La Habana 10400, Cuba – sequence: 3 givenname: Oscar surname: Raymond fullname: Raymond, Oscar email: raymond@cnyn.unam.mx. organization: Facultad de Física, Universidad de la Habana, San Lázaro y L, Vedado, La Habana 10400, Cuba – sequence: 4 givenname: Jorge surname: Portelles fullname: Portelles, Jorge organization: Facultad de Física, Universidad de la Habana, San Lázaro y L, Vedado, La Habana 10400, Cuba – sequence: 5 givenname: Jesús surname: Siqueiros middlename: M. fullname: Siqueiros, Jesús M. organization: Facultad de Física, Universidad de la Habana, San Lázaro y L, Vedado, La Habana 10400, Cuba |
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| Cites_doi | 10.1063/1.2201853 10.1063/1.2359581 10.1103/PhysRevB.65.024410 10.1016/j.jallcom.2003.09.058 10.1016/S1369-7021(07)70241-9 10.1103/PhysRevB.70.132101 10.1038/nmat1868 10.1103/PhysRevB.65.220407 10.1063/1.1870100 10.1038/nmat1860 10.1038/nmat1886 10.1063/1.1870099 10.1088/0953-8984/11/17/307 10.1063/1.2357926 10.1103/PhysRev.82.285.2 10.1023/A:1004815416774 10.1088/0953-8984/12/11/305 |
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| Copyright | 2008 American Institute of Physics |
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| DOI | 10.1063/1.3006433 |
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| References | Lampis, N.; Sciau, P.; Lehmann, A. 1999; 11 Ramesh, R.; Spaldin, N. 2007; 6 Scott, J. 2007; 6 English, S.; Wu, J.; Leighton, C. 2002; 65 Chu, Y.; Martin, L.; Holcomb, M.; Ramesh, R. 2007; 10 Varshney, D.; Choudhary, R.; Katiyar, R. 2006; 89 Yang, Y.; Liu, J.; Huang, H.; Zou, W.; Bao, P.; Liu, Z. 2004; 70 Raymond, O.; Font, R.; Suárez-Almodovar, N.; Portelles, J.; Siqueiros, J. 2006; 99 Montiel, H.; Alvarez, G.; Betancourt, I.; Zamorano, R.; Valenzuela, R. 2006; 384 Eerenstein, W.; Wiora, M.; Prieto, J.; Scott, J.; Mathur, N. 2007; 6 Ivanov, S.; Tellgreen, R.; Rundlof, H.; Thomas, N.; Ananta, S. 2000; 12 Yan, L.; Li, J.; Suchicital, C.; Viehland, D. 2006; 89 Okamura, T.; Torizuka, Y.; Kojima, Y. 1951; 82 Joshi, J.; Gupta, R.; Sood, A.; Bhat, S.; Raju, A.; Rao, C. 2001; 65 Gajek, M.; Bibes, M.; Fusil, S.; Bouzehouane, K.; Fontcuberta, J.; Barthelemy, A.; Fert, A. 2007; 6 Raymond, O.; Font, R.; Suárez-Almodovar, N.; Portelles, J.; Siqueiros, J. 2005; 97 Gao, X.; Chen, X.; Yin, J.; Wu, J.; Liu, Z.; Wang, M. 2000; 35 Alvarez, G.; Zamorano, R. 2004; 369 |
| References_xml | – volume: 99 start-page: 124101 year: 2006 publication-title: J. Appl. Phys. doi: 10.1063/1.2201853 contributor: fullname: Raymond, O.; Font, R.; Suárez-Almodovar, N.; Portelles, J.; Siqueiros, J. – volume: 89 start-page: 172901 year: 2006 publication-title: Appl. Phys. Lett. doi: 10.1063/1.2359581 contributor: fullname: Varshney, D.; Choudhary, R.; Katiyar, R. – volume: 65 start-page: 024410 year: 2001 publication-title: Phys. Rev. B doi: 10.1103/PhysRevB.65.024410 contributor: fullname: Joshi, J.; Gupta, R.; Sood, A.; Bhat, S.; Raju, A.; Rao, C. – volume: 369 start-page: 231 year: 2004 publication-title: J. Alloys Compd. doi: 10.1016/j.jallcom.2003.09.058 contributor: fullname: Alvarez, G.; Zamorano, R. – volume: 10 start-page: 16 year: 2007 publication-title: Mater. Today doi: 10.1016/S1369-7021(07)70241-9 contributor: fullname: Chu, Y.; Martin, L.; Holcomb, M.; Ramesh, R. – volume: 70 start-page: 132101 year: 2004 publication-title: Phys. Rev. B doi: 10.1103/PhysRevB.70.132101 contributor: fullname: Yang, Y.; Liu, J.; Huang, H.; Zou, W.; Bao, P.; Liu, Z. – volume: 6 start-page: 256 year: 2007 publication-title: Nature Mater. doi: 10.1038/nmat1868 contributor: fullname: Scott, J. – volume: 65 start-page: 220407 year: 2002 publication-title: Phys. Rev. B doi: 10.1103/PhysRevB.65.220407 contributor: fullname: English, S.; Wu, J.; Leighton, C. – volume: 97 start-page: 084108 year: 2005 publication-title: J. Appl. Phys. doi: 10.1063/1.1870100 contributor: fullname: Raymond, O.; Font, R.; Suárez-Almodovar, N.; Portelles, J.; Siqueiros, J. – volume: 6 start-page: 296 year: 2007 publication-title: Nature Mater. doi: 10.1038/nmat1860 contributor: fullname: Gajek, M.; Bibes, M.; Fusil, S.; Bouzehouane, K.; Fontcuberta, J.; Barthelemy, A.; Fert, A. – volume: 6 start-page: 348 year: 2007 publication-title: Nature Mater. doi: 10.1038/nmat1886 contributor: fullname: Eerenstein, W.; Wiora, M.; Prieto, J.; Scott, J.; Mathur, N. – volume: 97 start-page: 084107 year: 2005 publication-title: J. Appl. Phys. doi: 10.1063/1.1870099 contributor: fullname: Raymond, O.; Font, R.; Suárez-Almodovar, N.; Portelles, J.; Siqueiros, J. – volume: 6 start-page: 21 year: 2007 publication-title: Nature Mater. contributor: fullname: Ramesh, R.; Spaldin, N. – volume: 384 start-page: 297 year: 2006 publication-title: Physica B (Amsterdam) contributor: fullname: Montiel, H.; Alvarez, G.; Betancourt, I.; Zamorano, R.; Valenzuela, R. – volume: 11 start-page: 3489 year: 1999 publication-title: J. Phys.: Condens. Matter doi: 10.1088/0953-8984/11/17/307 contributor: fullname: Lampis, N.; Sciau, P.; Lehmann, A. – volume: 89 start-page: 132913 year: 2006 publication-title: Appl. Phys. Lett. doi: 10.1063/1.2357926 contributor: fullname: Yan, L.; Li, J.; Suchicital, C.; Viehland, D. – volume: 82 start-page: 285 year: 1951 publication-title: Phys. Rev. doi: 10.1103/PhysRev.82.285.2 contributor: fullname: Okamura, T.; Torizuka, Y.; Kojima, Y. – volume: 35 start-page: 5421 year: 2000 publication-title: J. Mater. Sci. doi: 10.1023/A:1004815416774 contributor: fullname: Gao, X.; Chen, X.; Yin, J.; Wu, J.; Liu, Z.; Wang, M. – volume: 12 start-page: 2393 year: 2000 publication-title: J. Phys.: Condens. Matter doi: 10.1088/0953-8984/12/11/305 contributor: fullname: Ivanov, S.; Tellgreen, R.; Rundlof, H.; Thomas, N.; Ananta, S. |
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| Snippet | Magnetodielectric coupling effects of single phase multiferroic
Pb
(
Fe
0.5
Nb
0.5
)
O
3
ceramics have been studied using standard ferroelectric measurements... |
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| StartPage | 172902 |
| Title | Evidence of magnetodielectric coupling in multiferroic Pb ( Fe 0.5 Nb 0.5 ) O 3 ceramics from ferroelectric measurements and electron paramagnetic resonance |
| URI | http://dx.doi.org/10.1063/1.3006433 |
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