Low-dimensional spin S = 1/2 system at the quantum critical limit: Na2V3O7

We report the results of measurements of the dc susceptibility and the 23Na-NMR response of Na2V3O7, a recently synthesized, nonmetallic low dimensional spin system. Our results indicate that, upon reducing the temperature to below 100 K, the V4+ moments are gradually quenched, leaving only one mome...

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Bibliographic Details
Published in:Physical review letters Vol. 90; no. 16; p. 167202
Main Authors: Gavilano, J L, Rau, D, Mushkolaj, S, Ott, H R, Millet, P, Mila, F
Format: Journal Article
Language:English
Published: United States 25-04-2003
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Summary:We report the results of measurements of the dc susceptibility and the 23Na-NMR response of Na2V3O7, a recently synthesized, nonmetallic low dimensional spin system. Our results indicate that, upon reducing the temperature to below 100 K, the V4+ moments are gradually quenched, leaving only one moment out of nine active. The NMR data reveal a phase transition at very low temperatures. With decreasing applied field H, the critical temperature shifts towards T=0 K, suggesting that Na2V3O7 may be regarded as an insulator reaching a quantum critical point at H=0.
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ISSN:0031-9007
DOI:10.1103/PhysRevLett.90.167202