Improved Electrical Properties of Solution-Processed ZrO2 Gate Dielectric for Large-Area Flexible Electronics
Zirconium oxide (ZrO 2 ), which has high dielectric constant, was investigated for application in flexible electronics. When the spun-cast film was annealed at a low temperature, the electrical properties were not encouraging because residual organic particles remained at the dielectric. To address...
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Published in: | Jpn J Appl Phys Vol. 52; no. 10; pp. 100206 - 100206-3 |
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The Japan Society of Applied Physics
01-10-2013
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Abstract | Zirconium oxide (ZrO 2 ), which has high dielectric constant, was investigated for application in flexible electronics. When the spun-cast film was annealed at a low temperature, the electrical properties were not encouraging because residual organic particles remained at the dielectric. To address this problem we used plasma annealing at a reasonably low temperature and achieved improved dielectric properties such as lower leakage current, higher dielectric constant, and better reliability. Auger depth profile spectroscopy results suggested reduction of carbon percentage at the dielectric. We demonstrated device application by fabricating transistor device with an organic channel layer. The transistor electrical properties were encouraging, exhibiting an electron mobility of 0.3 cm 2 /(V$\cdot$s). The results were very promising and suggest that ZrO 2 could be applied to all-printed electronic devices in the near future. |
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AbstractList | Zirconium oxide (ZrO 2 ), which has high dielectric constant, was investigated for application in flexible electronics. When the spun-cast film was annealed at a low temperature, the electrical properties were not encouraging because residual organic particles remained at the dielectric. To address this problem we used plasma annealing at a reasonably low temperature and achieved improved dielectric properties such as lower leakage current, higher dielectric constant, and better reliability. Auger depth profile spectroscopy results suggested reduction of carbon percentage at the dielectric. We demonstrated device application by fabricating transistor device with an organic channel layer. The transistor electrical properties were encouraging, exhibiting an electron mobility of 0.3 cm 2 /(V$\cdot$s). The results were very promising and suggest that ZrO 2 could be applied to all-printed electronic devices in the near future. |
Author | Jeong, Jae Kyeong Kim, Dong-Hyoub Yang, Hoichang Jang, Mi Nguyen, Manh Cuong Hasan, Musarrat Choi, Rino |
Author_xml | – sequence: 1 givenname: Musarrat surname: Hasan fullname: Hasan, Musarrat organization: Department of Materials Science and Engineering, Inha University, Incheon 402-751, Republic of Korea – sequence: 2 givenname: Mi surname: Jang fullname: Jang, Mi organization: Department of Advanced Fiber Engineering, Inha University, Incheon 402-751, Republic of Korea – sequence: 3 givenname: Dong-Hyoub surname: Kim fullname: Kim, Dong-Hyoub organization: Department of Materials Science and Engineering, Inha University, Incheon 402-751, Republic of Korea – sequence: 4 givenname: Manh Cuong surname: Nguyen fullname: Nguyen, Manh Cuong organization: Department of Materials Science and Engineering, Inha University, Incheon 402-751, Republic of Korea – sequence: 5 givenname: Hoichang surname: Yang fullname: Yang, Hoichang organization: Department of Advanced Fiber Engineering, Inha University, Incheon 402-751, Republic of Korea – sequence: 6 givenname: Jae Kyeong surname: Jeong fullname: Jeong, Jae Kyeong organization: Department of Materials Science and Engineering, Inha University, Incheon 402-751, Republic of Korea – sequence: 7 givenname: Rino surname: Choi fullname: Choi, Rino organization: Department of Materials Science and Engineering, Inha University, Incheon 402-751, Republic of Korea |
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ContentType | Journal Article |
DOI | 10.7567/JJAP.52.100206 |
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Notes | (Color online) (a) Auger electron depth profiles for ZrO 2 films plasma annealed under various conditions. Plasma annealing was performed for 1 h. (b) Leakage current density of capacitors annealed at 250 °C in O 2 plasma for various lengths of time. (Color online) (a) Capacitance densities for ZrO 2 films annealed at 250 °C in O 2 plasma for various length of time and compared them with device annealed at 250 °C for 60 min in O 2 atmosphere. (b) Current densities and EOTs for various films annealed at 250 °C for various lengths of time. (Color online) (a) Changes in interface trap density of ZrO 2 capacitor and in hysteresis with various lengths of plasma annealing time. (b) Change in flat-band voltage with application of prolonged negative bias stress. (Color online) (a) Transfer and (b) output characteristics of solution-processed TES-ADT TFT with plasma-annealed ZrO 2 as gate dielectric. |
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PublicationDate | 2013-10-01 |
PublicationDateYYYYMMDD | 2013-10-01 |
PublicationDate_xml | – month: 10 year: 2013 text: 2013-10-01 day: 01 |
PublicationDecade | 2010 |
PublicationTitle | Jpn J Appl Phys |
PublicationYear | 2013 |
Publisher | The Japan Society of Applied Physics |
Publisher_xml | – name: The Japan Society of Applied Physics |
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Snippet | Zirconium oxide (ZrO 2 ), which has high dielectric constant, was investigated for application in flexible electronics. When the spun-cast film was annealed at... |
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Title | Improved Electrical Properties of Solution-Processed ZrO2 Gate Dielectric for Large-Area Flexible Electronics |
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