Self‐Assembly of 2D Hybrid Double Perovskites on 3D Cs 2 AgBiBr 6 Crystals towards Ultrasensitive Detection of Weak Polarized Light
We report the self‐assembly of 2D double perovskite (BLA) 2 CsAgBiBr 7 (BLA=benzylammonium) on 3D Cs 2 AgBiBr 6 crystals, providing the first demonstration of polarization‐sensitive photodetection using lead‐free double perovskite heterocrystals (HCs). The (BLA) 2 CsAgBiBr 7 /Cs 2 AgBiBr 6 HC succes...
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| Published in: | Angewandte Chemie Vol. 134; no. 32 |
|---|---|
| Main Authors: | , , , , , |
| Format: | Journal Article |
| Language: | English |
| Published: |
08-08-2022
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| Abstract | We report the self‐assembly of 2D double perovskite (BLA)
2
CsAgBiBr
7
(BLA=benzylammonium) on 3D Cs
2
AgBiBr
6
crystals, providing the first demonstration of polarization‐sensitive photodetection using lead‐free double perovskite heterocrystals (HCs). The (BLA)
2
CsAgBiBr
7
/Cs
2
AgBiBr
6
HC successfully combines the anisotropy of 2D double perovskites with the well‐defined interface provided by heterogeneous integration. Driven by the built‐in electric field in junction, photodetectors of HCs exhibit unique polarization dependence of zero‐bias photocurrent with a large anisotropy ratio up to 9, which is 6 times amplified as compared to the pristine 2D (BLA)
2
CsAgBiBr
7
. More importantly, the present devices can remain polarization‐sensitive with incident light intensity down to the nW cm
−2
level. Our study on lead‐free hybrid perovskite HCs marks a step toward establishing robust material foundations for fundamental scientific investigations and the development of optoelectronic devices. |
|---|---|
| AbstractList | We report the self‐assembly of 2D double perovskite (BLA)
2
CsAgBiBr
7
(BLA=benzylammonium) on 3D Cs
2
AgBiBr
6
crystals, providing the first demonstration of polarization‐sensitive photodetection using lead‐free double perovskite heterocrystals (HCs). The (BLA)
2
CsAgBiBr
7
/Cs
2
AgBiBr
6
HC successfully combines the anisotropy of 2D double perovskites with the well‐defined interface provided by heterogeneous integration. Driven by the built‐in electric field in junction, photodetectors of HCs exhibit unique polarization dependence of zero‐bias photocurrent with a large anisotropy ratio up to 9, which is 6 times amplified as compared to the pristine 2D (BLA)
2
CsAgBiBr
7
. More importantly, the present devices can remain polarization‐sensitive with incident light intensity down to the nW cm
−2
level. Our study on lead‐free hybrid perovskite HCs marks a step toward establishing robust material foundations for fundamental scientific investigations and the development of optoelectronic devices. |
| Author | Wu, Jianbo Yao, Yunpeng Liang, Lishan Zhang, Xinyuan Luo, Junhua Niu, Xinyi |
| Author_xml | – sequence: 1 givenname: Xinyuan surname: Zhang fullname: Zhang, Xinyuan organization: State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences Fuzhou Fujian 350002 China, University of Chinese Academy of Sciences Beijing 100049 China – sequence: 2 givenname: Yunpeng surname: Yao fullname: Yao, Yunpeng organization: State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences Fuzhou Fujian 350002 China – sequence: 3 givenname: Lishan surname: Liang fullname: Liang, Lishan organization: State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences Fuzhou Fujian 350002 China – sequence: 4 givenname: Xinyi surname: Niu fullname: Niu, Xinyi organization: State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences Fuzhou Fujian 350002 China – sequence: 5 givenname: Jianbo surname: Wu fullname: Wu, Jianbo organization: State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences Fuzhou Fujian 350002 China – sequence: 6 givenname: Junhua orcidid: 0000-0002-3179-7652 surname: Luo fullname: Luo, Junhua organization: State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences Fuzhou Fujian 350002 China, School of Chemistry and Chemical Engineering Jiangxi Normal University Nanchang 330022 China, University of Chinese Academy of Sciences Beijing 100049 China |
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| Snippet | We report the self‐assembly of 2D double perovskite (BLA)
2
CsAgBiBr
7
(BLA=benzylammonium) on 3D Cs
2
AgBiBr
6
crystals, providing the first demonstration of... |
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| Title | Self‐Assembly of 2D Hybrid Double Perovskites on 3D Cs 2 AgBiBr 6 Crystals towards Ultrasensitive Detection of Weak Polarized Light |
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