Shelf‐basin exchange times of Arctic surface waters estimated from 228 Th/ 228 Ra disequilibrium

The transpolar drift is strongly enriched in 228 Ra accumulated on the wide Arctic shelves with subsequent rapid offshore transport. We present new data of Polarstern expeditions to the central Arctic and to the Kara and Laptev seas. Because 226 Ra activities in Pacific waters are 30% higher than in...

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Bibliographic Details
Published in:Journal of Geophysical Research: Oceans Vol. 117; no. C3
Main Authors: Rutgers van der Loeff, M., Cai, P., Stimac, I., Bauch, D., Hanfland, C., Roeske, T., Moran, S. B.
Format: Journal Article
Language:English
Published: 01-03-2012
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Summary:The transpolar drift is strongly enriched in 228 Ra accumulated on the wide Arctic shelves with subsequent rapid offshore transport. We present new data of Polarstern expeditions to the central Arctic and to the Kara and Laptev seas. Because 226 Ra activities in Pacific waters are 30% higher than in Atlantic waters, we correct 226 Ra for the Pacific admixture when normalizing 228 Ra with 226 Ra. The use of 228 Ra decay as age marker critically depends on the constancy in space and time of the source activity, a condition that has not yet adequately been tested. While 228 Ra decays during transit over the central basin, ingrowth of 228 Th could provide an alternative age marker. The high 228 Th/ 228 Ra activity ratio (AR = 0.8–1.0) in the central basins is incompatible with a mixing model based on horizontal eddy diffusion. An advective model predicts that 228 Th grows to an equilibrium AR, the value of which depends on the scavenging regime. The low AR over the Lomonosov Ridge (AR = 0.5) can be due to either rapid transport (minimum age without scavenging 1.1 year) or enhanced scavenging. Suspended particulate matter load (derived from beam transmission and particulate 234 Th) and total 234 Th depletion data show that scavenging, although extremely low in the central Arctic, is enhanced over the Lomonosov Ridge, making an age of 3 years more likely. The combined data of 228 Ra decay and 228 Th ingrowth confirm the existence of a recirculating gyre in the surface water of the eastern Eurasian Basin with a river water residence time of at least 3 years. Key Points 228Ra on Arctic shelves may not be sufficiently constant to serve as age marker 228Th ingrowth provides independent age information High 228Th/228Ra age infers a recirculating gyre above the Gakkel Ridge
ISSN:0148-0227
DOI:10.1029/2011JC007478