Adsorptive removal of heavy metals from wastewater using Cobalt-diphenylamine (Co-DPA) complex

Adsorptive removal of heavy metals from wastewater using Cobalt-diphenylamine (Co-DPA) complex

Heavy metals like Cadmium, Lead, and Chromium are the pollutants emitted into the environment through industrial development. In this work, a new diphenylamine coordinated cobalt complex (Co-DPA) has been synthesized and tested for its efficiency in removing heavy metals from wastewater, and its ads...

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Published in:BMC chemistry Vol. 18; no. 1; pp. 23 - 15
Main Authors: Yimer, Mesfin, Ansari, Shagufi Naz, Berehe, Biniyam Abdu, Gudimella, Krishna Kanthi, Gedda, Gangaraju, Girma, Wubshet Mekonnen, Hasan, Nazim, Tasneem, Shadma
Format: Journal Article
Language:English
Published: Cham Springer International Publishing 29-01-2024
BioMed Central Ltd
Springer Nature B.V
BMC
Subjects:
Adsorbents
Adsorption
Adsorptivity
Cadmium
Chemistry
Chemistry and Materials Science
Chemistry/Food Science
Cobalt
Cobalt compounds
Cu-DPA
Economic development
Freundlich isotherm
Heavy metals
Industrial development
Lead
Metal industry
Purification
Real estate development
Real sample
Sewage
Trivalent chromium
Wastewater
Wastewater treatment
Cu-DPA
Real sample
Adsorption
Wastewater
Freundlich isotherm
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Abstract Heavy metals like Cadmium, Lead, and Chromium are the pollutants emitted into the environment through industrial development. In this work, a new diphenylamine coordinated cobalt complex (Co-DPA) has been synthesized and tested for its efficiency in removing heavy metals from wastewater, and its adsorption capacity was investigated. The effectiveness of heavy metals removal by Co-DPA was evaluated by adjusting the adsorption parameters, such as adsorbent dose, pH, initial metals concentration, and adsorption period. Heavy metal concentrations in real sample were 0.267, 0.075, and 0.125 mg/L for Cd 2+ , Pb 2+ , and Cr 3+ before using as-synthesized Co-DPA to treat wastewater. After being treated with synthesized Co-DPA the concentration of heavy metals was reduced to 0.0129, 0.00028, 0.00054 mg/L for Cd 2+ , Pb 2+ , and Cr 3+ , respectively, in 80 min. The removal efficiency was 95.6%, 99.5%, and 99.5% for the respective metals. The adsorption process fitted satisfactorily with Freundlich isotherm with R 2 (0.999, 0.997, 0.995) for Cd 2+ , Pb 2+ , and Cr 3+ , respectively. The kinetic data obeyed the pseudo-second order for Cd 2+ and Cr 2+ and the pseudo-first order for Pb 2+ . Based on the results obtained within the framework of this study, it is concluded that the as-synthesized Co-DPA is a good adsorbent to eliminate heavy metal ions like Cd 2+ , Pb 2+ , and Cr 3+ from wastewater solution. In general, Co-DPA is a promising new material for the removal of heavy metal ions from water. Graphical Abstract
AbstractList Heavy metals like Cadmium, Lead, and Chromium are the pollutants emitted into the environment through industrial development. In this work, a new diphenylamine coordinated cobalt complex (Co-DPA) has been synthesized and tested for its efficiency in removing heavy metals from wastewater, and its adsorption capacity was investigated. The effectiveness of heavy metals removal by Co-DPA was evaluated by adjusting the adsorption parameters, such as adsorbent dose, pH, initial metals concentration, and adsorption period. Heavy metal concentrations in real sample were 0.267, 0.075, and 0.125 mg/L for Cd.sup.2+, Pb.sup.2+, and Cr.sup.3+ before using as-synthesized Co-DPA to treat wastewater. After being treated with synthesized Co-DPA the concentration of heavy metals was reduced to 0.0129, 0.00028, 0.00054 mg/L for Cd.sup.2+, Pb.sup.2+, and Cr.sup.3+, respectively, in 80 min. The removal efficiency was 95.6%, 99.5%, and 99.5% for the respective metals. The adsorption process fitted satisfactorily with Freundlich isotherm with R.sup.2(0.999, 0.997, 0.995) for Cd.sup.2+, Pb.sup.2+, and Cr.sup.3+, respectively. The kinetic data obeyed the pseudo-second order for Cd.sup.2+ and Cr.sup.2+ and the pseudo-first order for Pb.sup.2+. Based on the results obtained within the framework of this study, it is concluded that the as-synthesized Co-DPA is a good adsorbent to eliminate heavy metal ions like Cd.sup.2+, Pb.sup.2+, and Cr.sup.3+from wastewater solution. In general, Co-DPA is a promising new material for the removal of heavy metal ions from water.
Abstract Heavy metals like Cadmium, Lead, and Chromium are the pollutants emitted into the environment through industrial development. In this work, a new diphenylamine coordinated cobalt complex (Co-DPA) has been synthesized and tested for its efficiency in removing heavy metals from wastewater, and its adsorption capacity was investigated. The effectiveness of heavy metals removal by Co-DPA was evaluated by adjusting the adsorption parameters, such as adsorbent dose, pH, initial metals concentration, and adsorption period. Heavy metal concentrations in real sample were 0.267, 0.075, and 0.125 mg/L for Cd2+, Pb2+, and Cr3+ before using as-synthesized Co-DPA to treat wastewater. After being treated with synthesized Co-DPA the concentration of heavy metals was reduced to 0.0129, 0.00028, 0.00054 mg/L for Cd2+, Pb2+, and Cr3+, respectively, in 80 min. The removal efficiency was 95.6%, 99.5%, and 99.5% for the respective metals. The adsorption process fitted satisfactorily with Freundlich isotherm with R2(0.999, 0.997, 0.995) for Cd2+, Pb2+, and Cr3+, respectively. The kinetic data obeyed the pseudo-second order for Cd2+ and Cr2+ and the pseudo-first order for Pb2+. Based on the results obtained within the framework of this study, it is concluded that the as-synthesized Co-DPA is a good adsorbent to eliminate heavy metal ions like Cd2+, Pb2+, and Cr3+from wastewater solution. In general, Co-DPA is a promising new material for the removal of heavy metal ions from water. Graphical Abstract
Heavy metals like Cadmium, Lead, and Chromium are the pollutants emitted into the environment through industrial development. In this work, a new diphenylamine coordinated cobalt complex (Co-DPA) has been synthesized and tested for its efficiency in removing heavy metals from wastewater, and its adsorption capacity was investigated. The effectiveness of heavy metals removal by Co-DPA was evaluated by adjusting the adsorption parameters, such as adsorbent dose, pH, initial metals concentration, and adsorption period. Heavy metal concentrations in real sample were 0.267, 0.075, and 0.125 mg/L for Cd , Pb , and Cr before using as-synthesized Co-DPA to treat wastewater. After being treated with synthesized Co-DPA the concentration of heavy metals was reduced to 0.0129, 0.00028, 0.00054 mg/L for Cd , Pb , and Cr , respectively, in 80 min. The removal efficiency was 95.6%, 99.5%, and 99.5% for the respective metals. The adsorption process fitted satisfactorily with Freundlich isotherm with R (0.999, 0.997, 0.995) for Cd , Pb , and Cr , respectively. The kinetic data obeyed the pseudo-second order for Cd and Cr and the pseudo-first order for Pb . Based on the results obtained within the framework of this study, it is concluded that the as-synthesized Co-DPA is a good adsorbent to eliminate heavy metal ions like Cd , Pb , and Cr from wastewater solution. In general, Co-DPA is a promising new material for the removal of heavy metal ions from water.
Heavy metals like Cadmium, Lead, and Chromium are the pollutants emitted into the environment through industrial development. In this work, a new diphenylamine coordinated cobalt complex (Co-DPA) has been synthesized and tested for its efficiency in removing heavy metals from wastewater, and its adsorption capacity was investigated. The effectiveness of heavy metals removal by Co-DPA was evaluated by adjusting the adsorption parameters, such as adsorbent dose, pH, initial metals concentration, and adsorption period. Heavy metal concentrations in real sample were 0.267, 0.075, and 0.125 mg/L for Cd 2+ , Pb 2+ , and Cr 3+ before using as-synthesized Co-DPA to treat wastewater. After being treated with synthesized Co-DPA the concentration of heavy metals was reduced to 0.0129, 0.00028, 0.00054 mg/L for Cd 2+ , Pb 2+ , and Cr 3+ , respectively, in 80 min. The removal efficiency was 95.6%, 99.5%, and 99.5% for the respective metals. The adsorption process fitted satisfactorily with Freundlich isotherm with R 2 (0.999, 0.997, 0.995) for Cd 2+ , Pb 2+ , and Cr 3+ , respectively. The kinetic data obeyed the pseudo-second order for Cd 2+ and Cr 2+ and the pseudo-first order for Pb 2+ . Based on the results obtained within the framework of this study, it is concluded that the as-synthesized Co-DPA is a good adsorbent to eliminate heavy metal ions like Cd 2+ , Pb 2+ , and Cr 3+ from wastewater solution. In general, Co-DPA is a promising new material for the removal of heavy metal ions from water.
Heavy metals like Cadmium, Lead, and Chromium are the pollutants emitted into the environment through industrial development. In this work, a new diphenylamine coordinated cobalt complex (Co-DPA) has been synthesized and tested for its efficiency in removing heavy metals from wastewater, and its adsorption capacity was investigated. The effectiveness of heavy metals removal by Co-DPA was evaluated by adjusting the adsorption parameters, such as adsorbent dose, pH, initial metals concentration, and adsorption period. Heavy metal concentrations in real sample were 0.267, 0.075, and 0.125 mg/L for Cd.sup.2+, Pb.sup.2+, and Cr.sup.3+ before using as-synthesized Co-DPA to treat wastewater. After being treated with synthesized Co-DPA the concentration of heavy metals was reduced to 0.0129, 0.00028, 0.00054 mg/L for Cd.sup.2+, Pb.sup.2+, and Cr.sup.3+, respectively, in 80 min. The removal efficiency was 95.6%, 99.5%, and 99.5% for the respective metals. The adsorption process fitted satisfactorily with Freundlich isotherm with R.sup.2(0.999, 0.997, 0.995) for Cd.sup.2+, Pb.sup.2+, and Cr.sup.3+, respectively. The kinetic data obeyed the pseudo-second order for Cd.sup.2+ and Cr.sup.2+ and the pseudo-first order for Pb.sup.2+. Based on the results obtained within the framework of this study, it is concluded that the as-synthesized Co-DPA is a good adsorbent to eliminate heavy metal ions like Cd.sup.2+, Pb.sup.2+, and Cr.sup.3+from wastewater solution. In general, Co-DPA is a promising new material for the removal of heavy metal ions from water. Graphical Keywords: Wastewater, Adsorption, Cu-DPA, Real sample, Freundlich isotherm
Heavy metals like Cadmium, Lead, and Chromium are the pollutants emitted into the environment through industrial development. In this work, a new diphenylamine coordinated cobalt complex (Co-DPA) has been synthesized and tested for its efficiency in removing heavy metals from wastewater, and its adsorption capacity was investigated. The effectiveness of heavy metals removal by Co-DPA was evaluated by adjusting the adsorption parameters, such as adsorbent dose, pH, initial metals concentration, and adsorption period. Heavy metal concentrations in real sample were 0.267, 0.075, and 0.125 mg/L for Cd2+, Pb2+, and Cr3+ before using as-synthesized Co-DPA to treat wastewater. After being treated with synthesized Co-DPA the concentration of heavy metals was reduced to 0.0129, 0.00028, 0.00054 mg/L for Cd2+, Pb2+, and Cr3+, respectively, in 80 min. The removal efficiency was 95.6%, 99.5%, and 99.5% for the respective metals. The adsorption process fitted satisfactorily with Freundlich isotherm with R2(0.999, 0.997, 0.995) for Cd2+, Pb2+, and Cr3+, respectively. The kinetic data obeyed the pseudo-second order for Cd2+ and Cr2+ and the pseudo-first order for Pb2+. Based on the results obtained within the framework of this study, it is concluded that the as-synthesized Co-DPA is a good adsorbent to eliminate heavy metal ions like Cd2+, Pb2+, and Cr3+from wastewater solution. In general, Co-DPA is a promising new material for the removal of heavy metal ions from water.
Heavy metals like Cadmium, Lead, and Chromium are the pollutants emitted into the environment through industrial development. In this work, a new diphenylamine coordinated cobalt complex (Co-DPA) has been synthesized and tested for its efficiency in removing heavy metals from wastewater, and its adsorption capacity was investigated. The effectiveness of heavy metals removal by Co-DPA was evaluated by adjusting the adsorption parameters, such as adsorbent dose, pH, initial metals concentration, and adsorption period. Heavy metal concentrations in real sample were 0.267, 0.075, and 0.125 mg/L for Cd 2+ , Pb 2+ , and Cr 3+ before using as-synthesized Co-DPA to treat wastewater. After being treated with synthesized Co-DPA the concentration of heavy metals was reduced to 0.0129, 0.00028, 0.00054 mg/L for Cd 2+ , Pb 2+ , and Cr 3+ , respectively, in 80 min. The removal efficiency was 95.6%, 99.5%, and 99.5% for the respective metals. The adsorption process fitted satisfactorily with Freundlich isotherm with R 2 (0.999, 0.997, 0.995) for Cd 2+ , Pb 2+ , and Cr 3+ , respectively. The kinetic data obeyed the pseudo-second order for Cd 2+ and Cr 2+ and the pseudo-first order for Pb 2+ . Based on the results obtained within the framework of this study, it is concluded that the as-synthesized Co-DPA is a good adsorbent to eliminate heavy metal ions like Cd 2+ , Pb 2+ , and Cr 3+ from wastewater solution. In general, Co-DPA is a promising new material for the removal of heavy metal ions from water. Graphical Abstract
Heavy metals like Cadmium, Lead, and Chromium are the pollutants emitted into the environment through industrial development. In this work, a new diphenylamine coordinated cobalt complex (Co-DPA) has been synthesized and tested for its efficiency in removing heavy metals from wastewater, and its adsorption capacity was investigated. The effectiveness of heavy metals removal by Co-DPA was evaluated by adjusting the adsorption parameters, such as adsorbent dose, pH, initial metals concentration, and adsorption period. Heavy metal concentrations in real sample were 0.267, 0.075, and 0.125 mg/L for Cd2+, Pb2+, and Cr3+ before using as-synthesized Co-DPA to treat wastewater. After being treated with synthesized Co-DPA the concentration of heavy metals was reduced to 0.0129, 0.00028, 0.00054 mg/L for Cd2+, Pb2+, and Cr3+, respectively, in 80 min. The removal efficiency was 95.6%, 99.5%, and 99.5% for the respective metals. The adsorption process fitted satisfactorily with Freundlich isotherm with R2(0.999, 0.997, 0.995) for Cd2+, Pb2+, and Cr3+, respectively. The kinetic data obeyed the pseudo-second order for Cd2+ and Cr2+ and the pseudo-first order for Pb2+. Based on the results obtained within the framework of this study, it is concluded that the as-synthesized Co-DPA is a good adsorbent to eliminate heavy metal ions like Cd2+, Pb2+, and Cr3+from wastewater solution. In general, Co-DPA is a promising new material for the removal of heavy metal ions from water.Heavy metals like Cadmium, Lead, and Chromium are the pollutants emitted into the environment through industrial development. In this work, a new diphenylamine coordinated cobalt complex (Co-DPA) has been synthesized and tested for its efficiency in removing heavy metals from wastewater, and its adsorption capacity was investigated. The effectiveness of heavy metals removal by Co-DPA was evaluated by adjusting the adsorption parameters, such as adsorbent dose, pH, initial metals concentration, and adsorption period. Heavy metal concentrations in real sample were 0.267, 0.075, and 0.125 mg/L for Cd2+, Pb2+, and Cr3+ before using as-synthesized Co-DPA to treat wastewater. After being treated with synthesized Co-DPA the concentration of heavy metals was reduced to 0.0129, 0.00028, 0.00054 mg/L for Cd2+, Pb2+, and Cr3+, respectively, in 80 min. The removal efficiency was 95.6%, 99.5%, and 99.5% for the respective metals. The adsorption process fitted satisfactorily with Freundlich isotherm with R2(0.999, 0.997, 0.995) for Cd2+, Pb2+, and Cr3+, respectively. The kinetic data obeyed the pseudo-second order for Cd2+ and Cr2+ and the pseudo-first order for Pb2+. Based on the results obtained within the framework of this study, it is concluded that the as-synthesized Co-DPA is a good adsorbent to eliminate heavy metal ions like Cd2+, Pb2+, and Cr3+from wastewater solution. In general, Co-DPA is a promising new material for the removal of heavy metal ions from water.
ArticleNumber 23
Audience Academic
Author Ansari, Shagufi Naz
Berehe, Biniyam Abdu
Tasneem, Shadma
Hasan, Nazim
Girma, Wubshet Mekonnen
Yimer, Mesfin
Gudimella, Krishna Kanthi
Gedda, Gangaraju
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BackLink https://www.ncbi.nlm.nih.gov/pubmed/38287347$$D View this record in MEDLINE/PubMed
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Issue 1
Keywords Cu-DPA
Real sample
Adsorption
Wastewater
Freundlich isotherm
Language English
License 2024. The Author(s).
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Snippet Heavy metals like Cadmium, Lead, and Chromium are the pollutants emitted into the environment through industrial development. In this work, a new diphenylamine...
Abstract Heavy metals like Cadmium, Lead, and Chromium are the pollutants emitted into the environment through industrial development. In this work, a new...
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StartPage 23
SubjectTerms Adsorbents
Adsorption
Adsorptivity
Cadmium
Chemistry
Chemistry and Materials Science
Chemistry/Food Science
Cobalt
Cobalt compounds
Cu-DPA
Economic development
Freundlich isotherm
Heavy metals
Industrial development
Lead
Metal industry
Purification
Real estate development
Real sample
Sewage
Trivalent chromium
Wastewater
Wastewater treatment
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Title Adsorptive removal of heavy metals from wastewater using Cobalt-diphenylamine (Co-DPA) complex
URI https://link.springer.com/article/10.1186/s13065-024-01128-z
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Volume 18
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