Surface energy of strained amorphous solids
Surface stress and surface energy are fundamental quantities which characterize the interface between two materials. Although these quantities are identical for interfaces involving only fluids, the Shuttleworth effect demonstrates that this is not the case for most interfaces involving solids, sinc...
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| Published in: | Nature communications Vol. 9; no. 1; pp. 982 - 6 |
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| Main Authors: | , , , , |
| Format: | Journal Article |
| Language: | English |
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07-03-2018
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| Abstract | Surface stress and surface energy are fundamental quantities which characterize the interface between two materials. Although these quantities are identical for interfaces involving only fluids, the Shuttleworth effect demonstrates that this is not the case for most interfaces involving solids, since their surface energies change with strain. Crystalline materials are known to have strain-dependent surface energies, but in amorphous materials, such as polymeric glasses and elastomers, the strain dependence is debated due to a dearth of direct measurements. Here, we utilize contact angle measurements on strained glassy and elastomeric solids to address this matter. We show conclusively that interfaces involving polymeric glasses exhibit strain-dependent surface energies, and give strong evidence for the absence of such a dependence for incompressible elastomers. The results provide fundamental insight into our understanding of the interfaces of amorphous solids and their interaction with contacting liquids.
Whether or not amorphous solids exhibit strain-dependent surface energies, like those of crystalline materials, is still a matter of debate. Here, Schulman et al. monitor the contact angle of droplets on strained polymeric glasses and elastomers, which directly probes energy variation at the interfaces. |
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| AbstractList | Surface stress and surface energy are fundamental quantities which characterize the interface between two materials. Although these quantities are identical for interfaces involving only fluids, the Shuttleworth effect demonstrates that this is not the case for most interfaces involving solids, since their surface energies change with strain. Crystalline materials are known to have strain-dependent surface energies, but in amorphous materials, such as polymeric glasses and elastomers, the strain dependence is debated due to a dearth of direct measurements. Here, we utilize contact angle measurements on strained glassy and elastomeric solids to address this matter. We show conclusively that interfaces involving polymeric glasses exhibit strain-dependent surface energies, and give strong evidence for the absence of such a dependence for incompressible elastomers. The results provide fundamental insight into our understanding of the interfaces of amorphous solids and their interaction with contacting liquids. Surface stress and surface energy are fundamental quantities which characterize the interface between two materials. Although these quantities are identical for interfaces involving only fluids, the Shuttleworth effect demonstrates that this is not the case for most interfaces involving solids, since their surface energies change with strain. Crystalline materials are known to have strain-dependent surface energies, but in amorphous materials, such as polymeric glasses and elastomers, the strain dependence is debated due to a dearth of direct measurements. Here, we utilize contact angle measurements on strained glassy and elastomeric solids to address this matter. We show conclusively that interfaces involving polymeric glasses exhibit strain-dependent surface energies, and give strong evidence for the absence of such a dependence for incompressible elastomers. The results provide fundamental insight into our understanding of the interfaces of amorphous solids and their interaction with contacting liquids. Whether or not amorphous solids exhibit strain-dependent surface energies, like those of crystalline materials, is still a matter of debate. Here, Schulman et al. monitor the contact angle of droplets on strained polymeric glasses and elastomers, which directly probes energy variation at the interfaces. Surface stress and surface energy are fundamental quantities which characterize the interface between two materials. Although these quantities are identical for interfaces involving only fluids, the Shuttleworth effect demonstrates that this is not the case for most interfaces involving solids, since their surface energies change with strain. Crystalline materials are known to have strain-dependent surface energies, but in amorphous materials, such as polymeric glasses and elastomers, the strain dependence is debated due to a dearth of direct measurements. Here, we utilize contact angle measurements on strained glassy and elas-tomeric solids to address this matter. We show conclusively that interfaces involving poly-meric glasses exhibit strain-dependent surface energies, and give strong evidence for the absence of such a dependence for incompressible elastomers. The results provide fundamental insight into our understanding of the interfaces of amorphous solids and their interaction with contacting liquids. Whether or not amorphous solids exhibit strain-dependent surface energies, like those of crystalline materials, is still a matter of debate. Here, Schulman et al. monitor the contact angle of droplets on strained polymeric glasses and elastomers, which directly probes energy variation at the interfaces. |
| ArticleNumber | 982 |
| Author | Trejo, Miguel Schulman, Rafael D. Raphaël, Elie Dalnoki-Veress, Kari Salez, Thomas |
| Author_xml | – sequence: 1 givenname: Rafael D. surname: Schulman fullname: Schulman, Rafael D. organization: Department of Physics and Astronomy, McMaster University – sequence: 2 givenname: Miguel surname: Trejo fullname: Trejo, Miguel organization: Laboratoire de Physico-Chimie Théorique, UMR CNRS Gulliver 7083, ESPCI Paris, PSL Research University – sequence: 3 givenname: Thomas orcidid: 0000-0001-6111-8721 surname: Salez fullname: Salez, Thomas organization: Univ. Bordeaux, CNRS, LOMA, UMR 5798, Global Station for Soft Matter, Global Institution for Collaborative Research and Education, Hokkaido University – sequence: 4 givenname: Elie orcidid: 0000-0003-0007-4790 surname: Raphaël fullname: Raphaël, Elie organization: Laboratoire de Physico-Chimie Théorique, UMR CNRS Gulliver 7083, ESPCI Paris, PSL Research University – sequence: 5 givenname: Kari orcidid: 0000-0002-0885-6634 surname: Dalnoki-Veress fullname: Dalnoki-Veress, Kari email: dalnoki@mcmaster.ca organization: Department of Physics and Astronomy, McMaster University, Laboratoire de Physico-Chimie Théorique, UMR CNRS Gulliver 7083, ESPCI Paris, PSL Research University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29515162$$D View this record in MEDLINE/PubMed https://hal.science/hal-01804460$$DView record in HAL |
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| Snippet | Surface stress and surface energy are fundamental quantities which characterize the interface between two materials. Although these quantities are identical... Whether or not amorphous solids exhibit strain-dependent surface energies, like those of crystalline materials, is still a matter of debate. Here, Schulman et... |
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| SubjectTerms | 132/122 639/301/119/544 639/301/923/1030 639/766/119/544 Amorphous materials Condensed Matter Contact angle Elastomers Fluid flow Humanities and Social Sciences Incompressible flow Interfaces Materials Science multidisciplinary Physics Science Science (multidisciplinary) Solids Surface energy Surface properties |
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| Title | Surface energy of strained amorphous solids |
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