Metal-organic framework template-guided electrochemical lithography on substrates for SERS sensing applications
The templating method holds great promise for fabricating surface nanopatterns. To enhance the manufacturing capabilities of complex surface nanopatterns, it is important to explore new modes of the templates beyond their conventional masking and molding modes. Here, we employed the metal-organic fr...
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| Published in: | Nature communications Vol. 14; no. 1; p. 5860 |
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| Main Authors: | , , , , , , , |
| Format: | Journal Article |
| Language: | English |
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20-09-2023
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| Abstract | The templating method holds great promise for fabricating surface nanopatterns. To enhance the manufacturing capabilities of complex surface nanopatterns, it is important to explore new modes of the templates beyond their conventional masking and molding modes. Here, we employed the metal-organic framework (MOF) microparticles assembled monolayer films as templates for metal electrodeposition and revealed a previously unidentified guiding growth mode enabling the precise growth of metallic films exclusively underneath the MOF microparticles. The guiding growth mode was induced by the fast ion transportation within the nanochannels of the MOF templates. The MOF template could be repeatedly used, allowing for the creation of identical metallic surface nanopatterns for multiple times on different substrates. The MOF template-guided electrochemical growth mode provided a robust route towards cost-effective fabrication of complex metallic surface nanopatterns with promising applications in metamaterials, plasmonics, and surface-enhanced Raman spectroscopy (SERS) sensing fields.
Templating method holds great promise for fabricating surface nanopatterns. Here authors present a guiding growth mode using metal-organic framework microparticles as templates during metal electrodeposition, where metals exclusively grow underneath the microparticles. |
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| AbstractList | The templating method holds great promise for fabricating surface nanopatterns. To enhance the manufacturing capabilities of complex surface nanopatterns, it is important to explore new modes of the templates beyond their conventional masking and molding modes. Here, we employed the metal-organic framework (MOF) microparticles assembled monolayer films as templates for metal electrodeposition and revealed a previously unidentified guiding growth mode enabling the precise growth of metallic films exclusively underneath the MOF microparticles. The guiding growth mode was induced by the fast ion transportation within the nanochannels of the MOF templates. The MOF template could be repeatedly used, allowing for the creation of identical metallic surface nanopatterns for multiple times on different substrates. The MOF template-guided electrochemical growth mode provided a robust route towards cost-effective fabrication of complex metallic surface nanopatterns with promising applications in metamaterials, plasmonics, and surface-enhanced Raman spectroscopy (SERS) sensing fields.
Templating method holds great promise for fabricating surface nanopatterns. Here authors present a guiding growth mode using metal-organic framework microparticles as templates during metal electrodeposition, where metals exclusively grow underneath the microparticles. The templating method holds great promise for fabricating surface nanopatterns. To enhance the manufacturing capabilities of complex surface nanopatterns, it is important to explore new modes of the templates beyond their conventional masking and molding modes. Here, we employed the metal-organic framework (MOF) microparticles assembled monolayer films as templates for metal electrodeposition and revealed a previously unidentified guiding growth mode enabling the precise growth of metallic films exclusively underneath the MOF microparticles. The guiding growth mode was induced by the fast ion transportation within the nanochannels of the MOF templates. The MOF template could be repeatedly used, allowing for the creation of identical metallic surface nanopatterns for multiple times on different substrates. The MOF template-guided electrochemical growth mode provided a robust route towards cost-effective fabrication of complex metallic surface nanopatterns with promising applications in metamaterials, plasmonics, and surface-enhanced Raman spectroscopy (SERS) sensing fields. The templating method holds great promise for fabricating surface nanopatterns. To enhance the manufacturing capabilities of complex surface nanopatterns, it is important to explore new modes of the templates beyond their conventional masking and molding modes. Here, we employed the metal-organic framework (MOF) microparticles assembled monolayer films as templates for metal electrodeposition and revealed a previously unidentified guiding growth mode enabling the precise growth of metallic films exclusively underneath the MOF microparticles. The guiding growth mode was induced by the fast ion transportation within the nanochannels of the MOF templates. The MOF template could be repeatedly used, allowing for the creation of identical metallic surface nanopatterns for multiple times on different substrates. The MOF template-guided electrochemical growth mode provided a robust route towards cost-effective fabrication of complex metallic surface nanopatterns with promising applications in metamaterials, plasmonics, and surface-enhanced Raman spectroscopy (SERS) sensing fields.Templating method holds great promise for fabricating surface nanopatterns. Here authors present a guiding growth mode using metal-organic framework microparticles as templates during metal electrodeposition, where metals exclusively grow underneath the microparticles. Abstract The templating method holds great promise for fabricating surface nanopatterns. To enhance the manufacturing capabilities of complex surface nanopatterns, it is important to explore new modes of the templates beyond their conventional masking and molding modes. Here, we employed the metal-organic framework (MOF) microparticles assembled monolayer films as templates for metal electrodeposition and revealed a previously unidentified guiding growth mode enabling the precise growth of metallic films exclusively underneath the MOF microparticles. The guiding growth mode was induced by the fast ion transportation within the nanochannels of the MOF templates. The MOF template could be repeatedly used, allowing for the creation of identical metallic surface nanopatterns for multiple times on different substrates. The MOF template-guided electrochemical growth mode provided a robust route towards cost-effective fabrication of complex metallic surface nanopatterns with promising applications in metamaterials, plasmonics, and surface-enhanced Raman spectroscopy (SERS) sensing fields. |
| ArticleNumber | 5860 |
| Author | Zhao, Liyan Zhang, Xiaochen Mochizuki, Kenji Zhang, Xuan Yan, Mi Yang, Shikuan Lu, Youyou Liu, Hong |
| Author_xml | – sequence: 1 givenname: Youyou orcidid: 0009-0006-5437-2733 surname: Lu fullname: Lu, Youyou organization: Department of Medical Oncology, The First Affiliated Hospital, Zhejiang University School of Medicine, School of Materials Science and Engineering, Zhejiang University – sequence: 2 givenname: Xuan orcidid: 0000-0002-9279-800X surname: Zhang fullname: Zhang, Xuan organization: Department of Chemistry, Zhejiang University – sequence: 3 givenname: Liyan surname: Zhao fullname: Zhao, Liyan organization: School of Materials Science and Engineering, Zhejiang University – sequence: 4 givenname: Hong surname: Liu fullname: Liu, Hong organization: School of Materials Science and Engineering, Zhejiang University – sequence: 5 givenname: Mi surname: Yan fullname: Yan, Mi organization: School of Materials Science and Engineering, Zhejiang University, Baotou Research Institute of Rare Earths – sequence: 6 givenname: Xiaochen surname: Zhang fullname: Zhang, Xiaochen organization: Department of Medical Oncology, The First Affiliated Hospital, Zhejiang University School of Medicine – sequence: 7 givenname: Kenji orcidid: 0000-0002-8947-9980 surname: Mochizuki fullname: Mochizuki, Kenji email: kenji_mochizuki@zju.edu.cn organization: Department of Chemistry, Zhejiang University – sequence: 8 givenname: Shikuan orcidid: 0000-0001-6662-3057 surname: Yang fullname: Yang, Shikuan email: shkyang@zju.edu.cn organization: Department of Medical Oncology, The First Affiliated Hospital, Zhejiang University School of Medicine, School of Materials Science and Engineering, Zhejiang University, Baotou Research Institute of Rare Earths, State Key Laboratory of Fluid Power and Mechatronic Systems, Zhejiang University |
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| Title | Metal-organic framework template-guided electrochemical lithography on substrates for SERS sensing applications |
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