Enhanced Aluminum-Ion Storage Properties of N-Doped Titanium Dioxide Electrode in Aqueous Aluminum-Ion Batteries

Aqueous aluminum-ion batteries (AIBs) have great potential as devices for future large-scale energy storage systems due to the cost efficiency, environmentally friendly nature, and impressive theoretical energy density of Al. However, currently, available materials used as anodes for aqueous AIBs ar...

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Published in:	Nanomaterials (Basel, Switzerland) Vol. 14; no. 5; p. 472
Main Authors:	Jian, Le, Wu, Xibing, Li, Ruichun, Zhao, Fangzheng, Liu, Peng, Wang, Feng, Liu, Daosheng, Yao, Qingrong, Deng, Jianqiu
Format:	Journal Article
Language:	English
Published:	Switzerland MDPI AG 05-03-2024 MDPI
Subjects:	Aluminum Aluminum-ion batteries Analysis anode Anodes aqueous aluminum-ion batteries Aqueous solutions Batteries Carbon Charge transfer Chemical synthesis Composite materials Crystal structure Discharge capacity Electric properties Electrochemistry Electrode materials Electrodes Electrolytes Electrons Energy storage Fourier transforms Investigations Ion storage Lithium Low resistance Mechanical properties Methods Microscopy Nanoparticles Nitrogen nitrogen-doping rate performance Sol-gel processes Spectrum analysis Storage systems Titanium Titanium dioxide United States > US Japan rate performance anode titanium dioxide aqueous aluminum-ion batteries nitrogen-doping
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Abstract	Aqueous aluminum-ion batteries (AIBs) have great potential as devices for future large-scale energy storage systems due to the cost efficiency, environmentally friendly nature, and impressive theoretical energy density of Al. However, currently, available materials used as anodes for aqueous AIBs are scarce. In this study, a novel sol-gel method was used to synthesize nitrogen-doped titanium dioxide (N-TiO ) as a potential anode material for AIBs in water. The annealed N-TiO showed a high discharge capacity of 43.2 mAh g at a current density of 3 A g . Analysis of the electrode kinetics revealed that the N-TiO anodes exhibited rapid diffusion of aluminum ions, low resistance to charge transfer, and high electronic conductivity, enabling good rate performance. The successful implementation of a nitrogen-doping strategy provides a promising approach to enhance the electrochemical characteristics of electrode materials for aqueous AIBs.
AbstractList	Aqueous aluminum-ion batteries (AIBs) have great potential as devices for future large-scale energy storage systems due to the cost efficiency, environmentally friendly nature, and impressive theoretical energy density of Al. However, currently, available materials used as anodes for aqueous AIBs are scarce. In this study, a novel sol-gel method was used to synthesize nitrogen-doped titanium dioxide (N-TiO2) as a potential anode material for AIBs in water. The annealed N-TiO2 showed a high discharge capacity of 43.2 mAh g-1 at a current density of 3 A g-1. Analysis of the electrode kinetics revealed that the N-TiO2 anodes exhibited rapid diffusion of aluminum ions, low resistance to charge transfer, and high electronic conductivity, enabling good rate performance. The successful implementation of a nitrogen-doping strategy provides a promising approach to enhance the electrochemical characteristics of electrode materials for aqueous AIBs. Aqueous aluminum-ion batteries (AIBs) have great potential as devices for future large-scale energy storage systems due to the cost efficiency, environmentally friendly nature, and impressive theoretical energy density of Al. However, currently, available materials used as anodes for aqueous AIBs are scarce. In this study, a novel sol-gel method was used to synthesize nitrogen-doped titanium dioxide (N-TiO[sub.2] ) as a potential anode material for AIBs in water. The annealed N-TiO[sub.2] showed a high discharge capacity of 43.2 mAh g[sup.−1] at a current density of 3 A g[sup.−1] . Analysis of the electrode kinetics revealed that the N-TiO[sub.2] anodes exhibited rapid diffusion of aluminum ions, low resistance to charge transfer, and high electronic conductivity, enabling good rate performance. The successful implementation of a nitrogen-doping strategy provides a promising approach to enhance the electrochemical characteristics of electrode materials for aqueous AIBs. Aqueous aluminum-ion batteries (AIBs) have great potential as devices for future large-scale energy storage systems due to the cost efficiency, environmentally friendly nature, and impressive theoretical energy density of Al. However, currently, available materials used as anodes for aqueous AIBs are scarce. In this study, a novel sol-gel method was used to synthesize nitrogen-doped titanium dioxide (N-TiO ) as a potential anode material for AIBs in water. The annealed N-TiO showed a high discharge capacity of 43.2 mAh g at a current density of 3 A g . Analysis of the electrode kinetics revealed that the N-TiO anodes exhibited rapid diffusion of aluminum ions, low resistance to charge transfer, and high electronic conductivity, enabling good rate performance. The successful implementation of a nitrogen-doping strategy provides a promising approach to enhance the electrochemical characteristics of electrode materials for aqueous AIBs. Aqueous aluminum-ion batteries (AIBs) have great potential as devices for future large-scale energy storage systems due to the cost efficiency, environmentally friendly nature, and impressive theoretical energy density of Al. However, currently, available materials used as anodes for aqueous AIBs are scarce. In this study, a novel sol-gel method was used to synthesize nitrogen-doped titanium dioxide (N-TiO2) as a potential anode material for AIBs in water. The annealed N-TiO2 showed a high discharge capacity of 43.2 mAh g−1 at a current density of 3 A g−1. Analysis of the electrode kinetics revealed that the N-TiO2 anodes exhibited rapid diffusion of aluminum ions, low resistance to charge transfer, and high electronic conductivity, enabling good rate performance. The successful implementation of a nitrogen-doping strategy provides a promising approach to enhance the electrochemical characteristics of electrode materials for aqueous AIBs. Aqueous aluminum-ion batteries (AIBs) have great potential as devices for future large-scale energy storage systems due to the cost efficiency, environmentally friendly nature, and impressive theoretical energy density of Al. However, currently, available materials used as anodes for aqueous AIBs are scarce. In this study, a novel sol-gel method was used to synthesize nitrogen-doped titanium dioxide (N-TiO 2 ) as a potential anode material for AIBs in water. The annealed N-TiO 2 showed a high discharge capacity of 43.2 mAh g −1 at a current density of 3 A g −1 . Analysis of the electrode kinetics revealed that the N-TiO 2 anodes exhibited rapid diffusion of aluminum ions, low resistance to charge transfer, and high electronic conductivity, enabling good rate performance. The successful implementation of a nitrogen-doping strategy provides a promising approach to enhance the electrochemical characteristics of electrode materials for aqueous AIBs.
Audience	Academic
Author	Deng, Jianqiu Liu, Daosheng Jian, Le Wu, Xibing Yao, Qingrong Liu, Peng Li, Ruichun Zhao, Fangzheng Wang, Feng
AuthorAffiliation	Guangxi Key Laboratory of Information Materials, School of Materials Science and Engineering, Guilin University of Electronic Technology, Guilin 541004, China; jl198717@163.com (L.J.); xibingwu2022@163.com (X.W.); l1534092882@163.com (R.L.); zfz513723@163.com (F.Z.); liupeng@guet.edu.cn (P.L.); wf@guet.edu.cn (F.W.); dawson@guet.edu.cn (D.L.); qingry96@guet.edu.cn (Q.Y.)
AuthorAffiliation_xml	– name: Guangxi Key Laboratory of Information Materials, School of Materials Science and Engineering, Guilin University of Electronic Technology, Guilin 541004, China; jl198717@163.com (L.J.); xibingwu2022@163.com (X.W.); l1534092882@163.com (R.L.); zfz513723@163.com (F.Z.); liupeng@guet.edu.cn (P.L.); wf@guet.edu.cn (F.W.); dawson@guet.edu.cn (D.L.); qingry96@guet.edu.cn (Q.Y.)
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SubjectTerms	Aluminum Aluminum-ion batteries Analysis anode Anodes aqueous aluminum-ion batteries Aqueous solutions Batteries Carbon Charge transfer Chemical synthesis Composite materials Crystal structure Discharge capacity Electric properties Electrochemistry Electrode materials Electrodes Electrolytes Electrons Energy storage Fourier transforms Investigations Ion storage Lithium Low resistance Mechanical properties Methods Microscopy Nanoparticles Nitrogen nitrogen-doping rate performance Sol-gel processes Spectrum analysis Storage systems Titanium Titanium dioxide
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Title	Enhanced Aluminum-Ion Storage Properties of N-Doped Titanium Dioxide Electrode in Aqueous Aluminum-Ion Batteries
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