Thermal stability of superhydrophobic, nanostructured surfaces
[Display omitted] . ► The thermal stability of superhydrophobic surfaces after thermal annealing. ► SiOx-contained carbon coatings show robust superhydrophobicity up to 350°C. ► Superhydrophobicity is stable on nanostructured surfaces with high aspect ratio. ► Surfaces become superhydrophilic for an...
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| Published in: | Journal of colloid and interface science Vol. 391; pp. 152 - 157 |
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| Main Authors: | , , , , , , , |
| Format: | Journal Article |
| Language: | English |
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01-02-2013
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| Abstract | [Display omitted] .
► The thermal stability of superhydrophobic surfaces after thermal annealing. ► SiOx-contained carbon coatings show robust superhydrophobicity up to 350°C. ► Superhydrophobicity is stable on nanostructured surfaces with high aspect ratio. ► Surfaces become superhydrophilic for annealing temperatures higher than 500°C.
The thermal stability of superhydrophobic, nanostructured surfaces after thermal annealing was explored. Flat surfaces coated with hydrophobic diamond-like carbon (DLC) via plasma polymerization of hexamethyldisiloxane (HMDSO) showed a gradual decrease in the water contact angle from 90o to 60o while nanostructured surfaces maintained superhydrophobicity with more than 150° for annealing temperatures between 25 and 300°C. It was also found that surfaces with nanostructures having an aspect ratio of more than 5.2 may maintain superhydrophobicity for annealing temperatures as high as 350°C; above this temperature, however, the hydrophobicity on surfaces with lower aspect ratio nanostructures gradually degraded. It was observed that regardless of the aspect ratios of the nanostructure, all superhydrophobic surfaces became superhydrophilic after annealing at temperatures higher than 500°C. |
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| AbstractList | The thermal stability of superhydrophobic, nanostructured surfaces after thermal annealing was explored. Flat surfaces coated with hydrophobic diamond-like carbon (DLC) via plasma polymerization of hexamethyldisiloxane (HMDSO) showed a gradual decrease in the water contact angle from 90o to 60o while nanostructured surfaces maintained superhydrophobicity with more than 150 degree for annealing temperatures between 25 and 300 degree C. It was also found that surfaces with nanostructures having an aspect ratio of more than 5.2 may maintain superhydrophobicity for annealing temperatures as high as 350 degree C; above this temperature, however, the hydrophobicity on surfaces with lower aspect ratio nanostructures gradually degraded. It was observed that regardless of the aspect ratios of the nanostructure, all superhydrophobic surfaces became superhydrophilic after annealing at temperatures higher than 500 degree C. The thermal stability of superhydrophobic, nanostructured surfaces after thermal annealing was explored. Flat surfaces coated with hydrophobic diamond-like carbon (DLC) via plasma polymerization of hexamethyldisiloxane (HMDSO) showed a gradual decrease in the water contact angle from 90ᵒ to 60ᵒ while nanostructured surfaces maintained superhydrophobicity with more than 150° for annealing temperatures between 25 and 300°C. It was also found that surfaces with nanostructures having an aspect ratio of more than 5.2 may maintain superhydrophobicity for annealing temperatures as high as 350°C; above this temperature, however, the hydrophobicity on surfaces with lower aspect ratio nanostructures gradually degraded. It was observed that regardless of the aspect ratios of the nanostructure, all superhydrophobic surfaces became superhydrophilic after annealing at temperatures higher than 500°C. [Display omitted] . ► The thermal stability of superhydrophobic surfaces after thermal annealing. ► SiOx-contained carbon coatings show robust superhydrophobicity up to 350°C. ► Superhydrophobicity is stable on nanostructured surfaces with high aspect ratio. ► Surfaces become superhydrophilic for annealing temperatures higher than 500°C. The thermal stability of superhydrophobic, nanostructured surfaces after thermal annealing was explored. Flat surfaces coated with hydrophobic diamond-like carbon (DLC) via plasma polymerization of hexamethyldisiloxane (HMDSO) showed a gradual decrease in the water contact angle from 90o to 60o while nanostructured surfaces maintained superhydrophobicity with more than 150° for annealing temperatures between 25 and 300°C. It was also found that surfaces with nanostructures having an aspect ratio of more than 5.2 may maintain superhydrophobicity for annealing temperatures as high as 350°C; above this temperature, however, the hydrophobicity on surfaces with lower aspect ratio nanostructures gradually degraded. It was observed that regardless of the aspect ratios of the nanostructure, all superhydrophobic surfaces became superhydrophilic after annealing at temperatures higher than 500°C. The thermal stability of superhydrophobic, nanostructured surfaces after thermal annealing was explored. Flat surfaces coated with hydrophobic diamond-like carbon (DLC) via plasma polymerization of hexamethyldisiloxane (HMDSO) showed a gradual decrease in the water contact angle from 90(o) to 60(o) while nanostructured surfaces maintained superhydrophobicity with more than 150° for annealing temperatures between 25 and 300°C. It was also found that surfaces with nanostructures having an aspect ratio of more than 5.2 may maintain superhydrophobicity for annealing temperatures as high as 350°C; above this temperature, however, the hydrophobicity on surfaces with lower aspect ratio nanostructures gradually degraded. It was observed that regardless of the aspect ratios of the nanostructure, all superhydrophobic surfaces became superhydrophilic after annealing at temperatures higher than 500°C. |
| Author | Kim, Seong Jin Ko, Tae-Jun Lee, Kwang-Ryeol Cha, Sung-Chul Roh, Hyunchul Her, Eun Kyu Oh, Kyu Hwan Moon, Myoung-Woon |
| Author_xml | – sequence: 1 givenname: Sung-Chul surname: Cha fullname: Cha, Sung-Chul organization: Advanced Functional Materials Research Team, Automotive, Corporate R&D Division, Hyundai Motor Group, Republic of Korea – sequence: 2 givenname: Eun Kyu surname: Her fullname: Her, Eun Kyu organization: Institute for Multidisciplinary Convergence of Matters, Korea Institute of Science and Technology, Seoul 136-791, Republic of Korea – sequence: 3 givenname: Tae-Jun surname: Ko fullname: Ko, Tae-Jun organization: Institute for Multidisciplinary Convergence of Matters, Korea Institute of Science and Technology, Seoul 136-791, Republic of Korea – sequence: 4 givenname: Seong Jin surname: Kim fullname: Kim, Seong Jin organization: Institute for Multidisciplinary Convergence of Matters, Korea Institute of Science and Technology, Seoul 136-791, Republic of Korea – sequence: 5 givenname: Hyunchul surname: Roh fullname: Roh, Hyunchul organization: Department of Materials Science and Engineering, Seoul National University, Seoul 151-742, Republic of Korea – sequence: 6 givenname: Kwang-Ryeol surname: Lee fullname: Lee, Kwang-Ryeol organization: Institute for Multidisciplinary Convergence of Matters, Korea Institute of Science and Technology, Seoul 136-791, Republic of Korea – sequence: 7 givenname: Kyu Hwan surname: Oh fullname: Oh, Kyu Hwan organization: Department of Materials Science and Engineering, Seoul National University, Seoul 151-742, Republic of Korea – sequence: 8 givenname: Myoung-Woon surname: Moon fullname: Moon, Myoung-Woon email: mwmoon@kist.re.kr organization: Institute for Multidisciplinary Convergence of Matters, Korea Institute of Science and Technology, Seoul 136-791, Republic of Korea |
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| Keywords | Nanostructure Superhydrophobicity Wetting transition Thermal stability Hydrophobicity Wetting |
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► The thermal stability of superhydrophobic surfaces after thermal annealing. ► SiOx-contained carbon coatings show robust... The thermal stability of superhydrophobic, nanostructured surfaces after thermal annealing was explored. Flat surfaces coated with hydrophobic diamond-like... |
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| SubjectTerms | Annealing Aspect ratio carbon Chemistry contact angle Diamond-like carbon films Exact sciences and technology General and physical chemistry Hydrophobicity Nanocomposites Nanomaterials Nanostructure polymerization Solid-liquid interface Superhydrophobicity Surface physical chemistry temperature Thermal stability Wetting transition |
| Title | Thermal stability of superhydrophobic, nanostructured surfaces |
| URI | https://dx.doi.org/10.1016/j.jcis.2012.09.052 https://www.ncbi.nlm.nih.gov/pubmed/23116849 https://search.proquest.com/docview/1283658644 |
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