A Survey of Strain‐Promoted Azide–Alkyne Cycloaddition in Polymer Chemistry
Highly efficient reactions that enable the assembly of molecules into complex structures have driven extensive progress in synthetic chemistry. In particular, reactions that occur under mild conditions and in benign solvents, while producing no by‐products and rapidly reach completion are attracting...
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| Published in: | Chemistry : a European journal Vol. 27; no. 16; pp. 5057 - 5073 |
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| Main Authors: | , , , |
| Format: | Journal Article |
| Language: | English |
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17-03-2021
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| Abstract | Highly efficient reactions that enable the assembly of molecules into complex structures have driven extensive progress in synthetic chemistry. In particular, reactions that occur under mild conditions and in benign solvents, while producing no by‐products and rapidly reach completion are attracting significant attention. Amongst these, the strain‐promoted azide–alkyne cycloaddition, involving various cyclooctyne derivatives reacting with azide‐bearing molecules, has gained extensive popularity in organic synthesis and bioorthogonal chemistry. This reaction has also recently gained momentum in polymer chemistry, where it has been used to decorate, link, crosslink, and even prepare polymer chains. This survey highlights key achievements in the use of this reaction to produce a variety of polymeric constructs for disparate applications.
Click here: This review highlights recent examples of the use of strain‐promoted azide–alkyne cycloaddition (SPAAC) chemistry in the preparation, decoration, and assembly of macromolecular structures. This highly efficient reaction has found numerous applications in polymer chemistry, allowing the preparation of various polymer architectures and the modification of end‐groups, side‐chains, and backbones of polymers. |
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| AbstractList | Highly efficient reactions that enable the assembly of molecules into complex structures have driven extensive progress in synthetic chemistry. In particular, reactions that occur under mild conditions and in benign solvents, while producing no by‐products and rapidly reach completion are attracting significant attention. Amongst these, the strain‐promoted azide–alkyne cycloaddition, involving various cyclooctyne derivatives reacting with azide‐bearing molecules, has gained extensive popularity in organic synthesis and bioorthogonal chemistry. This reaction has also recently gained momentum in polymer chemistry, where it has been used to decorate, link, crosslink, and even prepare polymer chains. This survey highlights key achievements in the use of this reaction to produce a variety of polymeric constructs for disparate applications. Abstract Highly efficient reactions that enable the assembly of molecules into complex structures have driven extensive progress in synthetic chemistry. In particular, reactions that occur under mild conditions and in benign solvents, while producing no by‐products and rapidly reach completion are attracting significant attention. Amongst these, the strain‐promoted azide–alkyne cycloaddition, involving various cyclooctyne derivatives reacting with azide‐bearing molecules, has gained extensive popularity in organic synthesis and bioorthogonal chemistry. This reaction has also recently gained momentum in polymer chemistry, where it has been used to decorate, link, crosslink, and even prepare polymer chains. This survey highlights key achievements in the use of this reaction to produce a variety of polymeric constructs for disparate applications. Highly efficient reactions that enable the assembly of molecules into complex structures have driven extensive progress in synthetic chemistry. In particular, reactions that occur under mild conditions and in benign solvents, while producing no by‐products and rapidly reach completion are attracting significant attention. Amongst these, the strain‐promoted azide–alkyne cycloaddition, involving various cyclooctyne derivatives reacting with azide‐bearing molecules, has gained extensive popularity in organic synthesis and bioorthogonal chemistry. This reaction has also recently gained momentum in polymer chemistry, where it has been used to decorate, link, crosslink, and even prepare polymer chains. This survey highlights key achievements in the use of this reaction to produce a variety of polymeric constructs for disparate applications. Click here: This review highlights recent examples of the use of strain‐promoted azide–alkyne cycloaddition (SPAAC) chemistry in the preparation, decoration, and assembly of macromolecular structures. This highly efficient reaction has found numerous applications in polymer chemistry, allowing the preparation of various polymer architectures and the modification of end‐groups, side‐chains, and backbones of polymers. |
| Author | Fong, Darryl Li, Kelvin Meichsner, Eric Adronov, Alex |
| Author_xml | – sequence: 1 givenname: Kelvin surname: Li fullname: Li, Kelvin organization: McMaster University – sequence: 2 givenname: Darryl orcidid: 0000-0002-0231-683X surname: Fong fullname: Fong, Darryl organization: McMaster University – sequence: 3 givenname: Eric orcidid: 0000-0002-9193-2078 surname: Meichsner fullname: Meichsner, Eric organization: McMaster University – sequence: 4 givenname: Alex orcidid: 0000-0002-0770-3118 surname: Adronov fullname: Adronov, Alex email: adronov@mcmaster.ca organization: McMaster University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/33017499$$D View this record in MEDLINE/PubMed |
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| Keywords | click chemistry cycloaddition strained molecules polymers azides alkynes |
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| Snippet | Highly efficient reactions that enable the assembly of molecules into complex structures have driven extensive progress in synthetic chemistry. In particular,... Abstract Highly efficient reactions that enable the assembly of molecules into complex structures have driven extensive progress in synthetic chemistry. In... |
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| SubjectTerms | Alkynes azides Chemical synthesis Chemistry click chemistry Cycloaddition Polls & surveys Polymer chemistry Polymers strained molecules |
| Title | A Survey of Strain‐Promoted Azide–Alkyne Cycloaddition in Polymer Chemistry |
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