Octacyanidotungstate(IV) Coordination Chains Demonstrate a Light‐Induced Excited Spin State Trapping Behavior and Magnetic Exchange Photoswitching
A huge increase in the magnetization of two coordination chains based on tetravalent octacyanidometalates (WIV and MoIV) is observed on irradiation with 436 nm light, while no such behavior is observed for the NbIV analogue. A photomagnetic response based solely on [WIV(CN)8]4− is demonstrated for t...
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| Published in: | Angewandte Chemie International Edition Vol. 56; no. 43; pp. 13283 - 13287 |
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| Format: | Journal Article |
| Language: | English |
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| Abstract | A huge increase in the magnetization of two coordination chains based on tetravalent octacyanidometalates (WIV and MoIV) is observed on irradiation with 436 nm light, while no such behavior is observed for the NbIV analogue. A photomagnetic response based solely on [WIV(CN)8]4− is demonstrated for the first time. The observed behavior is attributed to the light‐induced excited spin state trapping (LIESST) effect at the octacyanidometalate, and to the resulting magnetic exchange ON/OFF photoswitching between the MnII center and the photoinduced high‐spin (S=1) WIV or MoIV centers.
Let it shine! Octacyanidotungstate(IV) demonstrates a light‐induced excited spin state trapping photomagnetic effect that can be used to produce very strong magnetic exchange photoswitching functionality in various bimetallic coordination polymers. |
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| AbstractList | A huge increase in the magnetization of two coordination chains based on tetravalent octacyanidometalates (WIV and MoIV ) is observed on irradiation with 436 nm light, while no such behavior is observed for the NbIV analogue. A photomagnetic response based solely on [WIV (CN)8 ]4- is demonstrated for the first time. The observed behavior is attributed to the light-induced excited spin state trapping (LIESST) effect at the octacyanidometalate, and to the resulting magnetic exchange ON/OFF photoswitching between the MnII center and the photoinduced high-spin (S=1) WIV or MoIV centers. A huge increase in the magnetization of two coordination chains based on tetravalent octacyanidometalates (WIV and MoIV) is observed on irradiation with 436 nm light, while no such behavior is observed for the NbIV analogue. A photomagnetic response based solely on [WIV(CN)8]4− is demonstrated for the first time. The observed behavior is attributed to the light‐induced excited spin state trapping (LIESST) effect at the octacyanidometalate, and to the resulting magnetic exchange ON/OFF photoswitching between the MnII center and the photoinduced high‐spin (S=1) WIV or MoIV centers. Let it shine! Octacyanidotungstate(IV) demonstrates a light‐induced excited spin state trapping photomagnetic effect that can be used to produce very strong magnetic exchange photoswitching functionality in various bimetallic coordination polymers. A huge increase in the magnetization of two coordination chains based on tetravalent octacyanidometalates (W IV and Mo IV ) is observed on irradiation with 436 nm light, while no such behavior is observed for the Nb IV analogue. A photomagnetic response based solely on [W IV (CN) 8 ] 4− is demonstrated for the first time. The observed behavior is attributed to the light‐induced excited spin state trapping (LIESST) effect at the octacyanidometalate, and to the resulting magnetic exchange ON/OFF photoswitching between the Mn II center and the photoinduced high‐spin ( S =1) W IV or Mo IV centers. A huge increase in the magnetization of two coordination chains based on tetravalent octacyanidometalates (W and Mo ) is observed on irradiation with 436 nm light, while no such behavior is observed for the Nb analogue. A photomagnetic response based solely on [W (CN) ] is demonstrated for the first time. The observed behavior is attributed to the light-induced excited spin state trapping (LIESST) effect at the octacyanidometalate, and to the resulting magnetic exchange ON/OFF photoswitching between the Mn center and the photoinduced high-spin (S=1) W or Mo centers. A huge increase in the magnetization of two coordination chains based on tetravalent octacyanidometalates (WIV and MoIV) is observed on irradiation with 436nm light, while no such behavior is observed for the NbIV analogue. A photomagnetic response based solely on [WIV(CN)8]4- is demonstrated for the first time. The observed behavior is attributed to the light-induced excited spin state trapping (LIESST) effect at the octacyanidometalate, and to the resulting magnetic exchange ON/OFF photoswitching between the MnII center and the photoinduced high-spin (S=1) WIV or MoIV centers. |
| Author | Sieklucka, Barbara Magott, Michał Stefańczyk, Olaf Pinkowicz, Dawid |
| Author_xml | – sequence: 1 givenname: Michał surname: Magott fullname: Magott, Michał organization: Jagiellonian University – sequence: 2 givenname: Olaf surname: Stefańczyk fullname: Stefańczyk, Olaf organization: The University of Tokyo – sequence: 3 givenname: Barbara surname: Sieklucka fullname: Sieklucka, Barbara organization: Jagiellonian University – sequence: 4 givenname: Dawid orcidid: 0000-0002-9958-3116 surname: Pinkowicz fullname: Pinkowicz, Dawid email: dawid.pinkowicz@uj.edu.pl organization: Jagiellonian University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28770580$$D View this record in MEDLINE/PubMed |
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| Copyright | 2017 Wiley‐VCH Verlag GmbH & Co. KGaA, Weinheim 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim. 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim |
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| Keywords | octacyanidometalates LIESST molecular magnets photomagnetism photoswitching |
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| Snippet | A huge increase in the magnetization of two coordination chains based on tetravalent octacyanidometalates (WIV and MoIV) is observed on irradiation with 436 nm... A huge increase in the magnetization of two coordination chains based on tetravalent octacyanidometalates (W and Mo ) is observed on irradiation with 436 nm... A huge increase in the magnetization of two coordination chains based on tetravalent octacyanidometalates (W IV and Mo IV ) is observed on irradiation with 436... A huge increase in the magnetization of two coordination chains based on tetravalent octacyanidometalates (WIV and MoIV) is observed on irradiation with 436nm... A huge increase in the magnetization of two coordination chains based on tetravalent octacyanidometalates (WIV and MoIV ) is observed on irradiation with 436... |
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| SubjectTerms | Chains Irradiation LIESST molecular magnets octacyanidometalates photomagnetism photoswitching Radiation Trapping |
| Title | Octacyanidotungstate(IV) Coordination Chains Demonstrate a Light‐Induced Excited Spin State Trapping Behavior and Magnetic Exchange Photoswitching |
| URI | https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fanie.201703934 https://www.ncbi.nlm.nih.gov/pubmed/28770580 https://www.proquest.com/docview/1949486425 https://search.proquest.com/docview/1925889556 |
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