Metal–Organic Frameworks Encapsulating Active Nanoparticles as Emerging Composites for Catalysis: Recent Progress and Perspectives
Beyond conventional porous materials, metal–organic frameworks (MOFs) have aroused great interest in the construction of nanocatalysts with the characteristics of catalytically active nanoparticles (NPs) confined into the cavities/channels of MOFs or surrounded by MOFs. The advantages of adopting MO...
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| Published in: | Advanced materials (Weinheim) Vol. 30; no. 51; pp. e1800702 - n/a |
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| Main Authors: | , , , |
| Format: | Journal Article |
| Language: | English |
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Germany
Wiley Subscription Services, Inc
01-12-2018
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| Abstract | Beyond conventional porous materials, metal–organic frameworks (MOFs) have aroused great interest in the construction of nanocatalysts with the characteristics of catalytically active nanoparticles (NPs) confined into the cavities/channels of MOFs or surrounded by MOFs. The advantages of adopting MOFs as the encapsulating matrix are multifold: uniform and long‐range ordered cavities can effectively promote the mass transfer and diffusion of substrates and products, while the diverse metal nodes and tunable organic linkers may enable outstanding synergy functions with the encapsulated active NPs. Herein, some key issues related to MOFs for catalysis are discussed. Then, state‐of‐the art progress in the encapsulation of catalytically active NPs by MOFs as well as their synergy functions for enhanced catalytic performance in the fields of thermo‐, photo‐, and electrocatalysis are summarized. Notably, encapsulation‐structured nanocatalysts exhibit distinct advantages over conventional supported catalysts, especially in terms of the catalytic selectivity and stability. Finally, challenges and future developments in MOF‐based encapsulation‐structured nanocatalysts are proposed. The aim is to deliver better insight into the design of well‐defined nanocatalysts with atomically accurate structures and high performance in challenging reactions.
Compared with conventional supported catalysts, controllable encapsulation of catalytically active nanoparticles by porous metal–organic frameworks can exhibit intriguing features, such as uniform catalytic interface, strong interactions, the pore confinement effect, high stability, and outstanding designability, all of which contribute to the design and construction of high‐performance nanocatalysts. |
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| AbstractList | Beyond conventional porous materials, metal-organic frameworks (MOFs) have aroused great interest in the construction of nanocatalysts with the characteristics of catalytically active nanoparticles (NPs) confined into the cavities/channels of MOFs or surrounded by MOFs. The advantages of adopting MOFs as the encapsulating matrix are multifold: uniform and long-range ordered cavities can effectively promote the mass transfer and diffusion of substrates and products, while the diverse metal nodes and tunable organic linkers may enable outstanding synergy functions with the encapsulated active NPs. Herein, some key issues related to MOFs for catalysis are discussed. Then, state-of-the art progress in the encapsulation of catalytically active NPs by MOFs as well as their synergy functions for enhanced catalytic performance in the fields of thermo-, photo-, and electrocatalysis are summarized. Notably, encapsulation-structured nanocatalysts exhibit distinct advantages over conventional supported catalysts, especially in terms of the catalytic selectivity and stability. Finally, challenges and future developments in MOF-based encapsulation-structured nanocatalysts are proposed. The aim is to deliver better insight into the design of well-defined nanocatalysts with atomically accurate structures and high performance in challenging reactions. Abstract Beyond conventional porous materials, metal–organic frameworks (MOFs) have aroused great interest in the construction of nanocatalysts with the characteristics of catalytically active nanoparticles (NPs) confined into the cavities/channels of MOFs or surrounded by MOFs. The advantages of adopting MOFs as the encapsulating matrix are multifold: uniform and long‐range ordered cavities can effectively promote the mass transfer and diffusion of substrates and products, while the diverse metal nodes and tunable organic linkers may enable outstanding synergy functions with the encapsulated active NPs. Herein, some key issues related to MOFs for catalysis are discussed. Then, state‐of‐the art progress in the encapsulation of catalytically active NPs by MOFs as well as their synergy functions for enhanced catalytic performance in the fields of thermo‐, photo‐, and electrocatalysis are summarized. Notably, encapsulation‐structured nanocatalysts exhibit distinct advantages over conventional supported catalysts, especially in terms of the catalytic selectivity and stability. Finally, challenges and future developments in MOF‐based encapsulation‐structured nanocatalysts are proposed. The aim is to deliver better insight into the design of well‐defined nanocatalysts with atomically accurate structures and high performance in challenging reactions. Beyond conventional porous materials, metal–organic frameworks (MOFs) have aroused great interest in the construction of nanocatalysts with the characteristics of catalytically active nanoparticles (NPs) confined into the cavities/channels of MOFs or surrounded by MOFs. The advantages of adopting MOFs as the encapsulating matrix are multifold: uniform and long‐range ordered cavities can effectively promote the mass transfer and diffusion of substrates and products, while the diverse metal nodes and tunable organic linkers may enable outstanding synergy functions with the encapsulated active NPs. Herein, some key issues related to MOFs for catalysis are discussed. Then, state‐of‐the art progress in the encapsulation of catalytically active NPs by MOFs as well as their synergy functions for enhanced catalytic performance in the fields of thermo‐, photo‐, and electrocatalysis are summarized. Notably, encapsulation‐structured nanocatalysts exhibit distinct advantages over conventional supported catalysts, especially in terms of the catalytic selectivity and stability. Finally, challenges and future developments in MOF‐based encapsulation‐structured nanocatalysts are proposed. The aim is to deliver better insight into the design of well‐defined nanocatalysts with atomically accurate structures and high performance in challenging reactions. Compared with conventional supported catalysts, controllable encapsulation of catalytically active nanoparticles by porous metal–organic frameworks can exhibit intriguing features, such as uniform catalytic interface, strong interactions, the pore confinement effect, high stability, and outstanding designability, all of which contribute to the design and construction of high‐performance nanocatalysts. |
| Author | Tang, Zhiyong Zhang, Yin Li, Guodong Zhao, Shenlong |
| Author_xml | – sequence: 1 givenname: Guodong surname: Li fullname: Li, Guodong organization: National Center for Nanoscience and Technology – sequence: 2 givenname: Shenlong surname: Zhao fullname: Zhao, Shenlong organization: National Center for Nanoscience and Technology – sequence: 3 givenname: Yin surname: Zhang fullname: Zhang, Yin organization: Peking University – sequence: 4 givenname: Zhiyong orcidid: 0000-0003-0610-0064 surname: Tang fullname: Tang, Zhiyong email: zytang@nanoctr.cn organization: University of Chinese Academy of Sciences |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30247789$$D View this record in MEDLINE/PubMed |
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| Snippet | Beyond conventional porous materials, metal–organic frameworks (MOFs) have aroused great interest in the construction of nanocatalysts with the characteristics... Beyond conventional porous materials, metal-organic frameworks (MOFs) have aroused great interest in the construction of nanocatalysts with the characteristics... Abstract Beyond conventional porous materials, metal–organic frameworks (MOFs) have aroused great interest in the construction of nanocatalysts with the... |
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| SubjectTerms | Catalysis Encapsulation heterogeneous catalysis Holes Mass transfer Metal-organic frameworks nanocomposite nanoparticle Nanoparticles Porous materials Selectivity Substrates |
| Title | Metal–Organic Frameworks Encapsulating Active Nanoparticles as Emerging Composites for Catalysis: Recent Progress and Perspectives |
| URI | https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.201800702 https://www.ncbi.nlm.nih.gov/pubmed/30247789 https://www.proquest.com/docview/2157462653 https://search.proquest.com/docview/2111738780 |
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