Interplay between Reaction and Phase Behaviour in Carbon Dioxide Hydrogenation to Methanol

Condensation promotes CO2 hydrogenation to CH3OH beyond equilibrium through in situ product separation. Although primordial for catalyst and reactor design, triggering conditions as well as the impact on sub‐equilibrium reaction behaviour remain unclear. Herein we used an in‐house designed micro‐vie...

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Bibliographic Details
Published in:	ChemSusChem Vol. 10; no. 6; pp. 1166 - 1174
Main Authors:	Reymond, Helena, Amado‐Blanco, Victor, Lauper, Andreas, Rudolf von Rohr, Philipp
Format:	Journal Article
Language:	English
Published:	Germany Wiley Subscription Services, Inc 22-03-2017
Subjects:	Aluminum Oxide - chemistry Behavior Carbon dioxide Carbon Dioxide - chemistry Catalysis Catalysts Copper - chemistry heterogeneous catalysis high pressure Hydrogenation Methanol - chemistry Methyl alcohol Optimization raman spectroscopy Reaction kinetics Selectivity Transition Temperature Zinc - chemistry raman spectroscopy carbon dioxide heterogeneous catalysis hydrogenation high pressure
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