Two-Steps Method to Prepare Multilayer Sandwich Structure Carbon Fiber Composite with Thermal and Electrical Anisotropy and Electromagnetic Interference Shielding
Carbon fiber (CF) composites performance enhancement is a research hotspot at present. In this work, first, a sandwich structure composite, CF@(carbon nanotube/Fe O )/epoxy (CF@(CNT/Fe O )/EP), is prepared by the free arc dispersion-CFs surface spraying-rolling process method, herein, CFs in the mid...
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Published in: | Materials Vol. 16; no. 2; p. 680 |
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Abstract | Carbon fiber (CF) composites performance enhancement is a research hotspot at present. In this work, first, a sandwich structure composite, CF@(carbon nanotube/Fe
O
)/epoxy (CF@(CNT/Fe
O
)/EP), is prepared by the free arc dispersion-CFs surface spraying-rolling process method, herein, CFs in the middle layer and (CNT/Fe
O
)/EP as top and substrate layer. Then, CF@(CNT/Fe
O
)/EP (on both sides) and CFs (in the middle) are overlapped by structure design, forming a multilayer CF@(CNT/Fe
O
)/EP-CFs composite with a CFs core sheath. A small amount of CNT/Fe
O
is consumed, (CNT/Fe
O
)/EP and CFs core sheath realize thermal and electrical anisotropy and directional enhancement, and multilayer sandwich structure makes the electromagnetic interference (EMI) shielding performance better strengthened by multiple absorption-reflection/penetration-reabsorption. From CF-0 to CF-8, CNT/Fe
O
content only increases by 0.045 wt%, axial thermal conductivity (λ
) increases from 0.59 W/(m·K) to 1.1 W/(m·K), growth rate is 86%, radial thermal conductivity (λ
) only increases by 0.05 W/(m·K), the maximum λ
/λ
is 2.9, axial electrical conductivity (σ
) increases from 6.2 S/cm to 7.7 S/cm, growth rate is 24%, radial electrical conductivity (σ
) only increases by 0.7 × 10
S/cm, the total EMI shielding effectiveness (EMI SE
) increases by 196%, from 10.3 dB to 30.5 dB. This provides a new idea for enhancing CFs composite properties. |
---|---|
AbstractList | Carbon fiber (CF) composites performance enhancement is a research hotspot at present. In this work, first, a sandwich structure composite, CF@(carbon nanotube/Fe
O
)/epoxy (CF@(CNT/Fe
O
)/EP), is prepared by the free arc dispersion-CFs surface spraying-rolling process method, herein, CFs in the middle layer and (CNT/Fe
O
)/EP as top and substrate layer. Then, CF@(CNT/Fe
O
)/EP (on both sides) and CFs (in the middle) are overlapped by structure design, forming a multilayer CF@(CNT/Fe
O
)/EP-CFs composite with a CFs core sheath. A small amount of CNT/Fe
O
is consumed, (CNT/Fe
O
)/EP and CFs core sheath realize thermal and electrical anisotropy and directional enhancement, and multilayer sandwich structure makes the electromagnetic interference (EMI) shielding performance better strengthened by multiple absorption-reflection/penetration-reabsorption. From CF-0 to CF-8, CNT/Fe
O
content only increases by 0.045 wt%, axial thermal conductivity (λ
) increases from 0.59 W/(m·K) to 1.1 W/(m·K), growth rate is 86%, radial thermal conductivity (λ
) only increases by 0.05 W/(m·K), the maximum λ
/λ
is 2.9, axial electrical conductivity (σ
) increases from 6.2 S/cm to 7.7 S/cm, growth rate is 24%, radial electrical conductivity (σ
) only increases by 0.7 × 10
S/cm, the total EMI shielding effectiveness (EMI SE
) increases by 196%, from 10.3 dB to 30.5 dB. This provides a new idea for enhancing CFs composite properties. Carbon fiber (CF) composites performance enhancement is a research hotspot at present. In this work, first, a sandwich structure composite, CF@(carbon nanotube/Fe3O4)/epoxy (CF@(CNT/Fe3O4)/EP), is prepared by the free arc dispersion-CFs surface spraying-rolling process method, herein, CFs in the middle layer and (CNT/Fe3O4)/EP as top and substrate layer. Then, CF@(CNT/Fe3O4)/EP (on both sides) and CFs (in the middle) are overlapped by structure design, forming a multilayer CF@(CNT/Fe3O4)/EP-CFs composite with a CFs core sheath. A small amount of CNT/Fe3O4 is consumed, (CNT/Fe3O4)/EP and CFs core sheath realize thermal and electrical anisotropy and directional enhancement, and multilayer sandwich structure makes the electromagnetic interference (EMI) shielding performance better strengthened by multiple absorption–reflection/penetration–reabsorption. From CF-0 to CF-8, CNT/Fe3O4 content only increases by 0.045 wt%, axial thermal conductivity (λ‖) increases from 0.59 W/(m·K) to 1.1 W/(m·K), growth rate is 86%, radial thermal conductivity (λ⊥) only increases by 0.05 W/(m·K), the maximum λ‖/λ⊥ is 2.9, axial electrical conductivity (σ‖) increases from 6.2 S/cm to 7.7 S/cm, growth rate is 24%, radial electrical conductivity (σ⊥) only increases by 0.7 × 10−4 S/cm, the total EMI shielding effectiveness (EMI SET) increases by 196%, from 10.3 dB to 30.5 dB. This provides a new idea for enhancing CFs composite properties. Carbon fiber (CF) composites performance enhancement is a research hotspot at present. In this work, first, a sandwich structure composite, CF@(carbon nanotube/Fe 3 O 4 )/epoxy (CF@(CNT/Fe 3 O 4 )/EP), is prepared by the free arc dispersion-CFs surface spraying-rolling process method, herein, CFs in the middle layer and (CNT/Fe 3 O 4 )/EP as top and substrate layer. Then, CF@(CNT/Fe 3 O 4 )/EP (on both sides) and CFs (in the middle) are overlapped by structure design, forming a multilayer CF@(CNT/Fe 3 O 4 )/EP-CFs composite with a CFs core sheath. A small amount of CNT/Fe 3 O 4 is consumed, (CNT/Fe 3 O 4 )/EP and CFs core sheath realize thermal and electrical anisotropy and directional enhancement, and multilayer sandwich structure makes the electromagnetic interference (EMI) shielding performance better strengthened by multiple absorption–reflection/penetration–reabsorption. From CF-0 to CF-8, CNT/Fe 3 O 4 content only increases by 0.045 wt%, axial thermal conductivity (λ ‖ ) increases from 0.59 W/(m·K) to 1.1 W/(m·K), growth rate is 86%, radial thermal conductivity (λ ⊥ ) only increases by 0.05 W/(m·K), the maximum λ ‖ /λ ⊥ is 2.9, axial electrical conductivity (σ ‖ ) increases from 6.2 S/cm to 7.7 S/cm, growth rate is 24%, radial electrical conductivity (σ ⊥ ) only increases by 0.7 × 10 −4 S/cm, the total EMI shielding effectiveness (EMI SE T ) increases by 196%, from 10.3 dB to 30.5 dB. This provides a new idea for enhancing CFs composite properties. |
Author | Zhang, Chuanqi He, Yan Shi, Song Wang, Huanhuan Zhang, Da Bi, Lansen Li, Wei |
AuthorAffiliation | 1 College of Electromechanical Engineering, Qingdao University of Science and Technology, Qingdao 266061, China 2 Shandong Laboratory for Preparation and Application of High-Performance Carbon Materials, Qingdao 266061, China 3 Shandong Collaborative Innovation Center of Intelligent Green Manufacturing Technology and Equipment, Qingdao 266061, China 4 Department of Energy Engineering, Zhejiang University, Hangzhou 310027, China |
AuthorAffiliation_xml | – name: 3 Shandong Collaborative Innovation Center of Intelligent Green Manufacturing Technology and Equipment, Qingdao 266061, China – name: 1 College of Electromechanical Engineering, Qingdao University of Science and Technology, Qingdao 266061, China – name: 4 Department of Energy Engineering, Zhejiang University, Hangzhou 310027, China – name: 2 Shandong Laboratory for Preparation and Application of High-Performance Carbon Materials, Qingdao 266061, China |
Author_xml | – sequence: 1 givenname: Chuanqi surname: Zhang fullname: Zhang, Chuanqi organization: College of Electromechanical Engineering, Qingdao University of Science and Technology, Qingdao 266061, China – sequence: 2 givenname: Lansen surname: Bi fullname: Bi, Lansen organization: College of Electromechanical Engineering, Qingdao University of Science and Technology, Qingdao 266061, China – sequence: 3 givenname: Song surname: Shi fullname: Shi, Song organization: College of Electromechanical Engineering, Qingdao University of Science and Technology, Qingdao 266061, China – sequence: 4 givenname: Huanhuan surname: Wang fullname: Wang, Huanhuan organization: College of Electromechanical Engineering, Qingdao University of Science and Technology, Qingdao 266061, China – sequence: 5 givenname: Da surname: Zhang fullname: Zhang, Da organization: College of Electromechanical Engineering, Qingdao University of Science and Technology, Qingdao 266061, China – sequence: 6 givenname: Yan surname: He fullname: He, Yan organization: Shandong Collaborative Innovation Center of Intelligent Green Manufacturing Technology and Equipment, Qingdao 266061, China – sequence: 7 givenname: Wei surname: Li fullname: Li, Wei organization: Department of Energy Engineering, Zhejiang University, Hangzhou 310027, China |
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SubjectTerms | Anisotropy Arc spraying Carbon fibers Carbon nanotubes Curing Dielectric properties Electrical resistivity Electromagnetic interference Electromagnetic shielding Epoxy resins Fiber composites Heat conductivity Heat transfer Iron oxides Morphology Multilayers Nanomaterials Performance enhancement plasma spraying Sandwich structures Scanning electron microscopy Sheaths structural composites Substrates Thermal conductivity |
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Title | Two-Steps Method to Prepare Multilayer Sandwich Structure Carbon Fiber Composite with Thermal and Electrical Anisotropy and Electromagnetic Interference Shielding |
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