Determination of Rational Conditions of Preliminary Ozonation of Nonionic Polyethoxylated Surfactants before Biosorption
The influence of preliminary oxidation of nonionic surfactants solutions on the biosorption efficiency of activated carbon was investigated. The Gibbs free energy of adsorption (−ΔG o a ) of oxidation products from water on an activated carbon was used as a parameter of the bacterial resistance of o...
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| Published in: | Ozone: science & engineering Vol. 28; no. 5; pp. 295 - 302 |
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| Main Authors: | , , , |
| Format: | Journal Article |
| Language: | English |
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Philadelphia, PA
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01-10-2006
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| Abstract | The influence of preliminary oxidation of nonionic surfactants solutions on the biosorption efficiency of activated carbon was investigated. The Gibbs free energy of adsorption (−ΔG
o
a
) of oxidation products from water on an activated carbon was used as a parameter of the bacterial resistance of oxidation products adsorption. It was established for nonionic surfactants, that ozonation essentially raised the contents of nonionic surfactant homologues with a low degree of ethoxylation. It leads to the increase in the Gibbs free energy of oxidation products adsorption and to inhibition of biodegradation process.
It was shown that the efficiency of biosorption process after preliminary ozonation was 2-3 times lower than without preliminary treatment that correlated with changes of the free energy of adsorption. |
|---|---|
| AbstractList | Rational conditions of preliminary ozonation on nonionic polyethoxylated surfactants before biosorption were determined. The Gibbs free energy of adsorption of oxidation products from water on an activated carbon was used as a parameter of the bacterial resistance of oxidation products adsorption. It was established for nonionic surfactants, that ozonation essentially raised the contents of nonionic surfactant homologous with a low degree of ethoxylation. It led to the increase in the Gibbs free energy of oxidation products adsorption and to inhibition of biodegradation process. It was showed that the efficiency of biosorption process after preliminary ozonation was 2-3 times lower than without preliminary treatment that correlated with changes of the free energy of adsorption. The influence of preliminary oxidation of nonionic surfactants solutions on the biosorption efficiency of activated carbon was investigated. The Gibbs free energy of adsorption (−ΔG o a ) of oxidation products from water on an activated carbon was used as a parameter of the bacterial resistance of oxidation products adsorption. It was established for nonionic surfactants, that ozonation essentially raised the contents of nonionic surfactant homologues with a low degree of ethoxylation. It leads to the increase in the Gibbs free energy of oxidation products adsorption and to inhibition of biodegradation process. It was shown that the efficiency of biosorption process after preliminary ozonation was 2-3 times lower than without preliminary treatment that correlated with changes of the free energy of adsorption. The influence of preliminary oxidation of nonionic surfactants solutions on the biosorption efficiency of activated carbon was investigated. The Gibbs free energy of adsorption (- Delta Goa) of oxidation products from water on an activated carbon was used as a parameter of the bacterial resistance of oxidation products adsorption. It was established for nonionic surfactants, that ozonation essentially raised the contents of nonionic surfactant homologues with a low degree of ethoxylation. It leads to the increase in the Gibbs free energy of oxidation products adsorption and to inhibition of biodegradation process. It was shown that the efficiency of biosorption process after preliminary ozonation was 2-3 times lower than without preliminary treatment that correlated with changes of the free energy of adsorption. The influence of preliminary oxidation of nonionic surfactants solutions on the biosorption efficiency of activated carbon was investigated. The Gibbs free energy of adsorption (-DeltaGoa) of oxidation products from water on an activated carbon was used as a parameter of the bacterial resistance of oxidation products adsorption. It was established for nonionic surfactants, that ozonation essentially raised the contents of nonionic surfactant homologues with a low degree of ethoxylation. It leads to the increase in the Gibbs free energy of oxidation products adsorption and to inhibition of biodegradation process. It was shown that the efficiency of biosorption process after preliminary ozonation was 2-3 times lower than without preliminary treatment that correlated with changes of the free energy of adsorption. |
| Author | Klimenko, N. A. Nevynna, L. V. Sydorenko Yu, V. Synelnikova, A. V. |
| Author_xml | – sequence: 1 givenname: N. A. surname: Klimenko fullname: Klimenko, N. A. email: klimenko@carrier.kiev.ua organization: Institute of Colloid and Water Chemistry of the National Academy of Sciences of Ukraine – sequence: 2 givenname: L. V. surname: Nevynna fullname: Nevynna, L. V. organization: Institute of Colloid and Water Chemistry of the National Academy of Sciences of Ukraine – sequence: 3 givenname: V. surname: Sydorenko Yu fullname: Sydorenko Yu, V. organization: Institute of Colloid and Water Chemistry of the National Academy of Sciences of Ukraine – sequence: 4 givenname: A. V. surname: Synelnikova fullname: Synelnikova, A. V. organization: Institute of Colloid and Water Chemistry of the National Academy of Sciences of Ukraine |
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| Cites_doi | 10.1080/01919510208901626 10.1016/S0043-1354(00)00149-4 10.1080/01919510390481676 10.1016/S0043-1354(02)00278-6 10.1021/ie990721a 10.1080/01919519908547261 10.1016/S0043-1354(97)00130-9 10.1002/j.1551-8833.1995.tb06304.x 10.1016/S0043-1354(00)00489-9 10.1016/0043-1354(94)90200-3 10.1021/es981228d 10.2166/wst.1998.0249 10.1080/01919510208901632 10.1080/01919512.1993.10555731 |
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| Keywords | Biodegradation Ozonization Gibbs free energy Biosorption Nonionic Surfactants Adsorption Non ionic surfactant Activated carbon Ozone Oxidation Gibbs Energy Surfactant |
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| References | CIT0021 Koganovskii A.M. (CIT0015) 1990 CIT0020 CIT0001 Bursova S.N. (CIT0003) 1990; 7 CIT0011 Wricke B. (CIT0022) 1996 Gonzalez P. (CIT0008) 2003; 38 Kofanov V.I. (CIT0014) 1986; 8 CIT0002 CIT0013 CIT0005 CIT0016 CIT0004 CIT0018 CIT0006 Goncharuk V.V. (CIT0007) 2003; 25 CIT0017 CIT0009 CIT0019 |
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| Snippet | The influence of preliminary oxidation of nonionic surfactants solutions on the biosorption efficiency of activated carbon was investigated. The Gibbs free... Rational conditions of preliminary ozonation on nonionic polyethoxylated surfactants before biosorption were determined. The Gibbs free energy of adsorption of... |
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| SubjectTerms | Activated Carbon Applied sciences Biosorption Exact sciences and technology Gibbs Energy Nonionic Surfactants Ozone Pollution |
| Title | Determination of Rational Conditions of Preliminary Ozonation of Nonionic Polyethoxylated Surfactants before Biosorption |
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