Ultralong spin coherence time in isotopically engineered diamond
As quantum mechanics ventures into the world of applications and engineering, materials science faces the necessity to design matter to quantum grade purity. For such materials, quantum effects define their physical behaviour and open completely new (quantum) perspectives for applications. Carbon-ba...
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| Published in: | Nature materials Vol. 8; no. 5; pp. 383 - 387 |
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| Main Authors: | , , , , , , , , , , , , , |
| Format: | Journal Article |
| Language: | English |
| Published: |
London
Nature Publishing Group UK
01-05-2009
Nature Publishing Group |
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| Online Access: | Get full text |
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| Abstract | As quantum mechanics ventures into the world of applications and engineering, materials science faces the necessity to design matter to quantum grade purity. For such materials, quantum effects define their physical behaviour and open completely new (quantum) perspectives for applications. Carbon-based materials are particularly good examples, highlighted by the fascinating quantum properties of, for example, nanotubes or graphene. Here, we demonstrate the synthesis and application of ultrapure isotopically controlled single-crystal chemical vapour deposition (CVD) diamond with a remarkably low concentration of paramagnetic impurities. The content of nuclear spins associated with the 13C isotope was depleted to 0.3% and the concentration of other paramagnetic defects was measured to be <1013 cm−3. Being placed in such a spin-free lattice, single electron spins show the longest room-temperature spin dephasing times ever observed in solid-state systems (T2=1.8 ms). This benchmark will potentially allow observation of coherent coupling between spins separated by a few tens of nanometres, making it a versatile material for room-temperature quantum information processing devices. We also show that single electron spins in the same isotopically engineered CVD diamond can be used to detect external magnetic fields with a sensitivity reaching 4 nT Hz−1/2 and subnanometre spatial resolution. |
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| AbstractList | As quantum mechanics ventures into the world of applications and engineering, materials science faces the necessity to design matter to quantum grade purity. For such materials, quantum effects define their physical behaviour and open completely new (quantum) perspectives for applications. Carbon-based materials are particularly good examples, highlighted by the fascinating quantum properties of, for example, nanotubes or graphene. Here, we demonstrate the synthesis and application of ultrapure isotopically controlled single-crystal chemical vapour deposition (CVD) diamond with a remarkably low concentration of paramagnetic impurities. The content of nuclear spins associated with the 13C isotope was depleted to 0.3% and the concentration of other paramagnetic defects was measured to be <1013 cm−3. Being placed in such a spin-free lattice, single electron spins show the longest room-temperature spin dephasing times ever observed in solid-state systems (T2=1.8 ms). This benchmark will potentially allow observation of coherent coupling between spins separated by a few tens of nanometres, making it a versatile material for room-temperature quantum information processing devices. We also show that single electron spins in the same isotopically engineered CVD diamond can be used to detect external magnetic fields with a sensitivity reaching 4 nT Hz−1/2 and subnanometre spatial resolution. As quantum mechanics ventures into the world of applications and engineering, materials science faces the necessity to design matter to quantum grade purity. For such materials, quantum effects define their physical behaviour and open completely new (quantum) perspectives for applications. Carbon-based materials are particularly good examples, highlighted by the fascinating quantum properties of, for example, nanotubes or graphene. Here, we demonstrate the synthesis and application of ultrapure isotopically controlled single-crystal chemical vapour deposition (CVD) diamond with a remarkably low concentration of paramagnetic impurities. The content of nuclear spins associated with the (13)C isotope was depleted to 0.3% and the concentration of other paramagnetic defects was measured to be <10(13) cm(-3). Being placed in such a spin-free lattice, single electron spins show the longest room-temperature spin dephasing times ever observed in solid-state systems (T2=1.8 ms). This benchmark will potentially allow observation of coherent coupling between spins separated by a few tens of nanometres, making it a versatile material for room-temperature quantum information processing devices. We also show that single electron spins in the same isotopically engineered CVD diamond can be used to detect external magnetic fields with a sensitivity reaching 4 nT Hz(-1/2) and subnanometre spatial resolution. The synthesis of highly pure diamond nanocrystals with a very small amount of paramagnetic impurities allows the observation of electron spin-dephasing times of up to 1.8 ms, a record for solid-state materials. The result could have important implications for quantum information processing methods based on diamond. As quantum mechanics ventures into the world of applications and engineering, materials science faces the necessity to design matter to quantum grade purity. For such materials, quantum effects define their physical behaviour and open completely new (quantum) perspectives for applications. Carbon-based materials are particularly good examples, highlighted by the fascinating quantum properties of, for example, nanotubes 1 or graphene 2 . Here, we demonstrate the synthesis and application of ultrapure isotopically controlled single-crystal chemical vapour deposition (CVD) diamond with a remarkably low concentration of paramagnetic impurities. The content of nuclear spins associated with the 13 C isotope was depleted to 0.3% and the concentration of other paramagnetic defects was measured to be <10 13 cm −3 . Being placed in such a spin-free lattice, single electron spins show the longest room-temperature spin dephasing times ever observed in solid-state systems ( T 2 =1.8 ms). This benchmark will potentially allow observation of coherent coupling between spins separated by a few tens of nanometres, making it a versatile material for room-temperature quantum information processing devices. We also show that single electron spins in the same isotopically engineered CVD diamond can be used to detect external magnetic fields with a sensitivity reaching 4 nT Hz −1/2 and subnanometre spatial resolution. As quantum mechanics ventures into the world of applications and engineering, materials science faces the necessity to design matter to quantum grade purity. For such materials, quantum effects define their physical behaviour and open completely new (quantum) perspectives for applications. Carbon-based materials are particularly good examples, highlighted by the fascinating quantum properties of, for example, nanotubes or graphene. Here, we demonstrate the synthesis and application of ultrapure isotopically controlled single-crystal chemical vapour deposition (CVD) diamond with a remarkably low concentration of paramagnetic impurities. The content of nuclear spins associated with the (13)C isotope was depleted to 0.3% and the concentration of other paramagnetic defects was measured to be <10(13) cm(-3). Being placed in such a spin-free lattice, single electron spins show the longest room-temperature spin dephasing times ever observed in solid-state systems (T2=1.8 ms). This benchmark will potentially allow observation of coherent coupling between spins separated by a few tens of nanometres, making it a versatile material for room-temperature quantum information processing devices. We also show that single electron spins in the same isotopically engineered CVD diamond can be used to detect external magnetic fields with a sensitivity reaching 4 nT Hz(-1/2) and subnanometre spatial resolution. [PUBLICATION ABSTRACT] |
| Author | Markham, Matthew Kolesov, Roman Jelezko, Fedor Tissler, Julia Balasubramanian, Gopalakrishnan Beck, Johannes Jacques, Vincent Mizuochi, Norikazu Wrachtrup, Jörg Neumann, Philipp Twitchen, Daniel Hemmer, Philip R Isoya, Junichi Achard, Jocelyn |
| Author_xml | – sequence: 1 givenname: Fedor surname: Jelezko fullname: Jelezko, Fedor organization: 3 Physikalisches Institut, Universität Stuttgart – sequence: 2 givenname: Jörg surname: Wrachtrup fullname: Wrachtrup, Jörg organization: 3 Physikalisches Institut, Universität Stuttgart – sequence: 3 givenname: Gopalakrishnan surname: Balasubramanian fullname: Balasubramanian, Gopalakrishnan organization: 3 Physikalisches Institut, Universität Stuttgart – sequence: 4 givenname: Philipp surname: Neumann fullname: Neumann, Philipp organization: 3 Physikalisches Institut, Universität Stuttgart – sequence: 5 givenname: Daniel surname: Twitchen fullname: Twitchen, Daniel organization: Element Six Ltd – sequence: 6 givenname: Matthew surname: Markham fullname: Markham, Matthew organization: Element Six Ltd – sequence: 7 givenname: Roman surname: Kolesov fullname: Kolesov, Roman organization: 3 Physikalisches Institut, Universität Stuttgart – sequence: 8 givenname: Norikazu surname: Mizuochi fullname: Mizuochi, Norikazu organization: 3 Physikalisches Institut, Universität Stuttgart Graduate School of Library, Information and Media Studies, University of Tsukuba – sequence: 9 givenname: Junichi surname: Isoya fullname: Isoya, Junichi organization: Graduate School of Library, Information and Media Studies, University of Tsukuba – sequence: 10 givenname: Jocelyn surname: Achard fullname: Achard, Jocelyn organization: LIMHP/CNRS, Université Paris 13 – sequence: 11 givenname: Johannes surname: Beck fullname: Beck, Johannes organization: 3 Physikalisches Institut, Universität Stuttgart – sequence: 12 givenname: Julia surname: Tissler fullname: Tissler, Julia organization: 3 Physikalisches Institut, Universität Stuttgart – sequence: 13 givenname: Vincent surname: Jacques fullname: Jacques, Vincent organization: 3 Physikalisches Institut, Universität Stuttgart – sequence: 14 givenname: Philip R surname: Hemmer fullname: Hemmer, Philip R organization: Texas A&M University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/19349970$$D View this record in MEDLINE/PubMed https://hal.science/hal-03575915$$DView record in HAL |
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| Snippet | As quantum mechanics ventures into the world of applications and engineering, materials science faces the necessity to design matter to quantum grade purity.... The synthesis of highly pure diamond nanocrystals with a very small amount of paramagnetic impurities allows the observation of electron spin-dephasing times... |
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| SubjectTerms | Biomaterials Carbon Isotopes Chemical engineering Chemical Engineering - methods Chemistry and Materials Science Condensed Matter Physics Diamond - chemistry Diamonds Engineering Sciences Isotopes letter Magnetic fields Materials Science Nanotechnology Nitrogen - chemistry Optical and Electronic Materials Physics Quantum Theory |
| Title | Ultralong spin coherence time in isotopically engineered diamond |
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