Adsorption of polar, nonpolar, and substituted aromatics to colloidal graphene oxide nanoparticles

We conducted batch adsorption experiments to understand the adsorptive properties of colloidal graphene oxide nanoparticles (GONPs) for a range of environmentally relevant aromatics and substituted aromatics, including model nonpolar compounds (pyrene, phenanthrene, naphthalene, and 1,3-dichlorobenz...

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Published in:	Environmental pollution (1987) Vol. 186; pp. 226 - 233
Main Authors:	Wang, Fang, Haftka, Joris J.-H., Sinnige, Theo L., Hermens, Joop L.M., Chen, Wei
Format:	Journal Article
Language:	English
Published:	Kidlington Elsevier Ltd 01-03-2014 Elsevier
Subjects:	Adsorption Affinity Applied sciences Aromatic compounds Aromatics Buckminsterfullerene Chlorobenzenes Chlorophenols Exact sciences and technology Fullerenes Global environmental pollution Graphene Graphene oxide nanoparticles Graphite - chemistry Nanoparticles - chemistry Nanotubes, Carbon - chemistry Oxides Polar compounds Pollution Polycyclic Aromatic Hydrocarbons - chemistry Surface chemistry Aromatics Adsorption Polar compounds Graphene oxide nanoparticles Carbonaceous materials Nanoparticle Adsorption capacity Polar compound Pollution Decontamination Model compound Environment Aromatic compound Graphene oxide Nanostructured materials Apolar compound Nanotechnology Organic compounds
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Abstract	We conducted batch adsorption experiments to understand the adsorptive properties of colloidal graphene oxide nanoparticles (GONPs) for a range of environmentally relevant aromatics and substituted aromatics, including model nonpolar compounds (pyrene, phenanthrene, naphthalene, and 1,3-dichlorobenzene) and model polar compounds (1-naphthol, 1-naphthylamine, 2,4-dichlorophenol, and 2,4-dinitrotoluene). GONPs exhibited strong adsorption affinities for all the test compounds, with distribution coefficients on the order of 103–106 L/kg. Adsorption to GONPs is much more linear than to carbon nanotubes (CNTs) and C60, likely because GO nanoflakes are essentially individually dispersed (rendering adsorption sites of similar adsorption energy) whereas CNT/C60 are prone to bundling/aggregation. For a given compound GONPs and CNTs often exhibit different adsorption affinities, which is attributable to the differences in both the morphology and surface chemistry between the two nanomaterials. Particularly, the high surface O-content of GONPs enables strong H-bonding and Lewis acid–base interactions with hydroxyl- and amino-substituted aromatics. •Graphene oxide nanoparticles (GONPs) exhibit strong adsorption for aromatics.•GONPs show distinctly different adsorption properties than other carbon particles.•Unique surface chemistry and morphology control adsorption properties of GONPs.•Adsorption is relatively linear because GO nanoflakes are individually dispersed.•High surface O-content enables strong H-bonding and Lewis acid–base interactions. Colloidal graphene oxide nanoparticles exhibit strong adsorption affinities and characteristic adsorption properties for environmentally relevant aromatics and substituted aromatics.
AbstractList	We conducted batch adsorption experiments to understand the adsorptive properties of colloidal graphene oxide nanoparticles (GONPs) for a range of environmentally relevant aromatics and substituted aromatics, including model nonpolar compounds (pyrene, phenanthrene, naphthalene, and 1,3-dichlorobenzene) and model polar compounds (1-naphthol, 1-naphthylamine, 2,4-dichlorophenol, and 2,4-dinitrotoluene). GONPs exhibited strong adsorption affinities for all the test compounds, with distribution coefficients on the order of 103–106 L/kg. Adsorption to GONPs is much more linear than to carbon nanotubes (CNTs) and C60, likely because GO nanoflakes are essentially individually dispersed (rendering adsorption sites of similar adsorption energy) whereas CNT/C60 are prone to bundling/aggregation. For a given compound GONPs and CNTs often exhibit different adsorption affinities, which is attributable to the differences in both the morphology and surface chemistry between the two nanomaterials. Particularly, the high surface O-content of GONPs enables strong H-bonding and Lewis acid–base interactions with hydroxyl- and amino-substituted aromatics. •Graphene oxide nanoparticles (GONPs) exhibit strong adsorption for aromatics.•GONPs show distinctly different adsorption properties than other carbon particles.•Unique surface chemistry and morphology control adsorption properties of GONPs.•Adsorption is relatively linear because GO nanoflakes are individually dispersed.•High surface O-content enables strong H-bonding and Lewis acid–base interactions. Colloidal graphene oxide nanoparticles exhibit strong adsorption affinities and characteristic adsorption properties for environmentally relevant aromatics and substituted aromatics. We conducted batch adsorption experiments to understand the adsorptive properties of colloidal graphene oxide nanoparticles (GONPs) for a range of environmentally relevant aromatics and substituted aromatics, including model nonpolar compounds (pyrene, phenanthrene, naphthalene, and 1,3-dichlorobenzene) and model polar compounds (1-naphthol, 1-naphthylamine, 2,4-dichlorophenol, and 2,4-dinitrotoluene). GONPs exhibited strong adsorption affinities for all the test compounds, with distribution coefficients on the order of 10(3)-10(6) L/kg. Adsorption to GONPs is much more linear than to carbon nanotubes (CNTs) and C60, likely because GO nanoflakes are essentially individually dispersed (rendering adsorption sites of similar adsorption energy) whereas CNT/C60 are prone to bundling/aggregation. For a given compound GONPs and CNTs often exhibit different adsorption affinities, which is attributable to the differences in both the morphology and surface chemistry between the two nanomaterials. Particularly, the high surface O-content of GONPs enables strong H-bonding and Lewis acid-base interactions with hydroxyl- and amino-substituted aromatics. We conducted batch adsorption experiments to understand the adsorptive properties of colloidal graphene oxide nanoparticles (GONPs) for a range of environmentally relevant aromatics and substituted aromatics, including model nonpolar compounds (pyrene, phenanthrene, naphthalene, and 1,3-dichlorobenzene) and model polar compounds (1-naphthol, 1-naphthylamine, 2,4-dichlorophenol, and 2,4-dinitrotoluene). GONPs exhibited strong adsorption affinities for all the test compounds, with distribution coefficients on the order of 103-106 L/kg. Adsorption to GONPs is much more linear than to carbon nanotubes (CNTs) and C60, likely because GO nanoflakes are essentially individually dispersed (rendering adsorption sites of similar adsorption energy) whereas CNT/C60 are prone to bundling/aggregation. For a given compound GONPs and CNTs often exhibit different adsorption affinities, which is attributable to the differences in both the morphology and surface chemistry between the two nanomaterials. Particularly, the high surface O-content of GONPs enables strong H-bonding and Lewis acid-base interactions with hydroxyl- and amino-substituted aromatics.
Author	Hermens, Joop L.M. Chen, Wei Wang, Fang Sinnige, Theo L. Haftka, Joris J.-H.
Author_xml	– sequence: 1 givenname: Fang surname: Wang fullname: Wang, Fang organization: College of Environmental Science and Engineering, Ministry of Education Key Laboratory of Pollution Processes and Environmental Criteria, Tianjin Key Laboratory of Environmental Remediation and Pollution Control, Nankai University, Wei Jin Road 94, Tianjin 300071, China – sequence: 2 givenname: Joris J.-H. surname: Haftka fullname: Haftka, Joris J.-H. organization: Institute for Risk Assessment Sciences (IRAS), Utrecht University, Yalelaan 104, P.O. Box 80177, 3508 TD Utrecht, The Netherlands – sequence: 3 givenname: Theo L. surname: Sinnige fullname: Sinnige, Theo L. organization: Institute for Risk Assessment Sciences (IRAS), Utrecht University, Yalelaan 104, P.O. Box 80177, 3508 TD Utrecht, The Netherlands – sequence: 4 givenname: Joop L.M. surname: Hermens fullname: Hermens, Joop L.M. email: j.hermens@uu.nl organization: Institute for Risk Assessment Sciences (IRAS), Utrecht University, Yalelaan 104, P.O. Box 80177, 3508 TD Utrecht, The Netherlands – sequence: 5 givenname: Wei surname: Chen fullname: Chen, Wei email: chenwei@nankai.edu.cn organization: College of Environmental Science and Engineering, Ministry of Education Key Laboratory of Pollution Processes and Environmental Criteria, Tianjin Key Laboratory of Environmental Remediation and Pollution Control, Nankai University, Wei Jin Road 94, Tianjin 300071, China
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Keywords	Aromatics Adsorption Polar compounds Graphene oxide nanoparticles Carbonaceous materials Nanoparticle Adsorption capacity Polar compound Pollution Decontamination Model compound Environment Aromatic compound Graphene oxide Nanostructured materials Apolar compound Nanotechnology Organic compounds
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Snippet	We conducted batch adsorption experiments to understand the adsorptive properties of colloidal graphene oxide nanoparticles (GONPs) for a range of...
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SubjectTerms	Adsorption Affinity Applied sciences Aromatic compounds Aromatics Buckminsterfullerene Chlorobenzenes Chlorophenols Exact sciences and technology Fullerenes Global environmental pollution Graphene Graphene oxide nanoparticles Graphite - chemistry Nanoparticles - chemistry Nanotubes, Carbon - chemistry Oxides Polar compounds Pollution Polycyclic Aromatic Hydrocarbons - chemistry Surface chemistry
Title	Adsorption of polar, nonpolar, and substituted aromatics to colloidal graphene oxide nanoparticles
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