Self-Optimizing Continuous Reactions in Supercritical Carbon Dioxide
Hands‐free optimization: A combination of an automated flow reactor, online analysis, and a control algorithm leads to efficient optimization of reactions to a given product without the need for human intervention.
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| Published in: | Angewandte Chemie International Edition Vol. 50; no. 16; pp. 3788 - 3792 |
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| Main Authors: | , , , , |
| Format: | Journal Article |
| Language: | English |
| Published: |
Weinheim
WILEY-VCH Verlag
11-04-2011
WILEY‐VCH Verlag Wiley Subscription Services, Inc |
| Edition: | International ed. in English |
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| Abstract | Hands‐free optimization: A combination of an automated flow reactor, online analysis, and a control algorithm leads to efficient optimization of reactions to a given product without the need for human intervention. |
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| AbstractList | Hands‐free optimization: A combination of an automated flow reactor, online analysis, and a control algorithm leads to efficient optimization of reactions to a given product without the need for human intervention. |
| Author | Akien, Geoffrey R. Poliakoff, Martyn Bourne, Richard A. Irvine, Derek J. Parrott, Andrew J. |
| Author_xml | – sequence: 1 givenname: Andrew J. surname: Parrott fullname: Parrott, Andrew J. organization: School of Chemistry, The University of Nottingham, University Park, Nottingham, NG7 2RD (UK) http://www.nottingham.ac.uk/supercritical – sequence: 2 givenname: Richard A. surname: Bourne fullname: Bourne, Richard A. organization: School of Chemistry, The University of Nottingham, University Park, Nottingham, NG7 2RD (UK) http://www.nottingham.ac.uk/supercritical – sequence: 3 givenname: Geoffrey R. surname: Akien fullname: Akien, Geoffrey R. organization: School of Chemistry, The University of Nottingham, University Park, Nottingham, NG7 2RD (UK) http://www.nottingham.ac.uk/supercritical – sequence: 4 givenname: Derek J. surname: Irvine fullname: Irvine, Derek J. email: derek.irvine@nottingham.ac.uk organization: School of Chemistry, The University of Nottingham, University Park, Nottingham, NG7 2RD (UK) http://www.nottingham.ac.uk/supercritical – sequence: 5 givenname: Martyn surname: Poliakoff fullname: Poliakoff, Martyn email: martyn.poliakoff@nottingham.ac.uk organization: School of Chemistry, The University of Nottingham, University Park, Nottingham, NG7 2RD (UK) http://www.nottingham.ac.uk/supercritical |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/21442710$$D View this record in MEDLINE/PubMed |
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| ContentType | Journal Article |
| Copyright | Copyright © 2011 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim Copyright © 2011 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim |
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| DOI | 10.1002/anie.201100412 |
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| Notes | EU ark:/67375/WNG-DV1ZCLHR-P We thank the EPSRC, grant no. EP/D501229/1 (the DICE project), the EU SYNFLOW project, AstraZeneca, and Croda Europe Ltd. for funding. We also thank David Litchfield, James Warren, Peter Fields, Richard Wilson, and Mark Guyler for technical support. We are grateful to Prof. Walter Leitner for suggesting the Simplex algorithm for self-optimization. EPSRC - No. EP/D501229/1 ArticleID:ANIE201100412 istex:BCEAB3A80DEE440911BEC8142DC22A964BE69390 We thank the EPSRC, grant no. EP/D501229/1 (the DICE project), the EU SYNFLOW project, AstraZeneca, and Croda Europe Ltd. for funding. We also thank David Litchfield, James Warren, Peter Fields, Richard Wilson, and Mark Guyler for technical support. We are grateful to Prof. Walter Leitner for suggesting the Simplex algorithm for self‐optimization. ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 |
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| SubjectTerms | Algorithms Alkylation Carbon Dioxide - chemistry Catalysis heterogeneous catalysis reaction optimization supercritical fluids sustainable chemistry |
| Title | Self-Optimizing Continuous Reactions in Supercritical Carbon Dioxide |
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