Enrichment of gas storage in clathrate hydrates by optimizing the molar liquid water-gas ratio

Enrichment of gas storage in clathrate hydrates by optimizing the molar liquid water-gas ratio

Natural gas (NG) is considered a modern source of energy. Gas hydrates are anticipated to be an alternative method for gas storage and transportation applications. The process must be handy, rapid, and proficient for scale-up. In the present study, methane (CH 4 ) and carbon dioxide (CO 2 ) hydrates...

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Published in:RSC advances Vol. 12; no. 4; pp. 274 - 282
Main Authors: Burla, Sai Kiran, Pinnelli, S. R. Prasad
Format: Journal Article
Language:English
Published: England Royal Society of Chemistry 12-01-2022
The Royal Society of Chemistry
Subjects:
Carbon dioxide
Chemistry
Energy sources
Gas hydrates
Kinetics
Metal surfaces
Methane
Natural gas
Optimization
Storage capacity
Transportation applications
Water
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Abstract Natural gas (NG) is considered a modern source of energy. Gas hydrates are anticipated to be an alternative method for gas storage and transportation applications. The process must be handy, rapid, and proficient for scale-up. In the present study, methane (CH 4 ) and carbon dioxide (CO 2 ) hydrates are synthesized by varying the guest (gas) to host (water) volume. The experiments are performed in a non-stirred system. The results specify that the maximum storage capacity is achieved when the molar liquid water-gas ratio is about 4.08 and 8.25 for CH 4 and CO 2 hydrates. At the optimal water-gas ratios, the total CH 4 and CO 2 gas uptake capacity is about 14.3 ± 0.4 and 9.1 ± 0.4 liters at standard temperature and pressure (STP) conditions. The gas uptake gradually increases with the solution volume and abruptly falls after a threshold point. The hydrate grows across the reactor's metal surface; when the process fully covers the surface, the growth continues horizontally (increase in thickness). With varying the liquid water-gas ratio (low to high), the formation kinetics ( t 90 ) is delayed. The hydrate growth rate gradually decreases and does not significantly influence the hydrate formation temperatures. Optimizing the molar liquid water-gas ratio yields a high gas storage capacity and faster process kinetics. Methane and carbon dioxide storage in hydrate form.
AbstractList Natural gas (NG) is considered a modern source of energy. Gas hydrates are anticipated to be an alternative method for gas storage and transportation applications. The process must be handy, rapid, and proficient for scale-up. In the present study, methane (CH4) and carbon dioxide (CO2) hydrates are synthesized by varying the guest (gas) to host (water) volume. The experiments are performed in a non-stirred system. The results specify that the maximum storage capacity is achieved when the molar liquid water-gas ratio is about 4.08 and 8.25 for CH4 and CO2 hydrates. At the optimal water-gas ratios, the total CH4 and CO2 gas uptake capacity is about 14.3 ± 0.4 and 9.1 ± 0.4 liters at standard temperature and pressure (STP) conditions. The gas uptake gradually increases with the solution volume and abruptly falls after a threshold point. The hydrate grows across the reactor's metal surface; when the process fully covers the surface, the growth continues horizontally (increase in thickness). With varying the liquid water-gas ratio (low to high), the formation kinetics (t 90) is delayed. The hydrate growth rate gradually decreases and does not significantly influence the hydrate formation temperatures. Optimizing the molar liquid water-gas ratio yields a high gas storage capacity and faster process kinetics.Natural gas (NG) is considered a modern source of energy. Gas hydrates are anticipated to be an alternative method for gas storage and transportation applications. The process must be handy, rapid, and proficient for scale-up. In the present study, methane (CH4) and carbon dioxide (CO2) hydrates are synthesized by varying the guest (gas) to host (water) volume. The experiments are performed in a non-stirred system. The results specify that the maximum storage capacity is achieved when the molar liquid water-gas ratio is about 4.08 and 8.25 for CH4 and CO2 hydrates. At the optimal water-gas ratios, the total CH4 and CO2 gas uptake capacity is about 14.3 ± 0.4 and 9.1 ± 0.4 liters at standard temperature and pressure (STP) conditions. The gas uptake gradually increases with the solution volume and abruptly falls after a threshold point. The hydrate grows across the reactor's metal surface; when the process fully covers the surface, the growth continues horizontally (increase in thickness). With varying the liquid water-gas ratio (low to high), the formation kinetics (t 90) is delayed. The hydrate growth rate gradually decreases and does not significantly influence the hydrate formation temperatures. Optimizing the molar liquid water-gas ratio yields a high gas storage capacity and faster process kinetics.
Natural gas (NG) is considered a modern source of energy. Gas hydrates are anticipated to be an alternative method for gas storage and transportation applications. The process must be handy, rapid, and proficient for scale-up. In the present study, methane (CH 4 ) and carbon dioxide (CO 2 ) hydrates are synthesized by varying the guest (gas) to host (water) volume. The experiments are performed in a non-stirred system. The results specify that the maximum storage capacity is achieved when the molar liquid water–gas ratio is about 4.08 and 8.25 for CH 4 and CO 2 hydrates. At the optimal water–gas ratios, the total CH 4 and CO 2 gas uptake capacity is about 14.3 ± 0.4 and 9.1 ± 0.4 liters at standard temperature and pressure (STP) conditions. The gas uptake gradually increases with the solution volume and abruptly falls after a threshold point. The hydrate grows across the reactor's metal surface; when the process fully covers the surface, the growth continues horizontally (increase in thickness). With varying the liquid water–gas ratio (low to high), the formation kinetics ( t 90 ) is delayed. The hydrate growth rate gradually decreases and does not significantly influence the hydrate formation temperatures. Optimizing the molar liquid water–gas ratio yields a high gas storage capacity and faster process kinetics.
Natural gas (NG) is considered a modern source of energy. Gas hydrates are anticipated to be an alternative method for gas storage and transportation applications. The process must be handy, rapid, and proficient for scale-up. In the present study, methane (CH 4 ) and carbon dioxide (CO 2 ) hydrates are synthesized by varying the guest (gas) to host (water) volume. The experiments are performed in a non-stirred system. The results specify that the maximum storage capacity is achieved when the molar liquid water–gas ratio is about 4.08 and 8.25 for CH 4 and CO 2 hydrates. At the optimal water–gas ratios, the total CH 4 and CO 2 gas uptake capacity is about 14.3 ± 0.4 and 9.1 ± 0.4 liters at standard temperature and pressure (STP) conditions. The gas uptake gradually increases with the solution volume and abruptly falls after a threshold point. The hydrate grows across the reactor's metal surface; when the process fully covers the surface, the growth continues horizontally (increase in thickness). With varying the liquid water–gas ratio (low to high), the formation kinetics ( t 90 ) is delayed. The hydrate growth rate gradually decreases and does not significantly influence the hydrate formation temperatures. Optimizing the molar liquid water–gas ratio yields a high gas storage capacity and faster process kinetics. Methane and carbon dioxide storage in hydrate form.
Natural gas (NG) is considered a modern source of energy. Gas hydrates are anticipated to be an alternative method for gas storage and transportation applications. The process must be handy, rapid, and proficient for scale-up. In the present study, methane (CH ) and carbon dioxide (CO ) hydrates are synthesized by varying the guest (gas) to host (water) volume. The experiments are performed in a non-stirred system. The results specify that the maximum storage capacity is achieved when the molar liquid water-gas ratio is about 4.08 and 8.25 for CH and CO hydrates. At the optimal water-gas ratios, the total CH and CO gas uptake capacity is about 14.3 ± 0.4 and 9.1 ± 0.4 liters at standard temperature and pressure (STP) conditions. The gas uptake gradually increases with the solution volume and abruptly falls after a threshold point. The hydrate grows across the reactor's metal surface; when the process fully covers the surface, the growth continues horizontally (increase in thickness). With varying the liquid water-gas ratio (low to high), the formation kinetics ( ) is delayed. The hydrate growth rate gradually decreases and does not significantly influence the hydrate formation temperatures. Optimizing the molar liquid water-gas ratio yields a high gas storage capacity and faster process kinetics.
Natural gas (NG) is considered a modern source of energy. Gas hydrates are anticipated to be an alternative method for gas storage and transportation applications. The process must be handy, rapid, and proficient for scale-up. In the present study, methane (CH4) and carbon dioxide (CO2) hydrates are synthesized by varying the guest (gas) to host (water) volume. The experiments are performed in a non-stirred system. The results specify that the maximum storage capacity is achieved when the molar liquid water–gas ratio is about 4.08 and 8.25 for CH4 and CO2 hydrates. At the optimal water–gas ratios, the total CH4 and CO2 gas uptake capacity is about 14.3 ± 0.4 and 9.1 ± 0.4 liters at standard temperature and pressure (STP) conditions. The gas uptake gradually increases with the solution volume and abruptly falls after a threshold point. The hydrate grows across the reactor's metal surface; when the process fully covers the surface, the growth continues horizontally (increase in thickness). With varying the liquid water–gas ratio (low to high), the formation kinetics (t90) is delayed. The hydrate growth rate gradually decreases and does not significantly influence the hydrate formation temperatures. Optimizing the molar liquid water–gas ratio yields a high gas storage capacity and faster process kinetics.
Author Pinnelli, S. R. Prasad
Burla, Sai Kiran
AuthorAffiliation Academy of Scientific and Innovative Research (AcSIR)
Gas Hydrate Division
CSIR-National Geophysical Research Institute (CSIR-NGRI)
AuthorAffiliation_xml – name: Gas Hydrate Division
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Snippet Natural gas (NG) is considered a modern source of energy. Gas hydrates are anticipated to be an alternative method for gas storage and transportation...
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StartPage 274
SubjectTerms Carbon dioxide
Chemistry
Energy sources
Gas hydrates
Kinetics
Metal surfaces
Methane
Natural gas
Optimization
Storage capacity
Transportation applications
Water
Title Enrichment of gas storage in clathrate hydrates by optimizing the molar liquid water-gas ratio
URI https://www.ncbi.nlm.nih.gov/pubmed/35425253
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https://www.proquest.com/docview/2651685664
https://pubmed.ncbi.nlm.nih.gov/PMC8979132
Volume 12
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