Diblock polymeric friction modifier (PFM) in the boundary regime: Tribological conditions leading to low friction
The aim of this paper is to investigate the tribological conditions required to obtain low friction with a diblock PIB-PEG polymer friction modifier (PFM) blended in base oil (PAO4 +1% wt PFM) under a severe lubrication regime. Two tribological conditions, rolling/sliding and reciprocating pure slid...
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| Published in: | Tribology international Vol. 163; p. 107186 |
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| Abstract | The aim of this paper is to investigate the tribological conditions required to obtain low friction with a diblock PIB-PEG polymer friction modifier (PFM) blended in base oil (PAO4 +1% wt PFM) under a severe lubrication regime. Two tribological conditions, rolling/sliding and reciprocating pure sliding, were investigated. A very low friction coefficient (μ ~ 0.035) was obtained at a temperature of 100 °C whatever the tribometer used. ECR measurements, ToF-SIMS characterizations of wear tracks and AFM analysis suggested the presence of an adsorbed polymer film on the rubbing surfaces. ToF-SIMS characterizations showed that the polymer bonds to the steel substrate through polar functions.
•Low CoF were achieved with a diblock PIB-PEG PFM in severe lubricated contacts.•µ obtained with this PFM are slightly lower than with classical MoDTC additive.•Temperature has a strong influence on the friction behavior of the PFM.•The polymer adsorbs on steel surface through ester linker group. |
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| AbstractList | The aim of this paper is to investigate the tribological conditions required to obtain low friction with a diblock PIB-PEG polymer friction modifier (PFM) blended in base oil (PAO4 + 1% wt PFM) under a severe lubrication regime. Two tribological conditions, rolling/sliding and reciprocating pure sliding, were investigated. A very low friction coefficient (μ ~ 0.035) was obtained at a temperature of 100 °C whatever the tribometer used. ECR measurements, ToF-SIMS characterizations of wear tracks and AFM analysis suggested the presence of an adsorbed polymer film on the rubbing surfaces. ToF-SIMS characterizations showed that the polymer bonds to the steel substrate through polar functions. The aim of this paper is to investigate the tribological conditions required to obtain low friction with a diblock PIB-PEG polymer friction modifier (PFM) blended in base oil (PAO4 +1% wt PFM) under a severe lubrication regime. Two tribological conditions, rolling/sliding and reciprocating pure sliding, were investigated. A very low friction coefficient (μ ~ 0.035) was obtained at a temperature of 100 °C whatever the tribometer used. ECR measurements, ToF-SIMS characterizations of wear tracks and AFM analysis suggested the presence of an adsorbed polymer film on the rubbing surfaces. ToF-SIMS characterizations showed that the polymer bonds to the steel substrate through polar functions. •Low CoF were achieved with a diblock PIB-PEG PFM in severe lubricated contacts.•µ obtained with this PFM are slightly lower than with classical MoDTC additive.•Temperature has a strong influence on the friction behavior of the PFM.•The polymer adsorbs on steel surface through ester linker group. |
| ArticleNumber | 107186 |
| Author | Minfray, Clotilde Thiébaut, Benoît Belin, Michel Dubreuil, Frédéric Kossoko, Nasrya F. |
| Author_xml | – sequence: 1 givenname: Nasrya F. surname: Kossoko fullname: Kossoko, Nasrya F. organization: Ecole Centrale de Lyon, Laboratoire de Tribologie et Dynamique des Systèmes, CNRS-UMR 5513, 36 avenue Guy de Collongue, 69130 Ecully, France – sequence: 2 givenname: Frédéric surname: Dubreuil fullname: Dubreuil, Frédéric organization: Ecole Centrale de Lyon, Laboratoire de Tribologie et Dynamique des Systèmes, CNRS-UMR 5513, 36 avenue Guy de Collongue, 69130 Ecully, France – sequence: 3 givenname: Benoît surname: Thiébaut fullname: Thiébaut, Benoît organization: Total Marketing & Services, Centre de Recherche de Solaize, Chemin du Canal, BP 22, 69360 Solaize, France – sequence: 4 givenname: Michel surname: Belin fullname: Belin, Michel organization: Ecole Centrale de Lyon, Laboratoire de Tribologie et Dynamique des Systèmes, CNRS-UMR 5513, 36 avenue Guy de Collongue, 69130 Ecully, France – sequence: 5 givenname: Clotilde surname: Minfray fullname: Minfray, Clotilde email: clotilde.minfray@ec-lyon.fr organization: Ecole Centrale de Lyon, Laboratoire de Tribologie et Dynamique des Systèmes, CNRS-UMR 5513, 36 avenue Guy de Collongue, 69130 Ecully, France |
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| CitedBy_id | crossref_primary_10_3390_lubricants11050196 crossref_primary_10_1016_j_jcis_2023_09_146 crossref_primary_10_1007_s00339_023_06873_x crossref_primary_10_1007_s40544_022_0685_7 crossref_primary_10_1115_1_4054398 |
| Cites_doi | 10.1021/la703152q 10.1002/ls.3010140204 10.1016/j.triboint.2016.10.042 10.1520/JAI100956 10.1007/s11249-019-1198-z 10.1007/s11249-011-9903-6 10.1016/S0167-8922(08)70476-0 10.1016/j.triboint.2017.05.010 10.1007/s11249-019-1162-y 10.1007/s11249-007-9231-z 10.1007/s11249-007-9272-3 10.1016/j.triboint.2008.12.012 10.1007/s11249-005-9000-9 10.1021/acs.langmuir.7b02528 10.1021/acs.langmuir.9b03668 10.1016/j.triboint.2019.105954 10.1080/10402009608983590 10.1007/s11249-015-0589-z 10.1007/s11249-016-0771-y 10.1016/j.apsusc.2019.145020 10.1007/s40544-016-0107-9 10.1021/acsami.8b16849 10.1023/A:1024861119372 |
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| Keywords | AFM Boundary lubrication ToF-SIMS Polymer friction modifier |
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| SubjectTerms | AFM Boundary lubrication Coefficient of friction Engineering Sciences Friction Polymer films Polymer friction modifier Polymers Rubbing Sliding Substrates ToF-SIMS Tribology |
| Title | Diblock polymeric friction modifier (PFM) in the boundary regime: Tribological conditions leading to low friction |
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