Adsorption on Heterogeneous Surfaces: Site Energy Distribution Functions from Fritz-Schlüender Isotherms
Different site energy distribution functions based on the condensation approximation method are proposed for the liquid‐phase or gas‐phase adsorption equilibrium data following the Fritz–Schlüender isotherm. Energy distribution functions for the four limiting cases of the Fritz–Schlüender isotherm a...
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| Published in: | Chemphyschem Vol. 11; no. 12; pp. 2555 - 2560 |
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| Format: | Journal Article |
| Language: | English |
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Weinheim
WILEY-VCH Verlag
23-08-2010
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| Abstract | Different site energy distribution functions based on the condensation approximation method are proposed for the liquid‐phase or gas‐phase adsorption equilibrium data following the Fritz–Schlüender isotherm. Energy distribution functions for the four limiting cases of the Fritz–Schlüender isotherm are also discussed. The proposed models are successfully applied to the experimental equilibrium data of nitrogen molecules at 77 K on a pitch‐based activated carbon (PA) and a pitch‐based activated carbon containing boron (PBA). An energy distribution function based on FS isotherm containing five parameters suggest a unimodal distribution of binding sites for carbon PA, the binding site energies being distributed as exponential or unimodal, depending on the pressure, in the case of carbon PBA. The advantages of the proposed models are discussed.
Binding sites: A model based on the Fritz–Schlüender isotherm predicts the site energy distribution of heterogeneous surfaces on pitch‐based activated carbon with and without boron (PBA and PA, respectively, see figure). A unimodal distribution of binding sites occurs for carbon PA, the binding site energies being distributed exponentially or unimodaly (depending on the pressure) in the case of PBA. |
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| AbstractList | Different site energy distribution functions based on the condensation approximation method are proposed for the liquid‐phase or gas‐phase adsorption equilibrium data following the Fritz–Schlüender isotherm. Energy distribution functions for the four limiting cases of the Fritz–Schlüender isotherm are also discussed. The proposed models are successfully applied to the experimental equilibrium data of nitrogen molecules at 77 K on a pitch‐based activated carbon (PA) and a pitch‐based activated carbon containing boron (PBA). An energy distribution function based on FS isotherm containing five parameters suggest a unimodal distribution of binding sites for carbon PA, the binding site energies being distributed as exponential or unimodal, depending on the pressure, in the case of carbon PBA. The advantages of the proposed models are discussed. Different site energy distribution functions based on the condensation approximation method are proposed for the liquid‐phase or gas‐phase adsorption equilibrium data following the Fritz–Schlüender isotherm. Energy distribution functions for the four limiting cases of the Fritz–Schlüender isotherm are also discussed. The proposed models are successfully applied to the experimental equilibrium data of nitrogen molecules at 77 K on a pitch‐based activated carbon (PA) and a pitch‐based activated carbon containing boron (PBA). An energy distribution function based on FS isotherm containing five parameters suggest a unimodal distribution of binding sites for carbon PA, the binding site energies being distributed as exponential or unimodal, depending on the pressure, in the case of carbon PBA. The advantages of the proposed models are discussed. Binding sites: A model based on the Fritz–Schlüender isotherm predicts the site energy distribution of heterogeneous surfaces on pitch‐based activated carbon with and without boron (PBA and PA, respectively, see figure). A unimodal distribution of binding sites occurs for carbon PA, the binding site energies being distributed exponentially or unimodaly (depending on the pressure) in the case of PBA. |
| Author | Molina-Sabio, Miguel Martinez-Escandell, Manuel Monteiro de Castro, Mateus Carvalho Kumar, Kannuchamy Vasanth Rodriguez-Reinoso, Francisco |
| Author_xml | – sequence: 1 givenname: Kannuchamy Vasanth surname: Kumar fullname: Kumar, Kannuchamy Vasanth email: vasanth@ua.es organization: Laboratorio de Materiales Avanzados, Departamento de Química Inorgánica, Universidad de Alicante, Apartado 99. 030080 Alicante (Spain), Fax: (+34)-9659 03454 – sequence: 2 givenname: Mateus Carvalho surname: Monteiro de Castro fullname: Monteiro de Castro, Mateus Carvalho organization: Laboratorio de Materiales Avanzados, Departamento de Química Inorgánica, Universidad de Alicante, Apartado 99. 030080 Alicante (Spain), Fax: (+34)-9659 03454 – sequence: 3 givenname: Manuel surname: Martinez-Escandell fullname: Martinez-Escandell, Manuel organization: Laboratorio de Materiales Avanzados, Departamento de Química Inorgánica, Universidad de Alicante, Apartado 99. 030080 Alicante (Spain), Fax: (+34)-9659 03454 – sequence: 4 givenname: Miguel surname: Molina-Sabio fullname: Molina-Sabio, Miguel organization: Laboratorio de Materiales Avanzados, Departamento de Química Inorgánica, Universidad de Alicante, Apartado 99. 030080 Alicante (Spain), Fax: (+34)-9659 03454 – sequence: 5 givenname: Francisco surname: Rodriguez-Reinoso fullname: Rodriguez-Reinoso, Francisco organization: Laboratorio de Materiales Avanzados, Departamento de Química Inorgánica, Universidad de Alicante, Apartado 99. 030080 Alicante (Spain), Fax: (+34)-9659 03454 |
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| Cites_doi | 10.1016/j.jhazmat.2004.09.016 10.1016/0095-8522(59)90067-4 10.1021/i160044a003 10.1021/ac0105686 10.1021/j150576a611 10.1016/0040-6090(74)90235-1 10.1016/j.carbon.2009.10.005 10.1016/j.carbon.2008.01.011 10.1016/j.jcis.2005.06.021 10.1016/j.snb.2006.10.068 10.1021/je800161m 10.1038/nprot.2006.370 10.1016/S0008-6223(99)00028-7 10.1016/0039-6028(75)90044-8 10.1016/j.jchromb.2004.01.064 10.1016/S0008-6223(99)00133-5 10.1016/0003-2697(75)90193-1 10.1021/je020161d 10.1021/es00007a013 10.1021/ja01187a013 10.1021/ja02268a002 10.1016/0375-9601(76)90785-4 10.1039/b002354j 10.1016/0009-2509(74)80128-4 10.1016/j.jcis.2007.09.091 |
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| Keywords | Heterogeneous surface Energy distribution functions Liquid solid adsorption Adsorption isotherm Nitrogen Condensation Fritz-Schlüender isotherm Gas solid adsorption Boron Adsorption Activated carbon Distribution function Isotherm heterogeneous surfaces site energy distribution Modified material condensation approximation method |
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| SubjectTerms | Adsorbents Chemistry condensation approximation method Exact sciences and technology Fritz-Schlüender isotherm General and physical chemistry heterogeneous surfaces site energy distribution Surface physical chemistry |
| Title | Adsorption on Heterogeneous Surfaces: Site Energy Distribution Functions from Fritz-Schlüender Isotherms |
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