Molecular functionalization of tantalum oxide surface towards development of apatite growth
We have studied the apatite growth dynamics on tantalum oxide surfaces. This nucleation is obtained via an organosilane intermediate layer between the apatite and the substrate surface. Four organosilane layers (differing by their terminal functionality) were investigated. Their characterization wit...
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| Published in: | Applied surface science Vol. 255; no. 9; pp. 4765 - 4772 |
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| Main Authors: | , , , , , , |
| Format: | Journal Article |
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Elsevier B.V
15-02-2009
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| Abstract | We have studied the apatite growth dynamics on tantalum oxide surfaces. This nucleation is obtained via an organosilane intermediate layer between the apatite and the substrate surface. Four organosilane layers (differing by their terminal functionality) were investigated. Their characterization with atomic force microscopy and other techniques such as X-ray photoelectron spectroscopy (XPS) and wetting measurements highlighted the influence of the organosilane terminal groups on the apatite growth rates. Results revealed that apatite is indeed growing faster on phosphate terminal groups than on the three other groups studied (vinyl, hydroxyl and carboxyl). |
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| AbstractList | We have studied the apatite growth dynamics on tantalum oxide surfaces. This nucleation is obtained via an organosilane intermediate layer between the apatite and the substrate surface. Four organosilane layers (differing by their terminal functionality) were investigated. Their characterization with atomic force microscopy and other techniques such as X-ray photoelectron spectroscopy (XPS) and wetting measurements highlighted the influence of the organosilane terminal groups on the apatite growth rates. Results revealed that apatite is indeed growing faster on phosphate terminal groups than on the three other groups studied (vinyl, hydroxyl and carboxyl). |
| Author | Aubry, D. Volcke, C. Humbert, C. Thiry, P.A. Delhalle, J. Arnould, Ch Mekhalif, Z. |
| Author_xml | – sequence: 1 givenname: D. surname: Aubry fullname: Aubry, D. organization: Laboratory of Chemistry and Electrochemistry of Surfaces (CES), University of Namur, FUNDP, Rue de Bruxelles 61, B-5000 Namur, Belgium – sequence: 2 givenname: C. surname: Volcke fullname: Volcke, C. organization: Research Center in Physics of Matter and Radiation (PMR), University of Namur, FUNDP, Rue de Bruxelles 61, B-5000 Namur, Belgium – sequence: 3 givenname: Ch surname: Arnould fullname: Arnould, Ch organization: Laboratory of Chemistry and Electrochemistry of Surfaces (CES), University of Namur, FUNDP, Rue de Bruxelles 61, B-5000 Namur, Belgium – sequence: 4 givenname: C. surname: Humbert fullname: Humbert, C. organization: Research Center in Physics of Matter and Radiation (PMR), University of Namur, FUNDP, Rue de Bruxelles 61, B-5000 Namur, Belgium – sequence: 5 givenname: P.A. surname: Thiry fullname: Thiry, P.A. organization: Research Center in Physics of Matter and Radiation (PMR), University of Namur, FUNDP, Rue de Bruxelles 61, B-5000 Namur, Belgium – sequence: 6 givenname: J. surname: Delhalle fullname: Delhalle, J. organization: Laboratory of Chemistry and Electrochemistry of Surfaces (CES), University of Namur, FUNDP, Rue de Bruxelles 61, B-5000 Namur, Belgium – sequence: 7 givenname: Z. surname: Mekhalif fullname: Mekhalif, Z. email: zineb.mekhalif@fundp.ac.be organization: Laboratory of Chemistry and Electrochemistry of Surfaces (CES), University of Namur, FUNDP, Rue de Bruxelles 61, B-5000 Namur, Belgium |
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| Keywords | Atomic force microscopy Apatite Tantalum Self-assembled monolayers X-ray photoelectron spectroscopy Biomaterials Transition elements Self-assembled layers X-ray photoelectron spectra |
| Language | English |
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| SubjectTerms | Apatite Atomic force microscopy Biomaterials Chemical Physics Condensed Matter Condensed matter: electronic structure, electrical, magnetic, and optical properties Condensed matter: structure, mechanical and thermal properties Cross-disciplinary physics: materials science; rheology Exact sciences and technology Materials Science Physics Self-assembled monolayers Tantalum X-ray photoelectron spectroscopy |
| Title | Molecular functionalization of tantalum oxide surface towards development of apatite growth |
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