Sources, distribution and variability of hydrocarbons in total atmospheric suspended particulates of two Brazilian areas influenced by sugarcane burning

Polycyclic aromatic hydrocarbons (PAHs) and aliphatic hydrocarbons (AHs), such as n-alkanes, hopanes and steranes, were studied in relation to total atmospheric suspended particulates (TSP). Two representative Brazilian cities affected by sugarcane monoculture practices, with their rural surrounding...

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Published in:	Journal of atmospheric chemistry Vol. 64; no. 2-3; pp. 159 - 178
Main Authors:	Maioli, Otávio L. G, Knoppers, Bastiaan A, Azevedo, Débora A
Format:	Journal Article
Language:	English
Published:	Dordrecht Dordrecht : Springer Netherlands 01-12-2009 Springer Netherlands Springer Springer Nature B.V
Subjects:	Air pollution Aliphatic hydrocarbons Applied sciences Atmospheric boundary layer Atmospheric pollution Atmospheric Protection/Air Quality Control/Air Pollution Atmospheric Sciences Earth and Environmental Science Earth Sciences Exact sciences and technology Fires Hydrocarbons Monoculture PAHs Petroleum biomarkers Pollutants physicochemistry study: properties, effects, reactions, transport and distribution Pollution Pollution sources Polycyclic aromatic hydrocarbons Sugarcane Sugarcane burning Suspended particulate matter Urban areas South America Brazil America ASW, Brazil, Alagoas Brazil, Alagoas Brazil, Rio de Janeiro PAHs Petroleum biomarkers Aliphatic hydrocarbons Pollution sources Sugarcane burning Biological marker Identification Urban area Mutagen Controlled burning Persistent organic pollutant Rural area Organic compounds Anthropogenic factor Natural origin pollution Hydrocarbon Aliphatic compound Polycyclic aromatic compound Carcinogen Biogenic factor Crop residues Aerosols Pollution source inventory Air pollution Dissolved inorganic carbon
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Abstract	Polycyclic aromatic hydrocarbons (PAHs) and aliphatic hydrocarbons (AHs), such as n-alkanes, hopanes and steranes, were studied in relation to total atmospheric suspended particulates (TSP). Two representative Brazilian cities affected by sugarcane monoculture practices, with their rural surroundings, were chosen for the study. The cities chosen were Maceió (state of Alagoas, NE-Brazil) and Campos dos Goytacazes (state of Rio de Janeiro, SE-Brazil). Samples were collected during the harvesting period, when sugarcane burning occurs, and during the non-harvesting period. The aliphatic hydrocarbon fingerprints suggest a marked contribution of biogenic inputs and a slight contamination by aliphatics in areas far from the urban regions. In the urban areas, some petroleum contributions were observed, marked by the presence of hopanes (m/z 191) and steranes (m/z 217) in the mass chromatographic profiles. A marked increase in PAH concentrations was detected during the sugarcane burning periods, mainly at Campos dos Goytacazes. In a similar approach, n-alkane concentrations and BaP/nC₂₄ ratios were higher during the sugarcane burning periods. These increases were mainly associated with PAH production by the pyrogenic process in relation to aliphatic hydrocarbons with the same carbon numbers. The PAH isomeric ratios and the mixture of petrogenic and pyrogenic compounds of the TSP suggest atmospheric contamination for all regions as a whole, but the more elevated pyrogenic contribution during the sugarcane burning period implies that the impact of this activity is relevant.
AbstractList	Polycyclic aromatic hydrocarbons (PAHs) and aliphatic hydrocarbons (AHs), such as n-alkanes, hopanes and steranes, were studied in relation to total atmospheric suspended particulates (TSP). Two representative Brazilian cities affected by sugarcane monoculture practices, with their rural surroundings, were chosen for the study. The cities chosen were Maceió (state of Alagoas, NE-Brazil) and Campos dos Goytacazes (state of Rio de Janeiro, SE-Brazil). Samples were collected during the harvesting period, when sugarcane burning occurs, and during the non-harvesting period. The aliphatic hydrocarbon fingerprints suggest a marked contribution of biogenic inputs and a slight contamination by aliphatics in areas far from the urban regions. In the urban areas, some petroleum contributions were observed, marked by the presence of hopanes (m/z 191) and steranes (m/z 217) in the mass chromatographic profiles. A marked increase in PAH concentrations was detected during the sugarcane burning periods, mainly at Campos dos Goytacazes. In a similar approach, n-alkane concentrations and BaP/nC^sub 24^ ratios were higher during the sugarcane burning periods. These increases were mainly associated with PAH production by the pyrogenic process in relation to aliphatic hydrocarbons with the same carbon numbers. The PAH isomeric ratios and the mixture of petrogenic and pyrogenic compounds of the TSP suggest atmospheric contamination for all regions as a whole, but the more elevated pyrogenic contribution during the sugarcane burning period implies that the impact of this activity is relevant.[PUBLICATION ABSTRACT] Polycyclic aromatic hydrocarbons (PAHs) and aliphatic hydrocarbons (AHs), such as n-alkanes, hopanes and steranes, were studied in relation to total atmospheric suspended particulates (TSP). Two representative Brazilian cities affected by sugarcane monoculture practices, with their rural surroundings, were chosen for the study. The cities chosen were Maceio (state of Alagoas, NE-Brazil) and Campos dos Goytacazes (state of Rio de Janeiro, SE-Brazil). Samples were collected during the harvesting period, when sugarcane burning occurs, and during the non-harvesting period. The aliphatic hydrocarbon fingerprints suggest a marked contribution of biogenic inputs and a slight contamination by aliphatics in areas far from the urban regions. In the urban areas, some petroleum contributions were observed, marked by the presence of hopanes (m/z 191) and steranes (m/z 217) in the mass chromatographic profiles. A marked increase in PAH concentrations was detected during the sugarcane burning periods, mainly at Campos dos Goytacazes. In a similar approach, n-alkane concentrations and BaP/nC sub(24) ratios were higher during the sugarcane burning periods. These increases were mainly associated with PAH production by the pyrogenic process in relation to aliphatic hydrocarbons with the same carbon numbers. The PAH isomeric ratios and the mixture of petrogenic and pyrogenic compounds of the TSP suggest atmospheric contamination for all regions as a whole, but the more elevated pyrogenic contribution during the sugarcane burning period implies that the impact of this activity is relevant. Polycyclic aromatic hydrocarbons (PAHs) and aliphatic hydrocarbons (AHs), such as n-alkanes, hopanes and steranes, were studied in relation to total atmospheric suspended particulates (TSP). Two representative Brazilian cities affected by sugarcane monoculture practices, with their rural surroundings, were chosen for the study. The cities chosen were Maceió (state of Alagoas, NE-Brazil) and Campos dos Goytacazes (state of Rio de Janeiro, SE-Brazil). Samples were collected during the harvesting period, when sugarcane burning occurs, and during the non-harvesting period. The aliphatic hydrocarbon fingerprints suggest a marked contribution of biogenic inputs and a slight contamination by aliphatics in areas far from the urban regions. In the urban areas, some petroleum contributions were observed, marked by the presence of hopanes (m/z 191) and steranes (m/z 217) in the mass chromatographic profiles. A marked increase in PAH concentrations was detected during the sugarcane burning periods, mainly at Campos dos Goytacazes. In a similar approach, n-alkane concentrations and BaP/nC₂₄ ratios were higher during the sugarcane burning periods. These increases were mainly associated with PAH production by the pyrogenic process in relation to aliphatic hydrocarbons with the same carbon numbers. The PAH isomeric ratios and the mixture of petrogenic and pyrogenic compounds of the TSP suggest atmospheric contamination for all regions as a whole, but the more elevated pyrogenic contribution during the sugarcane burning period implies that the impact of this activity is relevant. Polycyclic aromatic hydrocarbons (PAHs) and aliphatic hydrocarbons (AHs), such as n -alkanes, hopanes and steranes, were studied in relation to total atmospheric suspended particulates (TSP). Two representative Brazilian cities affected by sugarcane monoculture practices, with their rural surroundings, were chosen for the study. The cities chosen were Maceió (state of Alagoas, NE-Brazil) and Campos dos Goytacazes (state of Rio de Janeiro, SE-Brazil). Samples were collected during the harvesting period, when sugarcane burning occurs, and during the non-harvesting period. The aliphatic hydrocarbon fingerprints suggest a marked contribution of biogenic inputs and a slight contamination by aliphatics in areas far from the urban regions. In the urban areas, some petroleum contributions were observed, marked by the presence of hopanes ( m/z 191) and steranes ( m/z 217) in the mass chromatographic profiles. A marked increase in PAH concentrations was detected during the sugarcane burning periods, mainly at Campos dos Goytacazes. In a similar approach, n -alkane concentrations and BaP/ n C 24 ratios were higher during the sugarcane burning periods. These increases were mainly associated with PAH production by the pyrogenic process in relation to aliphatic hydrocarbons with the same carbon numbers. The PAH isomeric ratios and the mixture of petrogenic and pyrogenic compounds of the TSP suggest atmospheric contamination for all regions as a whole, but the more elevated pyrogenic contribution during the sugarcane burning period implies that the impact of this activity is relevant.
Author	Maioli, Otávio L. G Azevedo, Débora A Knoppers, Bastiaan A
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CitedBy_id	crossref_primary_10_5194_se_5_1305_2014 crossref_primary_10_1016_j_envpol_2018_04_109 crossref_primary_10_1134_S106422931603011X crossref_primary_10_1134_S106422931301002X crossref_primary_10_1016_j_csr_2011_04_004 crossref_primary_10_5094_APR_2014_011 crossref_primary_10_1007_s11270_011_0827_4 crossref_primary_10_1002_bbb_1405 crossref_primary_10_1134_S1064229313070090
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Keywords	PAHs Petroleum biomarkers Aliphatic hydrocarbons Pollution sources Sugarcane burning Biological marker Identification Urban area Mutagen Controlled burning Persistent organic pollutant Rural area Organic compounds Anthropogenic factor Natural origin pollution Hydrocarbon Aliphatic compound Polycyclic aromatic compound Carcinogen Biogenic factor Crop residues Aerosols Pollution source inventory Air pollution Dissolved inorganic carbon
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Publisher	Dordrecht : Springer Netherlands Springer Netherlands Springer Springer Nature B.V
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Snippet	Polycyclic aromatic hydrocarbons (PAHs) and aliphatic hydrocarbons (AHs), such as n-alkanes, hopanes and steranes, were studied in relation to total... Polycyclic aromatic hydrocarbons (PAHs) and aliphatic hydrocarbons (AHs), such as n -alkanes, hopanes and steranes, were studied in relation to total...
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SubjectTerms	Air pollution Aliphatic hydrocarbons Applied sciences Atmospheric boundary layer Atmospheric pollution Atmospheric Protection/Air Quality Control/Air Pollution Atmospheric Sciences Earth and Environmental Science Earth Sciences Exact sciences and technology Fires Hydrocarbons Monoculture PAHs Petroleum biomarkers Pollutants physicochemistry study: properties, effects, reactions, transport and distribution Pollution Pollution sources Polycyclic aromatic hydrocarbons Sugarcane Sugarcane burning Suspended particulate matter Urban areas
Title	Sources, distribution and variability of hydrocarbons in total atmospheric suspended particulates of two Brazilian areas influenced by sugarcane burning
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