Effect of ozonation on chemical oxygen demand fractionation and color profile of textile wastewaters
Filtration and ultrafiltration with a size range of 2–1600 nm were used to evaluate the effect of ozonation on the particle size distribution‐based chemical oxygen demand (COD) and color profiles of textile wastewater before and after biological treatment. Ozonation induced a net effect of 9% COD re...
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| Published in: | Journal of chemical technology and biotechnology (1986) Vol. 81; no. 3; pp. 426 - 432 |
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| Language: | English |
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Chichester, UK
John Wiley & Sons, Ltd
01-03-2006
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| Abstract | Filtration and ultrafiltration with a size range of 2–1600 nm were used to evaluate the effect of ozonation on the particle size distribution‐based chemical oxygen demand (COD) and color profiles of textile wastewater before and after biological treatment. Ozonation induced a net effect of 9% COD reduction in the influent and 15% in the effluent. However, a more in‐depth evaluation based on particle size distribution and mass balance for the influent revealed different mechanisms of ozonation, which were interpreted as total oxidation in the soluble range, replenishment of soluble COD through solubilization of organics into simpler compounds and polymerization towards the upper size range (>220 nm). For the biological treatment effluent, the greatest effect of ozonation was in the lower particle size range (<8 nm). Ozone was very effective for color removal, giving 80–93% optical density reductions in the influent and 96–99% in the effluent, depending on the excitation wavelength selected. Ozonation of the influent removed practically all color fractions, except in the particulate range. In the effluent, the particulate fraction was removed by biological treatment and settling and consequently the remaining color were almost entirely removed by ozonation. Copyright © 2005 Society of Chemical Industry |
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| AbstractList | Filtration and ultrafiltration with a size range of 2-1600 nm were used to evaluate the effect of ozonation on the particle size distribution-based chemical oxygen demand (COD) and color profiles of textile wastewater before and after biological treatment. Ozonation induced a net effect of 9% COD reduction in the influent and 15% in the effluent. However, a more in-depth evaluation based on particle size distribution and mass balance for the influent revealed different mechanisms of ozonation, which were interpreted as total oxidation in the soluble range, replenishment of soluble COD through solubilization of organics into simpler compounds and polymerization towards the upper size range ( > 220nm). For the biological treatment effluent, the greatest effect of ozonation was in the lower particle size range ( < 8 nm). Ozone was very effective for color removal, giving 80-93% optical density reductions in the influent and 96-99% in the effluent, depending on the excitation wavelength selected. Ozonation of the influent removed practically all color fractions, except in the particulate range. In the effluent, the particulate fraction was removed by biological treatment and settling and consequently the remaining color were almost entirely removed by ozonation. Filtration and ultrafiltration with a size range of 2–1600 nm were used to evaluate the effect of ozonation on the particle size distribution‐based chemical oxygen demand (COD) and color profiles of textile wastewater before and after biological treatment. Ozonation induced a net effect of 9% COD reduction in the influent and 15% in the effluent. However, a more in‐depth evaluation based on particle size distribution and mass balance for the influent revealed different mechanisms of ozonation, which were interpreted as total oxidation in the soluble range, replenishment of soluble COD through solubilization of organics into simpler compounds and polymerization towards the upper size range (>220 nm). For the biological treatment effluent, the greatest effect of ozonation was in the lower particle size range (<8 nm). Ozone was very effective for color removal, giving 80–93% optical density reductions in the influent and 96–99% in the effluent, depending on the excitation wavelength selected. Ozonation of the influent removed practically all color fractions, except in the particulate range. In the effluent, the particulate fraction was removed by biological treatment and settling and consequently the remaining color were almost entirely removed by ozonation. Copyright © 2005 Society of Chemical Industry |
| Author | Doǧruel, Serdar Dulekgurgen, Ebru Orhon, Derin |
| Author_xml | – sequence: 1 givenname: Serdar surname: Doǧruel fullname: Doǧruel, Serdar email: sdogruel@ins.itu.edu.tr organization: Environmental Engineering Department, Faculty of Civil Engineering, Istanbul Technical University, İTÜ İnşaat Fakültesi, Maslak 34469, Istanbul, Turkey – sequence: 2 givenname: Ebru surname: Dulekgurgen fullname: Dulekgurgen, Ebru organization: Environmental Engineering Department, Faculty of Civil Engineering, Istanbul Technical University, İTÜ İnşaat Fakültesi, Maslak 34469, Istanbul, Turkey – sequence: 3 givenname: Derin surname: Orhon fullname: Orhon, Derin organization: Environmental Engineering Department, Faculty of Civil Engineering, Istanbul Technical University, İTÜ İnşaat Fakültesi, Maslak 34469, Istanbul, Turkey |
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| Cites_doi | 10.2166/wst.1994.0115 10.1016/S0273-1223(99)00357-1 10.1016/j.chemosphere.2003.11.032 10.1016/0043-1354(92)90192-7 10.2166/wst.2002.0439 10.1016/0043-1354(91)90138-G 10.1002/jctb.713 10.1016/S0043-1354(01)00273-1 10.1016/S0273-1223(98)00296-0 10.2166/wst.2001.0265 |
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| Keywords | textile wastewaters Color Membrane separation Ozonization Particle size distribution Ultrafiltration Chemical oxygen demand Industrial waste water ozonation Textile industry Speciation chemical oxygen demand fractionation color profile |
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| References | Sophonsiri C and Morgenroth E, Chemical composition associated with different particle size fractions in municipal, industrial and agricultural wastewaters. Chemosphere 55: 691-703 (2004). Jekel MK, Effects and mechanisms involved in preoxidation and particle separation processes. Water Sci Technol 37: 1-7 (1998). Hu Z, Chandran K, Barth FS and Domenico G, Evaluation of a rapid physical-chemical method for the determination of extant soluble COD. Water Res 36: 617-624 (2002). Orhon D and Artan N, Modelling of Activated Sludge Systems. Technomic Press, Lancaster, PA (1994). American Public Health Association, American Water Works Association and Water Environment Federation, Standard Methods for the Examination of Water and Wastewater, 20th edn. APHA, Washington, DC (1998). Water Quality-Determination of the Chemical Oxygen Demand. ISO 6060-1986, 1st edn. International Standards Organization, Geneva (1986). Ollis DF, On the need for engineering models of integrated chemical and biological oxidation of wastewaters. Water Sci Technol 44: 117-123 (2001). Dulekgurgen E, Doǧruel S, Karahan Ö and Orhon D, Size distribution of wastewater COD fractions as an index for biodegradability. Water Res in press. Orhon D, Taşlı R and Sözen S, Experimental basis of activated sludge treatment for industrial wastewaters-the state of the art. Water Sci Technol 40: 1-11 (1999). Wentzel MC, Mbewe A, Lakay MT and Ekama GA, Batch test for characterization of the carbonaceous materials in municipal wastewaters. Water SA 25: 327-335 (1999). McGregor WC, Membrane Separations in Biotechnology. Marcel Dekker, New York, NY (1986). Gaehr F, Hermanutz F and Oppermann W, Ozonation-an important technique to comply with new German laws for textile wastewater treatment. Water Sci Technol 30: 255-263 (1994). Doǧruel S, Germirli-Babuna F, Kabdaşlı I, İnsel G and Orhon D, Effect of stream segregation on ozonation for the removal of significant COD fractions from textile wastewater. J Chem Technol Biotechnol 78: 6-14 (2003). Levine AD, Tchobanoglous G and Asano T, Size distributions of particulate contaminants wastewater and their impact on treatability. Water Res 25: 911-922 (1991). Cheryan M, Ultrafiltration and Microfiltration Handbook. Technomic, Lancaster, PA (1986). Kuo WG, Decolorizing dye wastewater with Fenton's reagent. Water Res 26: 881-886 (1992). Orhon D, Dulkadiroǧlu H, Doǧruel S, Kabdaşlı I, Sözen S and Germirli-Babuna F, Pre- or post ozonation application in activated sludge systems for a textile mill effluent. Water Sci Technol 45: 305-313 (2002). 2004; 55 1998; 37 2002; 36 1991; 25 2000 2002; 45 1999; 25 1998 1986 1994 2004 1992; 26 1999; 40 2001; 44 1994; 30 2003; 78 Orhon D (e_1_2_6_4_2) 1994 Dulekgurgen E (e_1_2_6_9_2) (e_1_2_6_11_2) 1986 e_1_2_6_20_2 Orhon D (e_1_2_6_6_2) 2002; 45 Wentzel MC (e_1_2_6_7_2) 1999; 25 American Public Health Association, American Water Works Association and Water Environment Federation (e_1_2_6_10_2) 1998 Gaehr F (e_1_2_6_3_2) 1994; 30 McGregor WC (e_1_2_6_16_2) 1986 e_1_2_6_8_2 e_1_2_6_18_2 Ollis DF (e_1_2_6_19_2) 2001; 44 Cheryan M (e_1_2_6_15_2) 1986 e_1_2_6_5_2 e_1_2_6_12_2 e_1_2_6_13_2 e_1_2_6_2_2 e_1_2_6_21_2 e_1_2_6_17_2 e_1_2_6_14_2 |
| References_xml | – volume: 44 start-page: 117 year: 2001 end-page: 123 article-title: On the need for engineering models of integrated chemical and biological oxidation of wastewaters publication-title: Water Sci Technol – volume: 45 start-page: 305 year: 2002 end-page: 313 article-title: Pre‐ or post ozonation application in activated sludge systems for a textile mill effluent publication-title: Water Sci Technol – year: 1986 – article-title: Size distribution of wastewater COD fractions as an index for biodegradability publication-title: Water Res – volume: 55 start-page: 691 year: 2004 end-page: 703 article-title: Chemical composition associated with different particle size fractions in municipal, industrial and agricultural wastewaters publication-title: Chemosphere – volume: 25 start-page: 911 year: 1991 end-page: 922 article-title: Size distributions of particulate contaminants wastewater and their impact on treatability publication-title: Water Res – volume: 78 start-page: 6 year: 2003 end-page: 14 article-title: Effect of stream segregation on ozonation for the removal of significant COD fractions from textile wastewater publication-title: J Chem Technol Biotechnol – volume: 25 start-page: 327 year: 1999 end-page: 335 article-title: Batch test for characterization of the carbonaceous materials in municipal wastewaters publication-title: Water SA – volume: 26 start-page: 881 year: 1992 end-page: 886 article-title: Decolorizing dye wastewater with Fenton's reagent publication-title: Water Res – year: 2004 – year: 2000 – volume: 40 start-page: 1 year: 1999 end-page: 11 article-title: Experimental basis of activated sludge treatment for industrial wastewaters—the state of the art publication-title: Water Sci Technol – volume: 37 start-page: 1 year: 1998 end-page: 7 article-title: Effects and mechanisms involved in preoxidation and particle separation processes publication-title: Water Sci Technol – volume: 30 start-page: 255 year: 1994 end-page: 263 article-title: Ozonation—an important technique to comply with new German laws for textile wastewater treatment publication-title: Water Sci Technol – year: 1994 – year: 1998 – volume: 36 start-page: 617 year: 2002 end-page: 624 article-title: Evaluation of a rapid physical–chemical method for the determination of extant soluble COD publication-title: Water Res – volume: 30 start-page: 255 year: 1994 ident: e_1_2_6_3_2 article-title: Ozonation—an important technique to comply with new German laws for textile wastewater treatment publication-title: Water Sci Technol doi: 10.2166/wst.1994.0115 contributor: fullname: Gaehr F – volume-title: Membrane Separations in Biotechnology year: 1986 ident: e_1_2_6_16_2 contributor: fullname: McGregor WC – ident: e_1_2_6_21_2 doi: 10.1016/S0273-1223(99)00357-1 – ident: e_1_2_6_5_2 – volume-title: Standard Methods for the Examination of Water and Wastewater year: 1998 ident: e_1_2_6_10_2 contributor: fullname: American Public Health Association, American Water Works Association and Water Environment Federation – ident: e_1_2_6_8_2 doi: 10.1016/j.chemosphere.2003.11.032 – ident: e_1_2_6_13_2 – volume-title: Ultrafiltration and Microfiltration Handbook year: 1986 ident: e_1_2_6_15_2 contributor: fullname: Cheryan M – ident: e_1_2_6_2_2 doi: 10.1016/0043-1354(92)90192-7 – volume: 25 start-page: 327 year: 1999 ident: e_1_2_6_7_2 article-title: Batch test for characterization of the carbonaceous materials in municipal wastewaters publication-title: Water SA contributor: fullname: Wentzel MC – volume: 45 start-page: 305 year: 2002 ident: e_1_2_6_6_2 article-title: Pre‐ or post ozonation application in activated sludge systems for a textile mill effluent publication-title: Water Sci Technol doi: 10.2166/wst.2002.0439 contributor: fullname: Orhon D – volume-title: Water Quality—Determination of the Chemical Oxygen Demand year: 1986 ident: e_1_2_6_11_2 – volume-title: Modelling of Activated Sludge Systems year: 1994 ident: e_1_2_6_4_2 contributor: fullname: Orhon D – ident: e_1_2_6_12_2 – ident: e_1_2_6_17_2 doi: 10.1016/0043-1354(91)90138-G – ident: e_1_2_6_14_2 doi: 10.1002/jctb.713 – ident: e_1_2_6_18_2 doi: 10.1016/S0043-1354(01)00273-1 – ident: e_1_2_6_9_2 article-title: Size distribution of wastewater COD fractions as an index for biodegradability publication-title: Water Res contributor: fullname: Dulekgurgen E – ident: e_1_2_6_20_2 doi: 10.1016/S0273-1223(98)00296-0 – volume: 44 start-page: 117 year: 2001 ident: e_1_2_6_19_2 article-title: On the need for engineering models of integrated chemical and biological oxidation of wastewaters publication-title: Water Sci Technol doi: 10.2166/wst.2001.0265 contributor: fullname: Ollis DF |
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| SubjectTerms | Applied sciences Chemical engineering chemical oxygen demand fractionation color profile Exact sciences and technology General purification processes Membrane separation (reverse osmosis, dialysis...) ozonation particle size distribution Pollution Reactors textile wastewaters ultrafiltration Wastewaters Water treatment and pollution |
| Title | Effect of ozonation on chemical oxygen demand fractionation and color profile of textile wastewaters |
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