On the regeneration of thermally regenerative ammonia batteries
In the past few years, thermally regenerative ammonia battery (TRAB) has been proposed as an effective tool to recover waste heat at temperatures below 130 °C. Most of the literature available is devoted to the power production step, with less attention being given to the regeneration step (e.g. the...
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| Published in: | Journal of applied electrochemistry Vol. 48; no. 12; pp. 1381 - 1388 |
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| Abstract | In the past few years, thermally regenerative ammonia battery (TRAB) has been proposed as an effective tool to recover waste heat at temperatures below 130 °C. Most of the literature available is devoted to the power production step, with less attention being given to the regeneration step (e.g. the removal of ammonia from the anolyte). In this paper, the TRAB is analyzed with particular attention to the regeneration step and to the study of various
generation of energy-regeneration
cycles. It was shown that approximately 90 °C is necessary for the regeneration step due to the fact that ammonia is present in the anolyte mainly as a complex. Various cycles were performed with success, demonstrating the efficacy of the proposed regeneration step.
Graphical abstract |
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| AbstractList | In the past few years, thermally regenerative ammonia battery (TRAB) has been proposed as an effective tool to recover waste heat at temperatures below 130 °C. Most of the literature available is devoted to the power production step, with less attention being given to the regeneration step (e.g. the removal of ammonia from the anolyte). In this paper, the TRAB is analyzed with particular attention to the regeneration step and to the study of various generation of energy-regeneration cycles. It was shown that approximately 90 °C is necessary for the regeneration step due to the fact that ammonia is present in the anolyte mainly as a complex. Various cycles were performed with success, demonstrating the efficacy of the proposed regeneration step.Graphical abstract In the past few years, thermally regenerative ammonia battery (TRAB) has been proposed as an effective tool to recover waste heat at temperatures below 130 °C. Most of the literature available is devoted to the power production step, with less attention being given to the regeneration step (e.g. the removal of ammonia from the anolyte). In this paper, the TRAB is analyzed with particular attention to the regeneration step and to the study of various generation of energy-regeneration cycles. It was shown that approximately 90 °C is necessary for the regeneration step due to the fact that ammonia is present in the anolyte mainly as a complex. Various cycles were performed with success, demonstrating the efficacy of the proposed regeneration step. Graphical abstract |
| Author | D’Angelo, Adriana Loffredi, Alessandro Galia, Alessandro Scialdone, Onofrio Vicari, Fabrizio Kouko, Yohan |
| Author_xml | – sequence: 1 givenname: Fabrizio surname: Vicari fullname: Vicari, Fabrizio organization: Department of Innovation, Industrial and Digital (DIID, Ingegneria Chimica, Gestionale, Informatica, Meccanica), Università degli Studi di Palermo – sequence: 2 givenname: Adriana surname: D’Angelo fullname: D’Angelo, Adriana organization: Department of Innovation, Industrial and Digital (DIID, Ingegneria Chimica, Gestionale, Informatica, Meccanica), Università degli Studi di Palermo – sequence: 3 givenname: Yohan surname: Kouko fullname: Kouko, Yohan organization: Department of Chemistry, Jean Perrin Faculty of Sciences, University of Artois – sequence: 4 givenname: Alessandro surname: Loffredi fullname: Loffredi, Alessandro organization: Department of Innovation, Industrial and Digital (DIID, Ingegneria Chimica, Gestionale, Informatica, Meccanica), Università degli Studi di Palermo – sequence: 5 givenname: Alessandro surname: Galia fullname: Galia, Alessandro organization: Department of Innovation, Industrial and Digital (DIID, Ingegneria Chimica, Gestionale, Informatica, Meccanica), Università degli Studi di Palermo – sequence: 6 givenname: Onofrio surname: Scialdone fullname: Scialdone, Onofrio email: onofrio.scialdone@unipa.it organization: Department of Innovation, Industrial and Digital (DIID, Ingegneria Chimica, Gestionale, Informatica, Meccanica), Università degli Studi di Palermo |
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| Keywords | TRAB Regeneration Thermally regenerative ammonia battery TREC Waste heat Ammonia–copper complex |
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| References_xml | – volume: 332416 start-page: 1 year: 1980 ident: CR5 article-title: Review of thermally regenerative electrochemical systems publication-title: Rep SERI/TR contributor: fullname: Osteryoung – volume: 322 start-page: 551 year: 2017 end-page: 556 ident: CR12 article-title: Removal of copper from water using a thermally regenerative electrodeposition battery publication-title: J Hazard Mater doi: 10.1016/j.jhazmat.2016.10.022 contributor: fullname: Zhu – volume: 9 start-page: 873 year: 2016 end-page: 879 ident: CR10 article-title: A thermally-regenerative ammonia-based flow battery for electrical energy recovery from waste heat publication-title: ChemSusChem doi: 10.1002/cssc.201501513 contributor: fullname: Logan – volume: 52 start-page: 6106 year: 2007 end-page: 6117 ident: CR13 article-title: Electrochemical study of binary and ternary copper complexes in ammonia-chloride medium publication-title: Electrochim Acta doi: 10.1016/j.electacta.2007.03.062 contributor: fullname: Cruz – volume: 8 start-page: 343 year: 2015 end-page: 349 ident: CR6 article-title: A thermally regenerative ammonia-based battery for efficient harvesting of low-grade thermal energy as electrical power publication-title: Energy Environ Sci doi: 10.1039/C4EE02824D contributor: fullname: Logan – ident: CR14 – volume: 351 start-page: 45 year: 2017 end-page: 50 ident: CR8 article-title: Electrical power production from low-grade waste heat using a thermally regenerative ethylenediamine battery publication-title: J Power Sources doi: 10.1016/j.jpowsour.2017.03.074 contributor: fullname: Gorski – volume: 8 start-page: 1043 year: 2015 end-page: 1048 ident: CR7 article-title: Enhancing low-grade thermal energy recovery in a thermally regenerative ammonia battery using elevated temperatures publication-title: ChemSusChem doi: 10.1002/cssc.201403290 contributor: fullname: Yang – volume: 5 start-page: 687 year: 1990 end-page: 688 ident: CR16 article-title: Lange’s handbook of chemistry publication-title: Mater Manuf Process doi: 10.1080/10426919008953291 contributor: fullname: Dean – volume: 2 start-page: 2326 year: 2017 end-page: 2334 ident: CR3 article-title: Thermally regenerative electrochemical cycle for low-grade heat harvesting publication-title: ACS Energy Lett doi: 10.1021/acsenergylett.7b00568 contributor: fullname: Yang – year: 2018 ident: CR2 article-title: Early mining and smelting lead anomalies in geological archives as potential stratigraphic markers for the base of an early Anthropocene publication-title: Anthr Rev doi: 10.1177/2053019618756682 contributor: fullname: Draganits – volume: 312 start-page: 193 year: 2005 end-page: 204 ident: CR15 article-title: Theoretical description of copper Cu(I)/Cu(II) complexes in mixed ammine-aqua environment. 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| SubjectTerms | Ammonia Anolytes Batteries Chemistry Chemistry and Materials Science Electrochemistry Industrial Chemistry/Chemical Engineering Physical Chemistry Regeneration Research Article Waste heat recovery |
| Title | On the regeneration of thermally regenerative ammonia batteries |
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