Use of kaolinite as adsorbent: Equilibrium, dynamics and thermodynamic studies on the adsorption of Rhodamine B from aqueous solution

The adsorption efficiency of kaolinite for Rhodamine B (RhB) removal from aqueous solution is reported. The optimized conditions for adsorption were evaluated as: initial concentration of RhB (90mg/L), agitation time (80min), adsorbent dose (3g/L), pH (7), and temperature (303K). The adsorption data...

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Bibliographic Details
Published in:	Applied clay science Vol. 69; pp. 58 - 66
Main Authors:	Khan, Tabrez A., Dahiya, Sarita, Ali, Imran
Format:	Journal Article
Language:	English
Published:	Kidlington Elsevier B.V 01-11-2012 Elsevier
Subjects:	Adsorption Dynamics Earth sciences Earth, ocean, space Exact sciences and technology Isotherms Kaolinite Mineralogy Rhodamine B Silicates Thermodynamics Thermodynamics Kaolinite Rhodamine B Adsorption Dynamics Isotherms models adsorption diffusion efficiency cost kaolinite aqueous solutions thermodynamics concentration isotherms entropy pH temperature clay minerals sheet silicates silicates equilibrium kinetics particles correlation coefficient
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Abstract	The adsorption efficiency of kaolinite for Rhodamine B (RhB) removal from aqueous solution is reported. The optimized conditions for adsorption were evaluated as: initial concentration of RhB (90mg/L), agitation time (80min), adsorbent dose (3g/L), pH (7), and temperature (303K). The adsorption data were evaluated using Langmuir, Temkin, Freundlich, Flory–Huggins and Dubinin–Kaganer–Radushkevich isothermal models, but high correlation coefficients (R2) confirmed the validity of Langmuir isotherm, with monolayer adsorption capacity (qm) equal to 46.08mg/g (83%). The kinetic data agreed well with pseudo-second order model with rate constants (K2) in the range 0.568–4.69×10−3g/mgmin. Diffusion studies indicated that intra-particle diffusion is not the sole rate-controlling factor. The thermodynamic parameters indicated that adsorption of RhB onto kaolinite was spontaneous, endothermic, and the entropy increased during adsorption. The study revealed that kaolinite can be utilized as an efficient low-cost adsorbent for decolorization of wastewater containing RhB dye. ► Kaolinite is used as an adsorbent for Rhodamine B dye removal from aqueous solution. ► The data followed Langmuir and Temkin isotherms, suggesting monolayer adsorption. ► Adsorption data obeyed pseudo-second order kinetics. ► The adsorption rate was controlled by both liquid-film and intra-particle diffusion. ► Results proved the kaolinite to be promising adsorbent for rhodamine B uptake.
AbstractList	The adsorption efficiency of kaolinite for Rhodamine B (RhB) removal from aqueous solution is reported. The optimized conditions for adsorption were evaluated as: initial concentration of RhB (90mg/L), agitation time (80min), adsorbent dose (3g/L), pH (7), and temperature (303K). The adsorption data were evaluated using Langmuir, Temkin, Freundlich, Flory–Huggins and Dubinin–Kaganer–Radushkevich isothermal models, but high correlation coefficients (R2) confirmed the validity of Langmuir isotherm, with monolayer adsorption capacity (qm) equal to 46.08mg/g (83%). The kinetic data agreed well with pseudo-second order model with rate constants (K2) in the range 0.568–4.69×10−3g/mgmin. Diffusion studies indicated that intra-particle diffusion is not the sole rate-controlling factor. The thermodynamic parameters indicated that adsorption of RhB onto kaolinite was spontaneous, endothermic, and the entropy increased during adsorption. The study revealed that kaolinite can be utilized as an efficient low-cost adsorbent for decolorization of wastewater containing RhB dye. ► Kaolinite is used as an adsorbent for Rhodamine B dye removal from aqueous solution. ► The data followed Langmuir and Temkin isotherms, suggesting monolayer adsorption. ► Adsorption data obeyed pseudo-second order kinetics. ► The adsorption rate was controlled by both liquid-film and intra-particle diffusion. ► Results proved the kaolinite to be promising adsorbent for rhodamine B uptake.
Author	Ali, Imran Dahiya, Sarita Khan, Tabrez A.
Author_xml	– sequence: 1 givenname: Tabrez A. surname: Khan fullname: Khan, Tabrez A. email: takhan501@yahoo.com – sequence: 2 givenname: Sarita surname: Dahiya fullname: Dahiya, Sarita – sequence: 3 givenname: Imran surname: Ali fullname: Ali, Imran
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Keywords	Thermodynamics Kaolinite Rhodamine B Adsorption Dynamics Isotherms models adsorption diffusion efficiency cost kaolinite aqueous solutions thermodynamics concentration isotherms entropy pH temperature clay minerals sheet silicates silicates equilibrium kinetics particles correlation coefficient
Language	English
License	CC BY 4.0
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PublicationDate	2012-11-01
PublicationDateYYYYMMDD	2012-11-01
PublicationDate_xml	– month: 11 year: 2012 text: 2012-11-01 day: 01
PublicationDecade	2010
PublicationPlace	Kidlington
PublicationPlace_xml	– name: Kidlington
PublicationTitle	Applied clay science
PublicationYear	2012
Publisher	Elsevier B.V Elsevier
Publisher_xml	– name: Elsevier B.V – name: Elsevier
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Snippet	The adsorption efficiency of kaolinite for Rhodamine B (RhB) removal from aqueous solution is reported. The optimized conditions for adsorption were evaluated...
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SubjectTerms	Adsorption Dynamics Earth sciences Earth, ocean, space Exact sciences and technology Isotherms Kaolinite Mineralogy Rhodamine B Silicates Thermodynamics
Title	Use of kaolinite as adsorbent: Equilibrium, dynamics and thermodynamic studies on the adsorption of Rhodamine B from aqueous solution
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