COPROX Fixed Bed Reactor - Temperature Control Schemes
Different temperature control schemes for the COPROX stage of a 5‐kW fuel cell system were analyzed. It was found that, among the schemes proposed, i.e., co‐ and countercurrent heat exchange, single adiabatic reactor and series of adiabatic reactors with interstage heat exchange, the best choice for...
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| Published in: | Chemical engineering & technology Vol. 35; no. 6; pp. 1055 - 1063 |
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| Main Authors: | , , , , |
| Format: | Journal Article Conference Proceeding |
| Language: | English |
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Weinheim
WILEY-VCH Verlag
01-06-2012
WILEY‐VCH Verlag Wiley-VCH |
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| Abstract | Different temperature control schemes for the COPROX stage of a 5‐kW fuel cell system were analyzed. It was found that, among the schemes proposed, i.e., co‐ and countercurrent heat exchange, single adiabatic reactor and series of adiabatic reactors with interstage heat exchange, the best choice for temperature control was the series of adiabatic reactors with interstage heat exchange. This scheme represented the best way to keep the average temperature around 443 K, which was found to be the most suitable temperature for selectivity towards CO oxidation. If hydrogen is produced from ethanol steam reforming, the heat withdrawal can be carried out by the water/ethanol reformer feed mixture, thus contributing to the energy integration of the overall system.
Preferential oxidation of CO with a Cu/CeO2 catalyst was employed to reduce the CO content to less than 20 ppm in a hydrogen stream obtained from hydrocarbons or alcohols. Temperature control is a key issue to achieve high CO conversion and simultaneously to avoid the oxidation of hydrogen. Heat transfer alternatives in a fixed bed reactor are analyzed and discussed. |
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| AbstractList | Different temperature control schemes for the COPROX stage of a 5‐kW fuel cell system were analyzed. It was found that, among the schemes proposed, i.e., co‐ and countercurrent heat exchange, single adiabatic reactor and series of adiabatic reactors with interstage heat exchange, the best choice for temperature control was the series of adiabatic reactors with interstage heat exchange. This scheme represented the best way to keep the average temperature around 443 K, which was found to be the most suitable temperature for selectivity towards CO oxidation. If hydrogen is produced from ethanol steam reforming, the heat withdrawal can be carried out by the water/ethanol reformer feed mixture, thus contributing to the energy integration of the overall system.
Preferential oxidation of CO with a Cu/CeO2 catalyst was employed to reduce the CO content to less than 20 ppm in a hydrogen stream obtained from hydrocarbons or alcohols. Temperature control is a key issue to achieve high CO conversion and simultaneously to avoid the oxidation of hydrogen. Heat transfer alternatives in a fixed bed reactor are analyzed and discussed. Different temperature control schemes for the COPROX stage of a 5‐kW fuel cell system were analyzed. It was found that, among the schemes proposed, i.e., co‐ and countercurrent heat exchange, single adiabatic reactor and series of adiabatic reactors with interstage heat exchange, the best choice for temperature control was the series of adiabatic reactors with interstage heat exchange. This scheme represented the best way to keep the average temperature around 443 K, which was found to be the most suitable temperature for selectivity towards CO oxidation. If hydrogen is produced from ethanol steam reforming, the heat withdrawal can be carried out by the water/ethanol reformer feed mixture, thus contributing to the energy integration of the overall system. |
| Author | Amadeo, N. Mariño, F. Lobarde, M. Giunta, P. Moreno, M. |
| Author_xml | – sequence: 1 givenname: P. surname: Giunta fullname: Giunta, P. organization: Laboratorio de Procesos Catalíticos, Facultad de Ingeniería, Universidad de Buenos Aires, Buenos Aires, Argentina – sequence: 2 givenname: M. surname: Moreno fullname: Moreno, M. organization: Laboratorio de Procesos Catalíticos, Facultad de Ingeniería, Universidad de Buenos Aires, Buenos Aires, Argentina – sequence: 3 givenname: F. surname: Mariño fullname: Mariño, F. email: fernando@di.fcen.uba.ar organization: Laboratorio de Procesos Catalíticos, Facultad de Ingeniería, Universidad de Buenos Aires, Buenos Aires, Argentina – sequence: 4 givenname: N. surname: Amadeo fullname: Amadeo, N. organization: Laboratorio de Procesos Catalíticos, Facultad de Ingeniería, Universidad de Buenos Aires, Buenos Aires, Argentina – sequence: 5 givenname: M. surname: Lobarde fullname: Lobarde, M. organization: Laboratorio de Procesos Catalíticos, Facultad de Ingeniería, Universidad de Buenos Aires, Buenos Aires, Argentina |
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| Keywords | Fixed bed reactor Adiabatic Oxidation Steam reforming Temperature control Countercurrent flow Fuel cell |
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| Snippet | Different temperature control schemes for the COPROX stage of a 5‐kW fuel cell system were analyzed. It was found that, among the schemes proposed, i.e., co‐... |
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| SubjectTerms | Applied sciences Chemical engineering Chemical reactors CO preferential oxidation Energy Energy. Thermal use of fuels Equipments for energy generation and conversion: thermal, electrical, mechanical energy, etc Exact sciences and technology Fuel cells Heat transfer Reactor design Reactor modeling Reactors |
| Title | COPROX Fixed Bed Reactor - Temperature Control Schemes |
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