Fe-substituted Mn-based Prussian white as cathode for high-performance potassium-ion battery
Prussian white (PW) has a stable three-dimensional frame structure and large ion migration channels, which has been widely studied as the cathode materials for potassium-ion batteries (PIB) in recent years. The multi-composition in PWs has a great impact on the electrochemical performance as cathode...
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| Published in: | Journal of materials science Vol. 57; no. 29; pp. 14015 - 14025 |
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| Main Authors: | , , , , , |
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| Abstract | Prussian white (PW) has a stable three-dimensional frame structure and large ion migration channels, which has been widely studied as the cathode materials for potassium-ion batteries (PIB) in recent years. The multi-composition in PWs has a great impact on the electrochemical performance as cathode materials. In this work, we investigated the relationship between Fe substitution content and electrochemical properties. The sample of PW with 10%Fe substitution shows the overall optimum electrochemical performance, which delivers a high reversible capacity of 124.3 mAh g
−1
and capacity retention of 70.0% after 200 cycles at 100 mA g
−1
, as well as 77.5 mAh g
−1
at a large current density of 500 mA g
−1
. Actually, partial Fe substitution could effectively stabilize the lattice structure and improve electrochemical properties. This work provides a practical strategy to synthesize PWs with stable crystal structure and preferable performance, which could serve as a reference for the electrochemical improvement of electrode materials.
Graphical Abstract |
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| AbstractList | Prussian white (PW) has a stable three-dimensional frame structure and large ion migration channels, which has been widely studied as the cathode materials for potassium-ion batteries (PIB) in recent years. The multi-composition in PWs has a great impact on the electrochemical performance as cathode materials. In this work, we investigated the relationship between Fe substitution content and electrochemical properties. The sample of PW with 10%Fe substitution shows the overall optimum electrochemical performance, which delivers a high reversible capacity of 124.3 mAh g.sup.-1 and capacity retention of 70.0% after 200 cycles at 100 mA g.sup.-1, as well as 77.5 mAh g.sup.-1 at a large current density of 500 mA g.sup.-1. Actually, partial Fe substitution could effectively stabilize the lattice structure and improve electrochemical properties. This work provides a practical strategy to synthesize PWs with stable crystal structure and preferable performance, which could serve as a reference for the electrochemical improvement of electrode materials. Graphical Prussian white (PW) has a stable three-dimensional frame structure and large ion migration channels, which has been widely studied as the cathode materials for potassium-ion batteries (PIB) in recent years. The multi-composition in PWs has a great impact on the electrochemical performance as cathode materials. In this work, we investigated the relationship between Fe substitution content and electrochemical properties. The sample of PW with 10%Fe substitution shows the overall optimum electrochemical performance, which delivers a high reversible capacity of 124.3 mAh g −1 and capacity retention of 70.0% after 200 cycles at 100 mA g −1 , as well as 77.5 mAh g −1 at a large current density of 500 mA g −1 . Actually, partial Fe substitution could effectively stabilize the lattice structure and improve electrochemical properties. This work provides a practical strategy to synthesize PWs with stable crystal structure and preferable performance, which could serve as a reference for the electrochemical improvement of electrode materials. Graphical Abstract Prussian white (PW) has a stable three-dimensional frame structure and large ion migration channels, which has been widely studied as the cathode materials for potassium-ion batteries (PIB) in recent years. The multi-composition in PWs has a great impact on the electrochemical performance as cathode materials. In this work, we investigated the relationship between Fe substitution content and electrochemical properties. The sample of PW with 10%Fe substitution shows the overall optimum electrochemical performance, which delivers a high reversible capacity of 124.3 mAh g.sup.-1 and capacity retention of 70.0% after 200 cycles at 100 mA g.sup.-1, as well as 77.5 mAh g.sup.-1 at a large current density of 500 mA g.sup.-1. Actually, partial Fe substitution could effectively stabilize the lattice structure and improve electrochemical properties. This work provides a practical strategy to synthesize PWs with stable crystal structure and preferable performance, which could serve as a reference for the electrochemical improvement of electrode materials. Prussian white (PW) has a stable three-dimensional frame structure and large ion migration channels, which has been widely studied as the cathode materials for potassium-ion batteries (PIB) in recent years. The multi-composition in PWs has a great impact on the electrochemical performance as cathode materials. In this work, we investigated the relationship between Fe substitution content and electrochemical properties. The sample of PW with 10%Fe substitution shows the overall optimum electrochemical performance, which delivers a high reversible capacity of 124.3 mAh g−1 and capacity retention of 70.0% after 200 cycles at 100 mA g−1, as well as 77.5 mAh g−1 at a large current density of 500 mA g−1. Actually, partial Fe substitution could effectively stabilize the lattice structure and improve electrochemical properties. This work provides a practical strategy to synthesize PWs with stable crystal structure and preferable performance, which could serve as a reference for the electrochemical improvement of electrode materials. |
| Audience | Academic |
| Author | Zhang, Kaicheng Fang, Xiangpeng Xiong, Yuli Jian, Zelang Xia, Yang Chen, Xuanjin |
| Author_xml | – sequence: 1 givenname: Xuanjin surname: Chen fullname: Chen, Xuanjin organization: State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, School of Materials Science and Engineering, Wuhan University of Technology – sequence: 2 givenname: Yang surname: Xia fullname: Xia, Yang organization: State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, School of Materials Science and Engineering, Wuhan University of Technology – sequence: 3 givenname: Xiangpeng surname: Fang fullname: Fang, Xiangpeng organization: Sichuan Shenghonghui New Energy Technology Co., Ltd – sequence: 4 givenname: Kaicheng surname: Zhang fullname: Zhang, Kaicheng organization: State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, School of Materials Science and Engineering, Wuhan University of Technology – sequence: 5 givenname: Yuli surname: Xiong fullname: Xiong, Yuli organization: State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, School of Materials Science and Engineering, Wuhan University of Technology – sequence: 6 givenname: Zelang orcidid: 0000-0003-1866-8474 surname: Jian fullname: Jian, Zelang email: zelangjian@whut.edu.cn organization: State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, School of Materials Science and Engineering, Wuhan University of Technology |
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| SubjectTerms | Batteries Cathodes Characterization and Evaluation of Materials Chemistry and Materials Science Classical Mechanics Crystal structure Crystallography and Scattering Methods Crystals Dimensional stability Electrochemical analysis Electrode materials Energy Materials Frame structures Ion migration Manganese Materials Science Materials substitution Polymer Sciences Potassium Rechargeable batteries Solid Mechanics Structure |
| Title | Fe-substituted Mn-based Prussian white as cathode for high-performance potassium-ion battery |
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